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Temporal correlations in pulsed electron beams reflect the microscopic dynamics of emission and interparticle interaction. In femtosecond electron emission from nanoscale field emitters, Coulomb interactions result in structured…

Mesoscale and Nanoscale Physics · Physics 2025-05-16 Rudolf Haindl , Valerio Di Giulio , Armin Feist , Claus Ropers

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

We demonstrate by time-resolved resonance fluorescence measurements on a single self-assembled quantum dot an internal photo-effect that emits electrons from the dot by an intra-band excitation. We find a linear dependence of the optically…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Pia Lochner , Jens Kerski , Annika Kurzmann , Andreas D. Wieck , Arne Ludwig , Martin Geller , Axel Lorke

Recent experimental techniques in multicolor waveform synthesis allow the temporal shaping of strong femtosecond laser pulses with applications in the control of quantum mechanical processes in atoms, molecules, and nanostructures.…

Atomic Physics · Physics 2017-10-11 Janne Solanpää , Marcelo F. Ciappina , Esa Räsänen

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

The extreme ultraviolet absorption spectrum of an atom is strongly modified in the presence of a synchronized intense infrared field. In this work we demonstrate control of the absorption properties of helium atoms dressed by an infrared…

A fundamental issue that limits the efficiency of many photoelectrochemical systems is that the photon absorption length is typically much longer than the electron diffusion length. Various photon management schemes have been developed to…

Single-cycle optical pulses with a controlled electromagnetic waveform allow to steer the motion of low-energy electrons in atoms, molecules, nanostructures or condensed-matter on attosecond dimensions in time. However, high-energy…

Optics · Physics 2020-11-11 Yuya Morimoto , Peter Baum

Ionization by relativistically intense laser pulses of finite duration is considered in the framework of strong-field quantum electrodynamics. Our main focus is on the formation of ionization supercontinua. More specifically, when studying…

Atomic Physics · Physics 2016-07-13 K. Krajewska , J. Z. Kamiński

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

We investigate the coherent control of the photo\-electron angular distribution in bichromatic atomic ionization. Neon is selected as target since it is one of the most popular systems in current gas-phase experiments with free-electron…

Atomic Physics · Physics 2018-01-31 E. V. Gryzlova , A. N. Grum-Grzhimailo , E. I. Staroselskaya , N. Douguet , K. Bartschat

Photoionization using attosecond pulses can lead to the formation of coherent superpositions of the electronic states of the parent ion. However, ultrafast electron ejection triggers not only electronic but also nuclear dynamics---leading…

Chemical Physics · Physics 2017-03-29 Caroline Arnold , Oriol Vendrell , Robin Santra

We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct…

Amplitude and phase of wavepackets encode the dynamics of quantum systems. However, the rapidity of electron dynamics on the attosecond timescale has precluded their complete measurement in the time domain. Here, we demonstrate that…

Attosecond pump-probe ionization process can be used to prepare atomic ions in the coherent superposition of states with opposite parity. The multiphoton shake-up ionization of Helium, in particular, generates ions with same principal…

Atomic Physics · Physics 2019-12-12 Saad Mehmood , Eva Lindroth , Luca Argenti

In this paper we explain the photoelectric effect in a variant of the standard model of non relativistic quantum electrodynamics, which is in some aspects more closely related to the physical picture, than the one studied in [BKZ]: Now we…

Mathematical Physics · Physics 2008-11-26 Heribert Zenk

We experimentally investigate the effects of the linear photon momentum on the momentum distributions of photoions and photoelectrons generated in one-photon ionization in an energy range of 300 eV $\leq~E_\gamma~\leq$ 40 keV. Our results…

Using the recently developed concept of the 2-electron streak camera (see NJP 12, 103024 (2010)), we have studied the energy-sharing between the two ionizing electrons in single-photon double ionization of He(1s2s). We find that the most…

Atomic Physics · Physics 2015-05-28 H. Price , A. Staudte , A. Emmanouilidou

We study theoretically single electron loss from helium-like highly charged ions involving excitation and decay of autoionizing states of the ion. Electron loss is caused by either photo absorption or the interaction with a fast atomic…

Atomic Physics · Physics 2017-11-15 K. N. Lyashchenko , O. Yu. Andreev , A. B. Voitkiv