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The electronic structure of V2O3 thin films is studied by means of the augmented spherical wave method as based on density functional theory and the local density approximation. We establish that effects of charge redistribution, induced by…

Strongly Correlated Electrons · Physics 2009-09-22 Udo Schwingenschloegl , Raymond Fresard , Volker Eyert

The material BaBiO$_{3}$ is known for its insulating character. However, for thin films, in the ultra-thin limit, metallicity is expected because BaBiO$_{3}$ is suggested to return to its undistorted cubic phase where the oxygen octahedra…

Strongly Correlated Electrons · Physics 2021-04-01 Rosa Luca Bouwmeester , Alexander Brinkman , Kai Sotthewes

The nature of the metal insulator transition in thin films and superlattices of LaNiO3 with only few unit cells in thickness remains elusive despite tremendous effort. Quantum confinement and epitaxial strain have been evoked as the…

Precise control of the chemical valence or oxidation state of vanadium in vanadium oxide thin films is highly desirable for not only fundamental research, but also technological applications that utilize the subtle change in the physical…

Materials Science · Physics 2015-06-23 Shinbuhm Lee , Tricia L. Meyer , Sungkyun Park , Takeshi Egami , Ho Nyung Lee

Metal mixed polymers are a cheap and effective way to produce flexible metals and superconductors. As part of an on-going effort to learn how to tune the properties of these systems with ion implantation, we present a study of the…

Materials Science · Physics 2009-06-15 Andrew P. Stephenson , Ujjual Divakar , Adam P. Micolich , Paul Meredith , Ben J. Powell

Correlated electrons in transition metal oxides (TMOs) exhibit a variety of emergent phases. When TMOs are confined to a single-atomic-layer thickness, experiments so far have shown that they usually lose diverse properties and become…

With the motive of unraveling the origin of native vacancy induced magnetization in ferroelectric perovskite oxide systems, here we explore the consequences of electronic structure modification in magnetic ordering of oxygen deficient…

Correlated electron materials (CEMs) host a rich variety of condensed matter phases. Vanadium dioxide (VO2) is a prototypical CEM with a temperature-dependent metal-to-insulator (MIT) transition with a concomitant crystal symmetry change.…

We calculate the properties of the 4$d$ ferromagnet SrRuO$_3$ in bulk and thin film form with the aim of understanding the experimentally observed metal to insulator transition at reduced thickness. Although the spatial extent of the 4$d$…

Materials Science · Physics 2008-10-08 James M. Rondinelli , Nuala M. Caffrey , Stefano Sanvito , Nicola A. Spaldin

Based on the Hubbard model of strongly correlated systems, a reduction in the bandwidth of the electrons can yield a substantial change in the properties of the material. One method to modify the bandwidth is geometrically confined doping,…

Strongly Correlated Electrons · Physics 2009-12-21 U. Luders , W. C. Sheets , A. David , W. Prellier , R. Fresard

Ultrathin two-dimensional (2D) electronic systems at the interfaces of layered materials are highly desirable platforms for exploring of novel quantum phenomena and developing advanced device applications. Here, we investigate ultrathin…

Mesoscale and Nanoscale Physics · Physics 2025-03-31 Zengxing Lu , Jiatai Feng , Xuan Zheng , You-guo Shi , Run-Wei Li , Carmine Autieri , Mario Cuoco , Milan Radovic , Zhiming Wang

An electronic effect on a macroscopic domain structure is found in a strongly correlated half-doped manganite film Nd$_{0.5}$Sr$_{0.5}$MnO3 grown on a (011) surface of SrTiO3. The sample has a high-temperature (HT) phase free from…

Strongly Correlated Electrons · Physics 2011-03-01 Y. Wakabayashi , H. Sagayama , T. Arima , M. Nakamura , Y. Ogimoto , Y. Kubo , K. Miyano , H. Sawa

Vanadium sesquioxide (V2O3) is an archetypal Mott insulator in which the atomic positions and electron correlations change as temperature, pressure or doping are varied giving rise to different structural, magnetic or electronic phase…

Strongly Correlated Electrons · Physics 2024-06-12 P. Homm , M. Menghini , J. W. Seo , S. Peters , J. -P. Locquet

High quality vanadium sesquioxide V2O3 films (170-1100 {\AA}) were grown using the pulsed laser deposition technique on (0001)-oriented sapphire substrates, and the effects of film thickness on the lattice strain and electronic properties…

Strongly Correlated Electrons · Physics 2008-01-07 C. Grygiel , Ch. Simon , B. Mercey , W. Prellier , P. Limelette , R. Fresard

Emergent phenomena at polar-nonpolar oxide interfaces have been studied intensely in pursuit of next-generation oxide electronics and spintronics. Here we report the disentanglement of critical thicknesses for electron reconstruction and…

We report a theoretical study of the effects of electron correlations and structural confinement on the electronic properties and magnetic state of LaNiO3 (LNO) thin films epitaxially deposited on the (001) LaAlO3 (LAO) substrate. Using the…

Strongly Correlated Electrons · Physics 2024-02-01 N. O. Vambold , G. A. Sazhaev , I. V. Leonov

Symmetry-lowering structural phase transitions result in multiple degenerate structures whose coexistence is determined by macroscopic strain compatibility. In quantum materials, these structural transformations often couple to electronic…

The electrodynamics near the metal-to-insulator transitions (MIT) induced, in V3O5 single crystals, by both temperature (T) and pressure (P) has been studied by infrared spectroscopy. The T- and P-dependence of the optical conductivity may…

Strongly Correlated Electrons · Physics 2009-11-13 L. Baldassarre , A. Perucchi , E. Arcangeletti , D. Nicoletti , D. Di Castro , P. Postorino , V. A. Sidorov , S. Lupi

WO$_3$ is a binary 5d compound which has attracted remarkable attention due to the vast array of structural transitions that it undergoes in its bulk form. In the bulk, a wide range of electronic properties has been demonstrated, including…

Micrometric domains of precise ferroelectric polarization have been written into a 20 nm thick epitaxial thin film of BaTiO3(001) (BTO) on a Nb doped SrTiO3 (STO) substrate using PiezoForce Microscopy (PFM). The domain dependent electronic…

Materials Science · Physics 2018-06-06 N. Barrett , J. Rault , I. Krug , B. Vilquin , G. Niu , B. Gautier , D. Albertini , O. Renault