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We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

The interferometric signals produced in conventional dual-comb laser ranging require femtosecond lasers with long-term f_CEO stability, and are limited to an upper sampling rate by radio-frequency aliasing considerations. By using…

Instrumentation and Detectors · Physics 2021-08-24 Hollie Wright , Jinghua Sun , David McKendrick , Nick Weston , Derryck T. Reid

We have generated frequency combs spanning 0.5 to 20 GHz in superconducting half wave resonators at T=3 K. Thin films of niobium-titanium nitride enabled this development due to their low loss, high nonlinearity, low frequency dispersion,…

Superconductivity · Physics 2014-11-05 R. P. Erickson , M. R. Vissers , M. Sandberg , S. R. Jefferts , D. P. Pappas

The characterization of Earth-like exoplanets and precision tests of cosmological models using next-generation telescopes such as the ELT will demand precise calibration of astrophysical spectrographs in the visible region, where stellar…

The broad and equidistant spectrum of frequency combs has had a profound impact on spectroscopic studies. Particularly, experiments involving the coupling of frequency combs to cavities have already enabled unprecedented broadband and…

Optics · Physics 2024-12-10 Andrei Diakonov , Konstantin Khrizman , Eliran Zano , Liron Stern

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…

This paper presents a novel approach to dual-frequency comb generation utilizing a single fiber Fabry-Perot resonator, advancing the implementation of these sources in fiber-based systems. Dual-comb applications such as spectroscopy,…

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…

Endoscopic imaging is essential for real-time visualization of internal organs, yet conventional systems remain bulky, complex, and expensive due to their reliance on large, multi-element optical components. This limits their accessibility…

Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…

Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…

We present a straightforward method to extend the noise-tracking bandwidth for self-correction algorithms in free-running dual-comb interferometry, leveraging coherent-harmonic-enhanced dual-comb spectroscopy. As a proof of concept, we…

Optics · Physics 2025-07-25 Wei Long , Yujia Ji , Xiangze Ma , Dijun Chen

Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…

Optics · Physics 2018-10-24 Bachana Lomsadze , Brad. C. Smith , Steven T. Cundiff

We introduce a novel ultra-broadband ultraviolet and visible frequency comb light source covering more than 240 THz by resonant dispersive wave emission in a gas-filled hollow-core fiber waveguide. The light source allows tuning from ~340…

Mid-infrared laser frequency combs are compelling sources for precise and sensitive metrology with applications in molecular spectroscopy and spectro-imaging. The infrared atmospheric window between 3-5.5 $\mu$m in particular provides vital…

Optical frequency combs enable all-solid-state spectrometers that will trigger a breakthrough in miniaturization and on-chip integration of mid-infrared sensing technology. Interband cascade lasers (ICLs) are an ideal candidate for…

The development of broadband microresonator frequency combs at visible wavelengths is pivotal for the advancement of compact and fieldable optical atomic clocks and spectroscopy systems. Yet, their realization necessitates resonators with…