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Recent experiments at the nanoscales confirm that thermal rectifiers, the thermal equivalent of electrical diodes, can operate in the quantum regime. We present a thorough investigation of the effect of different particle exchange…

Mesoscale and Nanoscale Physics · Physics 2022-11-10 Stephania Palafox , Ricardo Román-Ancheyta , Barış Çakmak , Özgür E. Müstecaplıoğlu

Within the framework of nonequilibrium Green's functions, we investigate the thermoelectric transport in a single molecular junction with electron-phonon and electron-electron interactions. By transforming into a displaced phonon basis, we…

Mesoscale and Nanoscale Physics · Physics 2012-04-26 Jie Ren , Jian-Xin Zhu , James E. Gubernatis , Chen Wang , Baowen Li

Thermoelectric materials convert a temperature gradient into a voltage. This phenomenon is relatively well understood for inorganic materials, but much less so for organic semiconductors (OSs). These materials present a challenge because…

We show that an increasingly strong thermal rectification effect occurs in the thermodynamic limit in a one-dimensional, graded rotor lattice with nearest-neighboring interactions only. The underlying mechanism is related to the transition…

Statistical Mechanics · Physics 2020-02-11 Shunjiang You , Daxing Xiong , Jiao Wang

We show that the combination of molecular chirality and phase-controlled driving can lead to rectification of vibrational energy transfer. We demonstrate this effect using classical models of (1) a single helical chain and (2) a more…

Chemical Physics · Physics 2025-10-31 Jichen Feng , Ethan Abraham , Joseph E. Subotnik , Abraham Nitzan

Vibrational heat transport in molecular junctions is a central issue in different contemporary research areas like Chemistry, material science, mechanical engineering, thermoelectrics and power generation. Our model system consists of a…

Statistical Mechanics · Physics 2025-07-04 Jayasmita Behera , Malay Bandyopadhyay

Heating and heat conduction in molecular junctions are considered within a general NEGF formalism. We obtain a unified description of heating in current carrying molecular junctions as well as the electron and phonon contributions to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Mark A. Ratner , Abraham Nitzan

The thermoelectric voltage developed across an atomic metal junction (i.e., a nanostructure in which one or a few atoms connect two metal electrodes) in response to a temperature difference between the electrodes, results from the quantum…

We present a theoretical analysis of heat transport through a single-molecule junction with two possible transport channels for electrons where interactions between electrons on the molecule and phonons in the nuclear environment is strong…

Mesoscale and Nanoscale Physics · Physics 2023-07-13 Natalya A. Zimbovskaya

Interference represents one of the most striking manifestation of quantum physics in low-dimensional systems. Despite evidences of quantum interference in charge transport have been known for a long time, only recently signatures of…

Mesoscale and Nanoscale Physics · Physics 2015-09-16 Luca Vannucci , Flavio Ronetti , Giacomo Dolcetto , Matteo Carrega , Maura Sassetti

We review recent developments in nonlinear quantum transport through nanostructures and mesoscopic systems driven by thermal gradients or in combination with voltage biases. Low-dimensional conductors are excellent platforms to analyze both…

Mesoscale and Nanoscale Physics · Physics 2016-11-14 David Sanchez , Rosa Lopez

We describe nonlinear phonon-thermoelectric devices where charge current and electronic and phononic heat currents are coupled, driven by voltage and temperature biases, when phonon-assisted inelastic processes dominate the transport. Our…

Mesoscale and Nanoscale Physics · Physics 2015-07-31 Jian-Hua Jiang , Manas Kulkarni , Dvira Segal , Yoseph Imry

It is shown that at low temperatures and moderate electron dephasing the electron transmission function reveales a structure containing information about donor/acceptor sites effectively participating in the electron transfer (ET) processes…

Biological Physics · Physics 2007-05-23 Natalya A. Zimbovskaya

We theoretically study thermal transport in an electronic interferometer comprising a parallel circuit of two quantum dots, each of which has a tunable single electronic state which are connected to two leads at different temperature.As a…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Sam Young Cho , Ross H. McKenzie

We present a unified description of heat flow in two-terminal hybrid quantum systems. Using simple models, we analytically study nonlinear aspects of heat transfer between various reservoirs: metals, solids, and spin baths, mediated by the…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Lian-Ao Wu , Claire X. Yu , Dvira Segal

Thermal conductivity, a fundamental parameter characterizing thermal transport in solids, is typically determined by electron and phonon transport. Although other transport properties including electrical conductivity and thermoelectric…

We investigate the heat conduction properties of molecular junctions comprising anharmonic interactions. We find that nonlinear interactions can lead to novel phenomena: it negative differential thermal conductance and heat rectification.…

Soft Condensed Matter · Physics 2009-11-11 Dvira Segal

A first-principles approach is presented for the thermoelectricity in molecular junctions formed by a single molecule contact. The study investigates the Seebeck coefficient considering the source-drain electrodes with distinct temperatures…

Mesoscale and Nanoscale Physics · Physics 2009-05-07 Yu-Shen Liu , Yu-Chang Chen

Several models of thermionic energy nanoconverters have been proposed to study the transport phenomena that take place in electronic devices. For example, in resonant tunneling junctions those phenomena are manifested through the…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 G. Valencia-Ortega , L. A. Arias-Hernandez

A framework for estimating heating and expected temperature rise in current carrying molecular junctions is described. Our approach is based on applying the Redfield approximation to a tight binding model for the molecular bridge…

Condensed Matter · Physics 2009-11-07 Dvira Segal , Abraham Nitzan