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We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…

Optics · Physics 2017-11-22 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

The two opposite concepts - multiphoton and effective photon - readily describing the photoelectric effect under strong irradiation in the case that the energy of the incident light is essentially smaller than the ionisation potential of…

Quantum Physics · Physics 2007-05-23 Volodymyr Krasnoholovets

Electron capture by {\it isolated} atoms and ions proceeds by photorecombination. In this process a species captures a free electron by emitting a photon which carries away the excess energy. It is shown here that in the presence of an {\it…

Quantum Physics · Physics 2010-03-18 Kirill Gokhberg , Lorenz S. Cederbaum

Photoelectron spectra and photoelectron angular distributions obtained in photoionization reveal important information on e.g. charge transfer or hole coherence in the parent ion. Here we show that optimal control of the underlying quantum…

Atomic Physics · Physics 2016-01-20 R. Esteban Goetz , Antonia Karamatskou , Robin Santra , Christiane P. Koch

Autoionization, which results from the interference between direct photoionization and photoexcitation to a discrete state decaying to the continuum by configuration interaction, is a well known example of the important role of electron…

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons. Except of the already…

Atomic Physics · Physics 2018-03-14 F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

We analyze two-photon double ionization of helium in both the nonsequential and sequential regime. We show that the energy spacing between the two emitted electrons provides the key parameter that controls both the energy and the angular…

Atomic Physics · Physics 2013-05-24 R. Pazourek , J. Feist , S. Nagele , E. Persson , B. I. Schneider , L. A. Collins , J. Burgörfer

We investigate the effect of dynamic electron correlation on high-harmonic generation in helium atoms using intense visible light (\lambda=390nm). Two complementary approaches are used which account for correlation in an approximate manner:…

Quantum Physics · Physics 2009-05-21 G. A. McKenna , R. Nepstad , J. F. McCann , D. Dundas

The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…

Atomic Physics · Physics 2008-02-27 J. Mauritsson , P. Johnsson , E. Gustafsson , M. Swoboda , T. Ruchon , A. LHuillier , K. J. Schafer

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We calculate the photoionization with excitation-to photoionization ratios for atomic helium and heliumlike ions at intermediate values of the photon energies. The final state interactions between the electrons are included in the lowest…

Quantum Physics · Physics 2009-11-13 E. G. Drukarev , E. Z. Liverts , M. Ya. Amusia , R. Krivec , V. B. Mandelzweig

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

Atomic Physics · Physics 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We calculate the distributions in recoil momenta and their energy distributions for the high energy non-relativistic double photoionization of helium caused by the quasifree mechanism of the process. The distributions obtain local maxima at…

Atomic Physics · Physics 2013-03-06 M. Ya. Amusia , E. G. Drukarev , E. Z. Liverts , A. I. Mikhailov

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…

We investigate the angle-resolved photoelectron spectra from laser-assisted photoionization for helium and neon atoms using an \textit{ab initio} method based on time-dependent surface flux and configuration interaction singles. We find…

Atomic Physics · Physics 2020-08-26 Mattias Bertolino , David Busto , Felipe Zapata , Jan Marcus Dahlström

Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…

Atomic Physics · Physics 2016-05-30 Paul Hockett , Matthias Wollenhaupt , Thomas Baumert

We report on the observation of phase space modulations in the correlated electron emission after strong field double ionization of helium using laser pulses with a wavelength of 394~nm and an intensity of $3\cdot10^{14}$W/cm$^2$. Those…