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We perform Raman spectroscopy studies on $\alpha$-RuCl$_3$ at room temperature to explore its phase transitions of magnetism and chemical bonding under pressures. The Raman measurements resolve two critical pressures, about $p_1=1.1$~GPa…

We performed 23Na NMR measurements on a single-domain crystal of the Kitaev material Na3Co2SbO6, with magnetic field applied along the crystalline a axis. A positive Curie-Weiss constant is obtained from the NMR Knight shift, which suggests…

Strongly Correlated Electrons · Physics 2024-02-14 Ze Hu , Yue Chen , Yi Cui , Shuo Li , Cong Li , Xiaoyu Xu , Ying Chen , Xintong Li , Yuchen Gu , Rong Yu , Rui Zhou , Yuan Li , Weiqiang Yu

The 2D layered insulator $\alpha$-RuCl$_3$ is a candidate material for a quantum spin-liquid state, which may be realized when a magnetic field suppresses the antiferromagnetic order present at low temperature. Oscillations in the field…

Strongly Correlated Electrons · Physics 2023-02-10 Étienne Lefrançois , Jordan Baglo , Quentin Barthélemy , Subin Kim , Young-June Kim , Louis Taillefer

$\alpha$-RuCl$_3$ is a Mott insulator with a honeycomb lattice with strong spin-orbit coupling. We report dielectric measurements on $\alpha$-RuCl$_3$ single crystals under field. At zero field, the dielectric constant, $\epsilon$, drops…

Strongly Correlated Electrons · Physics 2018-02-20 Jia-Cheng Zheng , Yi Cui , Tian-Run Li , Ke-Jing Ran , Jinsheng Wen , Weiqiang Yu

The frustrated magnet $\alpha$-RuCl3 is one of the prime candidates for realizing a Kitaev quantum spin liquid (QSL). However, the existence of a field-induced intermediate QSL phase in this material remains under debate. Here, we employ…

Strongly Correlated Electrons · Physics 2025-10-07 Xuan Zou , Shuo Liu , Wenan Guo , Hong Yao

Motivated by the largely unexplored domain of multi-polar ordered spin states in the Kitaev-Heisenberg (KH) systems we investigate the ground state dynamics of the spin-$\frac{1}{2}$ KH model, focusing on quadrupolar (QP) order in 2-leg…

Strongly Correlated Electrons · Physics 2025-03-28 Manodip Routh , Sayan Ghosh , Jeroen van den Brink , Satoshi Nishimoto , Manoranjan Kumar

The quasi two-dimensional Mott insulator $\alpha$-RuCl$_3$ is proximate to the sought-after Kitaev quantum spin liquid (QSL). In a layer of $\alpha$-RuCl$_3$ on graphene the dominant Kitaev exchange is further enhanced by strain. Recently,…

Strongly Correlated Electrons · Physics 2021-03-24 V. Leeb , K. Polyudov , S. Mashhadi , S. Biswas , Roser Valenti , M. Burghard , J. Knolle

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

The unconventional electronic ground state of Sr$_3$IrRuO$_7$ is explored via resonant x-ray scattering techniques and angle-resolved photoemission measurements. As the Ru content approaches $x=0.5$ in Sr$_3$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$,…

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6…

Polycrystalline samples of NaYbO$_2$ are investigated by bulk magnetization and specific-heat measurements, as well as by nuclear magnetic resonance (NMR) and electron spin resonance (ESR) as local probes. No signatures of long-range…

Strongly Correlated Electrons · Physics 2019-05-08 K. M. Ranjith , D. Dmytriieva , S. Khim , J. Sichelschmidt , S. Luther , D. Ehlers , H. Yasuoka , J. Wosnitza , A. A. Tsirlin , H. Kühne , M. Baenitz

Inspired by experiments on the magnetic field induced phases of the spin-orbit coupled $2d$ Mott insulator $\alpha$-RuCl$_3$, we study some general aspects of gapped $Z_2$ Quantum Spin Liquids (QSL) enriched by lattice translation symmetry.…

Strongly Correlated Electrons · Physics 2022-07-25 Xue-Yang Song , T. Senthil

Magnetization and high-resolution x-ray diffraction measurements of the Kitaev-Heisenberg material alpha-RuCl3 reveal a pressure-induced crystallographic and magnetic phase transition at a hydrostatic pressure of p=0.2 GPa. This structural…

KCuCl$_3$ is a three-dimensional coupled spin-dimer system and has a singlet ground state with an excitation gap ${\Delta}/k_{\rm B}=31$ K. High-field magnetization measurements for KCuCl$_3$ have been performed in static magnetic fields of…

Strongly Correlated Electrons · Physics 2009-11-07 A. Oosawa , T. Takamasu , K. Tatani , H. Abe , N. Tsujii , O. Suzuki , H. Tanaka , G. Kido , K. Kindo

The majority of research on $\alpha$-RuCl$_3$ has focused on applying in-plane magnetic fields to suppress antiferromagnetic order and induce a quantum spin liquid (QSL). However, this effort has been complicated by the materials…

Strongly Correlated Electrons · Physics 2026-05-14 Hamza Nasir Daniel Balazs , Muhammad Nauman , Ezekiel Horsley , Subin Kim , Young-June Kim , K. A. Modic

We study the effect of bond disorder in extended Heisenberg-Kitaev models on the honeycomb lattice, relevant for materials such as $\alpha$-RuCl$_3$, in the semiclassical limit using a combination of T-matrix and real-space spin-wave…

Strongly Correlated Electrons · Physics 2024-11-27 Georgia Fragkopoulou , Matthias Vojta

The material $\alpha$-RuCl$_3$ has been the subject of intense scrutiny as a potential Kitaev quantum spin liquid, predicted to display Majorana fermions as low energy excitations. In practice, $\alpha$-RuCl$_3$ undergoes a transition to a…

Measurements of the magnetic Gr\"uneisen parameter ($\Gamma_B$) and specific heat on the Kitaev material candidate $\alpha$-RuCl$_3$ are used to access in-plane field- and temperature-dependence of the entropy up to 12 T and down to 1 K. No…

Strongly Correlated Electrons · Physics 2020-08-28 S. Bachus , D. A. S. Kaib , Y. Tokiwa , A. Jesche , V. Tsurkan , A. Loidl , S. M. Winter , A. A. Tsirlin , R. Valenti , P. Gegenwart

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…