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Coherent dual-comb spectroscopy (DCS) enables high-resolution measurements at high speeds without the trade-off between resolution and update rate inherent to mechanical delay scanning approaches. However, high system complexity and limited…

Mid-infrared (mid-IR) spectroscopy is a crucial workhorse for a plethora of analytical applications and is suitable for diverse materials, including gases, polymers or biological tissue. However, this technologically significant wavelength…

Optics · Physics 2022-02-23 Paul Kaufmann , Helen M. Chrzanowski , Aron Vanselow , Sven Ramelow

Supercontinuum generation using chip-integrated photonic waveguides is a powerful approach for spectrally broadening pulsed laser sources with very low pulse energies and compact form factors. When pumped with a mode-locked laser frequency…

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

Fourier-transform spectroscopy is an indispensable tool for analyzing chemical samples in scientific research as well as chemical and pharmaceutical industries. Recently, its measurement speed, sensitivity, and precision have been shown to…

Optics · Physics 2025-05-06 Takuro Ideguchi , Tasuku Nakamura , Yohei Kobayashi , Keisuke Goda

Dual-comb spectroscopy has emerged as an indispensable analytical technique in applications that require high resolution and broadband coverage within short acquisition times. Its experimental realization, however, remains hampered by…

Instrumentation and Detectors · Physics 2019-12-02 Łukasz A. Sterczewski , Aleksandra Przewłoka , Wawrzyniec Kaszub , Jarosław Sotor

While being invented for precision measurement of single atomic transitions, frequency combs have also become a versatile tool for broadband spectroscopy in the last years. In this paper we present a novel and simple approach for broadband…

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

Optics · Physics 2021-07-21 Brad C. Smith , Bachana Lomsadze , Steven T. Cundiff

Supercontinuum generation in optical fibers is one of the most dramatic nonlinear effects discovered, allowing short pulses to be converted into multi-octave spanning coherent spectra. However, generating supercontinua that are both…

We demonstrate cantilever-enhanced photoacoustic spectroscopy in the mid-infrared using a supercontinuum source. The approach is broadband, compact, and allows for higher photoacoustic signal intensity and enhanced signal-to-noise ratio as…

Instrumentation and Detectors · Physics 2018-11-14 Tommi Mikkonen , Caroline Amiot , Antti Aalto , Kim Patokoski , Goëry Genty , Juha Toivonen

A mid-Infrared frequency comb is produced via an optical parametric oscillator (OPO) pumped by an amplified 100 MHz Yb:fiber mode-locked laser. We use this source to make measurements of the concentration of the atmospherically-relevant…

Optics · Physics 2015-05-20 Lora Nugent-Glandorf , Fabrizio Giorgetta , Scott A. Diddams

The mid-infrared spectral window is essential for molecular fingerprinting and atmospheric sensing, yet unlocking its full potential is currently constrained by a fundamental instrumental trade-off: existing systems cannot simultaneously…

Microcombs - optical frequency combs generated in microresonators - have advanced tremendously in the last decade, and are advantageous for applications in frequency metrology, navigation, spectroscopy, telecommunications, and microwave…

We demonstrate a route to supercontinuum generation in gas-filled hollow-core anti-resonant fibers through the creation of a broad vibrational Raman frequency comb followed by continuous broadening and merging of the comb lines through…

Sustained mutual coherence between two combs over extended periods is a prerequisite for dual-comb spectroscopy (DCS), particularly in achieving high-resolution molecular spectroscopy and precise spectral measurements. However, achieving…

A chirped-pulse interleaving method is reported for generation of dual optical frequency combs based on electro-optic phase modulators (EOM) in a free-running all-fiber based system. Methods are discussed to easily modify the linear chirp…

Development of the optical frequency comb has revolutionised metrology and precision spectroscopy due to its ability to provide a precise and direct link between microwave and optical frequencies. A novel application of frequency comb…

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…

Ultraviolet frequency combs enable applications ranging from precision spectroscopy to atomic clocks by addressing the electronic transitions of atoms and molecules. Access to ultraviolet light via integrated nonlinear optics is usually…

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