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The atomic variations of electronic wavefunctions at the surface and electron scattering near a defect have been detected unprecedentedly by tracing thermoelectric voltages given a temperature bias [Cho et al., Nature Mater. 12, 913…

Mesoscale and Nanoscale Physics · Physics 2014-04-02 Eui-Sup Lee , Sanghee Cho , Ho-Ki Lyeo , Yong-Hyun Kim

The thermoelectric transport through a molecular bridge is discussed, with an emphasis on the effects of inelastic processes of the transport electrons caused by the coupling to the vibrational modes of the molecule. In particular it is…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 O. Entin-Wohlman , Y. Imry , A. Aharony

We study heat transfer between conductors, mediated by the excitation of a monomodal harmonic oscillator. Using a simple model, we show that the onset of rectification in the system is directly related to the nonlinearity of the electron…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Dvira Segal

We study heat conduction in (n, 0)/(2n, 0) intramolecular junctions by using molecular dynamics method. It is found that the heat conduction is asymmetric, namely, heat transports preferably in one direction. This phenomenon is also called…

Mesoscale and Nanoscale Physics · Physics 2007-08-18 Gang Wu , Baowen Li

A minimal model for coherent transport through a donor/acceptor molecular junction is presented. The two donor and acceptor sites are described by single levels energetically separated by an intramolecular tunnel barrier. In the limit of…

Disordered Systems and Neural Networks · Physics 2009-11-11 Florian Pump , Gianaurelio Cuniberti

A theory is developed to describe the coupled transport of energy and charge in networks of electron donor-acceptor sites which are seated in a thermally heterogeneous environment, where the transfer kinetics are dominated by Marcus-type…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Galen T. Craven , Abraham Nitzan

The realization of single-molecule thermal conductance measurements has driven the need for theoretical tools to describe conduction processes that occur over atomistic length scales. In macroscale systems, the principle that is typically…

Mesoscale and Nanoscale Physics · Physics 2023-05-17 Galen T. Craven , Abraham Nitzan

We study charge and energy transfer in two-site molecular electronic junctions in which electron transport is assisted by a vibrational mode. To understand the role of mode harmonicity/anharmonicity on transport behavior, we consider two…

Mesoscale and Nanoscale Physics · Physics 2015-09-01 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

The rate of electron transfer between a molecular species and a metal, each at a different local temperature, is examined theoretically through implementation of a bithermal (characterized by two temperatures) Marcus formalism. Expressions…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Galen T. Craven , Abraham Nitzan

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

We introduce a direct (Seebeck) and inverse (Peltier) thermoelectric effect induced by electron tunneling between closely separated conducting films. When a transverse temperature gradient is applied along one of two films, a bias voltage…

Mesoscale and Nanoscale Physics · Physics 2024-09-10 Mauricio Gómez Viloria , Riccardo Messina , Philippe Ben-Abdallah

The understanding of the underlying dynamical mechanisms which determine the macroscopic laws of heat conduction is a long standing task of non-equilibrium statistical mechanics. A better understanding of the mechanism of heat conduction…

Statistical Mechanics · Physics 2011-09-08 Giulio Casati , Carlos Mejia-Monasterio

We explore heat transfer in molecular junctions between two leads in the absence of a finite net thermal bias. The application of an unbiased, time-periodic temperature modulation of the leads entails a dynamical breaking of reflection…

Mesoscale and Nanoscale Physics · Physics 2009-12-18 Fei Zhan , Nianbei Li , Sigmund Kohler , Peter Hänggi

We present a theoretical study of radiative heat transport in nonlinear solid-state quantum circuits. We give a detailed account of heat rectification effects, i.e. the asymmetry of heat current with respect to a reversal of the thermal…

Mesoscale and Nanoscale Physics · Physics 2009-04-28 Tomi Ruokola , Teemu Ojanen , Antti-Pekka Jauho

Maxwell's equations incorporating thermoelectric and thermomagnetic effects are studied. Energy transport involving electric field only flows along the velocity direction and a direction perpendicular to it. Magnetic energy transport…

General Physics · Physics 2017-09-12 A. I. Arbab

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

Mesoscale and Nanoscale Physics · Physics 2011-03-15 R. Härtle , M. Thoss

The effect of a thermal environment on electron (or hole) transfer through molecular bridges and on the electron conduction properties of such bridges is studied. Our steady state formalism based on an extension of the Redfield theory (D.…

Condensed Matter · Physics 2009-11-07 Dvira Segal , Abraham Nitzan

We consider a molecular junction immersed in a solvent where the electron transfer is dominated by Marcus-type steps. However, the successive nature of the charge transfer through the junction does not imply that the solvent reach thermal…

Statistical Mechanics · Physics 2022-03-23 Henning Kirchberg , Abraham Nitzan

We investigate the thermopower of a metal-molecule-metal junction taking into account thermal effects on the junction. Based on analytical expressions and numerical simulations we show that the thermoelectric potential reveals valuable…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dvira Segal

Asymmetric heat transfer systems, often referred to as thermal diodes or thermal rectifiers, have garnered increasing interest due to their wide range of application possibilities. Most of those previous macroscopic thermal diodes either…

Applied Physics · Physics 2022-09-09 Yishu Su , Ying Li , Minghong Qi , Sebastien Guenneau , Huagen Li , Jian Xiong
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