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An autoionizing resonance in molecular N$_2$ is excited by an ultrashort XUV pulse and probed by a subsequent weak IR pulse, which ionizes the contributing Rydberg states. Time- and angular-resolved photoelectron spectra recorded with a…

State-dependent conformational changes play a central role in molecular dynamics, yet they are often difficult to observe or simulate due to their complexity and ultrafast nature. One alternative approach is to emulate such phenomena using…

Trapped ions are among the most advanced platforms for quantum simulation and computation. Their capabilities can be further augmented by making use of electronically highly excited Rydberg states, which enable the realization of…

Atomic Physics · Physics 2025-05-27 Wilson S. Martins , Joseph W. P. Wilkinson , Markus Hennrich , Igor Lesanovsky

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

We investigate a microwave ionization of highly excited atom in a low frequency field and show that such a process may be studied on the bases of map for the electron energy change during the period of the electron motion between two…

chao-dyn · Physics 2016-08-31 B. Kaulakys , G. Vilutis

We characterize the effect of quantum interference on the line shapes and measured line positions in atomic spectra. These effects, which occur when the excited state splittings are of order the excited state line widths, represent an…

We explore the possibility of calculating electronic excited states by using perturbation theory along a range-separated adiabatic connection. Starting from the energies of a partially interacting Hamiltonian, a first-order correction is…

Chemical Physics · Physics 2014-12-15 Elisa Rebolini , Julien Toulouse , Andrew M. Teale , Trygve Helgaker , Andreas Savin

In this chapter, we present an overview of experiments with trapped Rydberg ions and outline the advantages and challenges of developing applications of this new platform for quantum computing, sensing and simulation. Trapped Rydberg ions…

Quantum Physics · Physics 2020-07-28 Arezoo Mokhberi , Markus Hennrich , Ferdinand Schmidt-Kaler

New experimental quantum simulation platforms have recently been implemented with divalent atoms trapped in optical tweezer arrays with promising performance. The second valence electron also brings new propects through the so-called…

Atomic Physics · Physics 2022-06-15 Ky-Luc Pham , Thomas Gallagher , Pierre Pillet , Steven Lepoutre , Patrick Cheinet

Using trapped ions in an entangled state we propose detecting a magnetic dipole of a single atom at distance of a few $\mu$m. This requires a measurement of the magnetic field gradient at a level of about 10$^{-13}$ Tesla/$\mu$m. We discuss…

Quantum Physics · Physics 2015-06-05 F. Schmidt-Kaler , R. Gerritsma

We study the localization and addressability of ultra cold atoms in a combined parabolic and periodic potential. Such a potential supports the existence of localized stationary states and we show that using a radio frequency field allows to…

Statistical Mechanics · Physics 2009-11-10 H. Ott , E. de Mirandes , F. Ferlaino , G. Roati , V. Türck , G. Modugno , M. Inguscio

We present and analyze a simple model to illustrate the possibility of Rydberg state control by means of a moving guided electron. Specifically, we consider alkali metal atoms whose valence electron is initially prepared in a Rydberg…

Quantum Physics · Physics 2015-06-15 T. Laycock , B. Olmos , T. W. A. Montgomery , W. Li , T. M. Fromhold , I. Lesanovsky

Precision study of few-electron, high-$Z$ ions is a privileged field for probing high-field, bound-state quantum electrodynamics (BSQED). However, the accuracy of such tests is plagued by nuclear uncertainties, which are often larger than…

Atomic Physics · Physics 2021-05-05 Nancy Paul , Guojie Bian , Toshiyuki Azuma , Shinji Okada , Paul Indelicato

We report the measurement of ultrafast relaxation dynamics of excited states of carbon dioxide molecule using time-resolved pump-probe photoelectron spectroscopy. Neutral ground state carbon dioxide is excited to $nd\sigma_g$ Henning sharp…

Atomic Physics · Physics 2024-07-26 D. Biswas , J. K. Wood , I. Shalaby , A. Sandhu

The twisted light modes used in modern atomic physics experiments can be contaminated by small admixtures of plane wave radiation. Although these admixtures hardly reveal themselves in the beam intensity profile, they may seriously affect…

Atomic Physics · Physics 2024-01-30 R. P. Schmidt , S. Ramakrishna , A. A. Peshkov , N. Huntemann , E. Peik , S. Fritzsche , A. Surzhykov

We report on the observation and numerical calculation of ionization spectra of highly Stark-shifted Rydberg states of rubidium beyond the classical ionization threshold. In the numerical calculations, a complex absorbing potential (CAP)…

Scalable, local control over gate operations is an outstanding challenge in the field of quantum computing and programmable quantum simulation with Rydberg atom arrays. One approach is to use a global field to excite atoms to the Rydberg…

When ultracold plasma is generated using photonization of laser cooled atoms, some atoms reach only upto Rydberg states. These in turn interact with the free electrons of the plasma and get ionized further. We study the interaction of…

Atomic Physics · Physics 2026-03-18 Satyam Prakash , Ashok S Vudayagiri

We introduce a method to dispersively detect alkali atoms in radio-frequency dressed states. In particular, we use dressed detection to measure populations and population differences of atoms prepared in their clock states. Linear…

Atomic Physics · Physics 2018-04-26 Sindhu Jammi , Tadas Pyragius , Mark G. Bason , Hans Marin Florez , Thomas Fernholz

Using Resonant Pulsed Rydberg Field-ionization (RPRFI) technique, we generate low-energy electron bunches at high repetition rates. By combining continuous-wave laser excitation with a pulsed electric field, this method selectively ionizes…

Atomic Physics · Physics 2024-01-10 R. Hahn , D. Comparat