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We report on the local control of the transition frequency of a spin-$1/2$ encoded in two Rydberg levels of an individual atom by applying a state-selective light shift using an addressing beam. With this tool, we first study the spectrum…
Helium (He) is the ideal atom to perform tests of ab-initio calculations in two-electron systems that consider all known effects, including quantum-electrodynamics and nuclear-size contributions. Recent state-of-the-art calculations and…
By periodical two-step modulation, we demonstrate that the dynamics of multilevel system can still evolve even in multiple large detunings regime, and provide the effective Hamiltonian (of interest) for this system. We then illustrate this…
Photonic interconnects are a key technology for scaling up atomic based quantum computers. By facilitating the connection of multiple systems, high-performance modular quantum processing units may be constructed to perform deeper and more…
Calculating the energy spectrum of a quantum system is an important task, for example to analyse reaction rates in drug discovery and catalysis. There has been significant progress in developing algorithms to calculate the ground state…
An ionization-induced plasma grating can be formed by spatially selective ionization of gases by the interference of two intersecting ultra-short laser pulses. The density modulation of a plasma grating can approach unity since the plasma…
We present absolute-frequency measurements for the transitions from the 6s$_{1/2}$ ground state of $^{133}$Cs to $n$p$_{1/2}$ and $n$p$_{3/2}$ Rydberg states. The transition frequencies are determined by one-photon UV spectroscopy in…
The interaction of a trapped ion with a laser beam in the strong excitation regime is analyzed. In this regime, a variety of non--classical states of motion can be prepared either by using laser pulses of well defined area, or by an…
Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…
We develop a scheme for deterministic generation of an entangled state between two atoms on different Rydberg states via a chirped adiabatic passage, which directly connects the initial ground and target entangled states and also does not…
Neutral atom arrays are promising for large-scale quantum computing especially because it is possible to prepare large-scale qubit arrays. An unsolved issue is how to selectively excite one qubit deep in a 3D atomic array to Rydberg states.…
We observe electromagnetically induced transparency (EIT) on the 5s to 5p transition in a room temperature rubidium vapour cell by coupling the 5p state to a Rydberg state (ns or nd with n=26 to 124). We demonstrate that the narrow…
Rydberg atom-based sensors are a new type of radio frequency sensor that is inherently quantum mechanical. Several configurations of the sensor use a local oscillator to determine the properties of the target radio frequency field. We…
We demonstrate spatially resolved, coherent excitation of Rydberg atoms on an atom chip. Electromagnetically induced transparency (EIT) is used to investigate the properties of the Rydberg atoms near the gold coated chip surface. We measure…
We analyze the multipole excitation of atoms with twisted light, i.e., by a vortex light field that carries orbital angular momentum. A single trapped $^{40}$Ca$^+$ ion serves as a localized and positioned probe of the exciting field. We…
The full-dimensional time-dependent Schrodinger equation for the electronic dynamics of single-electron systems in intense external fields is solved directly using a discrete method. Our approach combines the finite-difference and Lagrange…
We present a theoretical analysis of the implementation of an entangling quantum gate between two trapped Ca$^+$ ions which is based on the dipolar interaction among ionic Rydberg states. In trapped ions the Rydberg excitation dynamics is…
I analyze a metrological strategy for improving the precision of frequency estimation via Ramsey interferometry with strings of atoms in the presence of correlated dephasing. This strategy does not employ entangled states, but rather a…
The ability to image electromagnetic fields holds key scientific and industrial applications, including electromagnetic compatibility, diagnostics of high-frequency devices, and experimental scientific work involving field interactions.…
Excited-state vibrations are crucial for determining photophysical and photochemical properties of molecular compounds. Stimulated Raman scattering can coherently stimulate and probe molecular vibrations with optical pulses, but it is…