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We have investigated the magnetic properties and mapped out the phase diagram of the honeycomb magnet Na2Co2TeO6 with Co 3d7 in out-of-plane magnetic fields. This material has previously been proposed to show nearest-neighbor Kitaev…

Strongly Correlated Electrons · Physics 2024-06-03 Shengzhi Zhang , Sangyun Lee , Eric Brosha , Qing Huang , Haidong Zhou , Vivien S. Zapf , Minseong Lee

The candidate Kitaev magnet Na$_2$Co$_2$TeO$_6$ exhibits a characteristic ferrimagnetic response at low temperatures, with a finite residual magnetization that changes sign at a compensation point located at around half the ordering…

Strongly Correlated Electrons · Physics 2025-02-21 Niccolò Francini , Lukas Janssen

In this work we present a comprehensive investigation on magnetic and thermodynamic properties of the two-dimensional layered honeycomb system Cr$_2$Ge$_2$Te$_6$. Using magnetization and specific heat measurements under magnetic field…

Strongly Correlated Electrons · Physics 2020-01-29 Sebastian Selter , Gaël Bastien , Anja U. B. Wolter , Saicharan Aswartham , Bernd Büchner

We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

Strongly Correlated Electrons · Physics 2021-05-26 Wenjie Chen , Xintong Li , Zhenhai Hu , Ze Hu , Li Yue , Ronny Sutarto , Feizhou He , Kazuki Iida , Kazuya Kamazawa , Weiqiang Yu , Xi Lin , Yuan Li

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Recent theoretical studies have suggested that the low-energy Hamiltonian of honeycomb cobaltate systems could be dominated by anisotropic Kitaev interactions. Motivated by the theory, a honeycomb layered material Na$_{2}$Co$_{2}$TeO$_{6}$…

Strongly Correlated Electrons · Physics 2023-08-14 Emilie Dufault , Faranak Bahrami , Alenna Streeter , Xiaohan Yao , Enrique Gonzalez , Qiang Zhang , Fazel Tafti

Spin systems with honeycomb structures have recently attracted a great deal of attention in connection with the Kitaev quantum spin liquid state (QSL) predicted theoretically. One possible Kitaev QSL candidate is Na$_2$Co$_2$TeO$_6$…

Strongly Correlated Electrons · Physics 2023-12-11 A. K. Bera , S. M. Yusuf , F. Orlandi , P. Manuel , L. Bhaskaran , S. A. Zvyagin

We performed 23Na NMR measurements on a single-domain crystal of the Kitaev material Na3Co2SbO6, with magnetic field applied along the crystalline a axis. A positive Curie-Weiss constant is obtained from the NMR Knight shift, which suggests…

Strongly Correlated Electrons · Physics 2024-02-14 Ze Hu , Yue Chen , Yi Cui , Shuo Li , Cong Li , Xiaoyu Xu , Ying Chen , Xintong Li , Yuchen Gu , Rong Yu , Rui Zhou , Yuan Li , Weiqiang Yu

We report the magnetic, magnetodielectric, and electric polarization properties of single crystals of the Co-based Kitaev Spin Liquid (KSL) candidate Na$_2$Co$_2$TeO$_6$ (NCTO). The sample shows magnetic transitions at 26 K, 16 K, and 5 K,…

The Kitaev model is a rare example of an analytically solvable and physically instantiable Hamiltonian yielding a topological quantum spin liquid ground state. Here we report signatures of Kitaev spin liquid physics in the honeycomb magnet…

Strongly Correlated Electrons · Physics 2021-01-04 Hector K. Vivanco , Benjamin A. Trump , Craig M. Brown , Tyrel M. McQueen

We report a study on low-temperature heat transport of Kitaev magnet Na$_2$Co$_2$TeO$_6$, with the heat current and magnetic fields along the honeycomb spin layer (the $ab$ plane). The zero-field thermal conductivity of $\kappa^a_{xx}$ and…

