English

Rethinking $\alpha$-RuCl$_3$

Strongly Correlated Electrons 2020-07-06 v4 Materials Science

Abstract

We argue that several empirical constraints strongly restrict parameters of the effective microscopic spin model describing α\alpha-RuCl3_3. In particular, such constraints dictate a substantial \emph{positive} off-diagonal anisotropic coupling, Γ ⁣> ⁣0\Gamma^\prime\!>\!0, not anticipated previously. The renormalization by quantum fluctuations allows to reconcile larger values of the advocated bare parameters with their earlier assessments and provides a consistent description of the field evolution of spin excitations in the paramagnetic phase. We assert that large anisotropic terms inevitably result in strong anharmonic coupling of magnons, necessarily leading to broad features in their spectra due to decays, in accord with the observations in α\alpha-RuCl3_3. Using duality transformations, we explain the origin of the pseudo-Goldstone mode that is ubiquitous to the studied parameter space and is present in α\alpha-RuCl3_3. Our analysis offers a description of α\alpha-RuCl3_3 as an easy-plane ferromagnet with antiferromagnetic further-neighbor and strong off-diagonal couplings, which is in a fluctuating zigzag ground state proximate to an incommensurate phase that is continuously connected to a ferromagnetic one.

Keywords

Cite

@article{arxiv.2004.10753,
  title  = {Rethinking $\alpha$-RuCl$_3$},
  author = {P. A. Maksimov and A. L. Chernyshev},
  journal= {arXiv preprint arXiv:2004.10753},
  year   = {2020}
}

Comments

As accepted to Phys. Rev. of Rethinking (PRR). Typos in Appendix fixed, award-winning acknowledgements

R2 v1 2026-06-23T15:02:05.748Z