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The two-dimensional van der Waals (vdW) materials MPS_3(M = Mn, Fe, Co, Ni) display antiferromagnetic ordering of the magnetic moments at the transition metal ions. The possibility to exfoliate thin layers that preserve the magnetic order…

Materials Science · Physics 2024-08-28 Mohammad Amirabbasi , Peter Kratzer

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

Strongly Correlated Electrons · Physics 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

The behavior of 2-dimensional (2D) van der Waals (vdW) layered magnetic materials in the 2D limit of the few-layer thickness is an important fundamental issue for the understanding of the magnetic ordering in lower dimensions. The…

Materials Science · Physics 2020-12-02 Soo Yeon Lim , Kangwon Kim , Sungmin Lee , Je-Geun Park , Hyeonsik Cheong

Lamellar structures of transition metal phosphorus trisulfides possess strong intralayer bonding, albeit adjacent layers are held by weak van der Waals interactions. Those compounds received enormous interest due to their unique combination…

The recent emergence of 2D van der Waals magnets down to atomic layer thickness provides an exciting platform for exploring quantum magnetism and spintronics applications. The van der Waals nature stabilizes the long-range ferromagnetic…

Materials Science · Physics 2019-02-14 Wenyu Xing , Luyi Qiu , Xirui Wang , Yunyan Yao , Yang Ma , Ranran Cai , Shuang Jia , X. C. Xie , Wei Han

We report on the temperature evolution of the polarization-dependent Raman spectrum of exfoliated MoI$_3$, a van der Waals material with a "true one-dimensional" crystal structure that can be exfoliated to individual atomic chains. The…

Although the magnetic order is suppressed by a strong magnetic frustration, it is maintained but appears in complex order forms such as a cycloid or spin density wave in weakly frustrated systems. Herein, we report a weakly…

We investigated low-frequency current fluctuations, i.e. noise, in the quasi-two-dimensional (2D) van der Waals antiferromagnetic semiconductor FePS3 with the electronic bandgap of 1.5 eV. The electrical and noise characteristics of the…

The Raman scattering response of the biaxial antiferromagnet CoPS$_3$ has been investigated as a function of both magnetic field and temperature. The peaks observed in the low-frequency spectral range (90--200~cm$^{-1}$) have been…

Layered van der Waals magnets have attracted much recent attention as a promising and versatile platform for exploring intrinsic two-dimensional magnetism. Within this broader class, the transition metal phosphorous trichalcogenides…

The observation of magnetism in atomically thin van der Waals (vdW) antiferromagnets (FePS$_3$, NiPS$_3$, and MnPS$_3$) in 2016 marked an important moment in the development of two-dimensional (2D) physics. In this personal reflection, I…

History and Philosophy of Physics · Physics 2026-01-16 Je-Geun Park

Among the numerous 2D system that can be prepared via exfoliation, iron phosphorus trisulfide (FePS3) attracts a lot of attention recently due to its broad-range photoresponse, its unusual Ising-type magnetic order and possible applications…

Materials Science · Physics 2023-01-16 Mohammad Amirabbasi , Peter Kratzer

Magnetic order in van der Waals magnets can strongly influence their lattice dynamics, yet how this interaction manifests across different phonon length scales remains unclear. Optical phonons probe bond-scale exchange modulation and…

This work reports an experimental study on an antiferromagnetic honeycomb lattice of MnPS$_3$ that couples the valley degree of freedom to a macroscopic antiferromagnetic order. The crystal structure of MnPS$_3$ is identified by high…

FePS$_3$ is a prototype van der Waals layered antiferromagnet and a Mott insulator under ambient conditions, which has been recently reported to go through a pressure-induced dimensionality crossover and an insulator-to-metal transition.…

Strongly Correlated Electrons · Physics 2023-07-19 Shiyu Deng , Siyu Chen , Bartomeu Monserrat , Emilio Artacho , Siddharth S Saxena

In two-dimensional (2D) nearly square-lattice quantum materials, electron correlations can induce an electronic nematic phase with twofold rotational ($C_2$) symmetry that profoundly impacts their properties. For 2D materials with threefold…

Mermin-Wagner theorem forbid spontaneous symmetry breaking of spins in one/two-dimensional systems at finite temperature and rules out the stabilization of this ordered state. However, it does not apply to all types of phase transitions in…

Materials Science · Physics 2023-12-05 N. Khan , D. Kumar , V. Kumar , Y. Shemerliuk , S. Selter , B. Büchner , K. Pal , S. Aswartham , Pradeep Kumar

A broad family of the nowadays studied low-dimensional systems, including 2D materials, demonstrate many fascinating properties, which however depend on the atomic composition as well as on the system dimensionality. Therefore, the studies…

Materials Science · Physics 2021-12-24 Yichen Jin , Mouhui Yan , Tomislav Kremer , Elena Voloshina , Yuriy Dedkov

The discovery of 2-dimensional (2D) materials, such as CrI3, that retain magnetic ordering at monolayer thickness has resulted in a surge of research in 2D magnetism from both pure and applied perspectives. Here, we report a magneto-Raman…

A new compound with a quasi-two-dimensional array of FeSe3O tetrahedra and an orthorombic structure, namely BaFe2Se2O, has been successfully fabricated. Experimental results show that this compound is an insulator and has an…

Strongly Correlated Electrons · Physics 2015-06-05 Fei Han , Xiangang Wan , Bing Shen , Hai-Hu Wen