Strongly Correlated Electrons · Physics 2024-06-19 Shuangkui Guang , Na Li , Qing Huang , Ke Xia , Yiyan Wang , Hui Liang , Yan Sun , Qiuju Li , Xia Zhao , Rui Leonard Luo , Gang Chen , Haidong Zhou , Xuefeng Sun

Ferrimagnetism appears in the temperature-field phase diagrams of several candidate Kitaev materials, such as the honeycomb cobaltates Na$_2$Co$_2$TeO$_6$ and Na$_3$Co$_2$SbO$_6$. In a number of instances, however, the exact nature of the…

Strongly Correlated Electrons · Physics 2025-10-31 Niccolò Francini , Pedro M. Cônsoli , Lukas Janssen

The honeycomb antiferromagnet BaCo2(AsO4)2, in which small in-plane magnetic fields (H1 = 0.26 T and H2 = 0.52 T at T = 1.8 K < TN = 5.4 K) induce two magnetic phase transitions, has attracted attention as a possible candidate material for…

Strongly Correlated Electrons · Physics 2022-06-15 Shuyuan Huyan , Juan Schmidt , Elena Gati , Ruidan Zhong , Robert J. Cava , Paul C. Canfield , Sergey L. Bud'ko

We report the magnetic properties of CaCo$_2$TeO$_6$ as a Kitaev candidate. CaCo$_2$TeO$_6$ was synthesized through a topochemical process, wherein all Na$^+$ ions in Na$_2$Co$_2$TeO$_6$ were replaced with half the amount of Ca$^{2+}$ ions.…

Strongly Correlated Electrons · Physics 2025-04-03 Yuya Haraguchi , Yuto Yoshida , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

Thermodynamic properties as well as low-energy magnon excitations of $S=1$ honeycomb-layered Na$_3$Ni$_2$SbO$_6$ have been investigated by high-resolution dilatometry, static magnetisation, and high-frequency electron spin resonance studies…

Strongly Correlated Electrons · Physics 2017-08-02 Johannes Werner , Waldemar Hergett , Mario Gertig , Jaena Park , Changhyun Koo , Rüdiger Klingeler

The crystal structure, magnetic ground state, and the temperature dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet Na2Co2TeO6 have been investigated by powder neutron diffraction. A three…

Strongly Correlated Electrons · Physics 2017-03-29 A. K. Bera , S. M. Yusuf , Amit Kumar , C. Ritter

We report magnetometry data obtained on twin-free single crystals of Na3Co2SbO6, which is considered a candidate material for realizing the Kitaev honeycomb model for quantum spin liquids. Contrary to a common belief that such materials can…

Despite exhibiting magnetic long-range order below $T_\mathrm{N} = 26.7\,\mathrm{K}$, the honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ is predicted to enter a Kitaev spin liquid state when subjected to small external perturbations. While most of…

Strongly Correlated Electrons · Physics 2026-03-04 J. Arneth , R. Kalaivanan , R. Sankar , K. -Y. Choi , R. Klingeler

Recent theoretical studies have suggested that Kitaev physics and such effects as formation of a mysterious spin-liquid state can be expected not only in RuCl3 and iridates, but also in conventional $3d$ transition metal compounds. Using DC…

Strongly Correlated Electrons · Physics 2023-02-22 E. Vavilova , T. Vasilchikova , A. Vasiliev , D. Mikhailova , V. Nalbandyan , E. Zvereva , S. V. Streltsov

As a candidate Kitaev material, Na$_2$Co$_2$TeO$_6$ exhibits intriguing magnetism on a honeycomb lattice that is believed to be $C_3$-symmetric. Here we report a neutron diffraction study of high quality single crystals under $a$-axis…

Strongly Correlated Electrons · Physics 2023-06-06 Weiliang Yao , Yang Zhao , Yiming Qiu , Christian Balz , J. Ross Stewart , Jeffrey W. Lynn , Yuan Li
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