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The interface of complex oxide heterostructures sets the stage for various electronic and magnetic phenomena. Many of these collective effects originate from the precise structural arrangement at the interface that in turn governs local…

Mesoscale and Nanoscale Physics · Physics 2021-03-17 Max Burian , Bill Francesco Pedrini , Nazaret Ortiz Hernandez , Hiroki Ueda , C. A. F. Vaz , Milan Radovic , Urs Staub

We perform first-principles density functional calculations to elucidate structural, electronic and magnetic properties at the interface of \ce{(0001)Cr2O3-(111)Pt} bilayers. This investigation is motivated by the fact that, despite the…

Materials Science · Physics 2024-05-09 Marlies Reher , Nicola A. Spaldin , Sophie F. Weber

Silicon dioxide and silicon (SiO$_{2}$/Si) interface plays a very important role in semiconductor industry. However, at nanoscale, its interfacial thermal properties haven't been well understood so far. In this paper, we systematically…

Materials Science · Physics 2015-06-11 Jie Chen , Gang Zhang , Baowen Li

Surface and ferroelectric properties of PbTiO$_3$ thin films are investigated using an interatomic potential approach with parameters computed from first-principles calculations. We show that a model developed for the bulk describes…

Materials Science · Physics 2009-11-11 M. Sepliarsky , M. G. Stachiotti , R. L. Migoni

Low dimensional structures comprised of ferroelectric (FE) PbTiO$_3$ (PTO) and quantum paraelectric SrTiO$_3$ (STO) are hosts to complex polarization textures such as polar waves, flux-closure domains and polar skyrmion phases. Density…

Materials Science · Physics 2022-02-16 Jack S. Baker , David R. Bowler

Employing a first-principles and model Hamiltonian approach, we work out the electronic properties of polar-polar LaVO$_3$/KTaO$_3$ (LVO/KTO, 001) heterostrctures, with up to six layers of KTO and five layers of LVO. Our analyses indicate…

Materials Science · Physics 2024-08-02 Shubham Patel , Narayan Mohanta , Snehasish Nandy , Subhendra D. Mahanti , A Taraphder

Unconventional ferroelectricity, robust at reduced nanoscale sizes, exhibited by hafnia-based thin-films presents tremendous opportunities in nanoelectronics. However, the exact nature of polarization switching remains controversial. Here,…

Heteroepitaxial growth of transition-metal oxide films on the open (111) surface of SrTiO3 results in significant restructuring due to the polar mismatch. Monitoring the structural and composition on an atomic scale of LaNiO3/SrTiO3 (111)…

Materials Science · Physics 2017-04-26 Mohammad Saghayezhian , Zhen Wang , Hangwen Guo , Yimei Zhu , E. W. Plummer , Jiandi Zhang

An unresolved issue in the commonly used Pb(Zr1-xTix)O3 (PZT) ceramics is understanding the intrinsic piezoelectric behaviors of its crystal around the morphotropic phase boundary (MPB). Here, we demonstrate a novel approach to grow c-axis…

Materials Science · Physics 2024-08-26 Desheng Fu , Seiji Sogen , Hisao Suzuki

We have studied magnetoresistance and Hall effects for 1.8-nm-thick Pt films grown on a ferrimagnetic insulator Y3Fe5O12 in a wide temperature (0.46-300 K) and magnetic-field (-15-15 T) region. In the low-temperature regime where quantum…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Y. Shiomi , T. Ohtani , S. Iguchi , T. Sasaki , Z. Qiu , H. Nakayama , K. Uchida , E. Saitoh

Interfacial charge transfer in oxide heterostructures gives rise to a rich variety of electronic and magnetic phenomena. Designing heterostructures where one of the thin-film components exhibits a metal-insulator transition opens a…

Renewed interest has been witnessed in utilizing the piezoelectric response of $PbZr_{0.52}Ti_{0.48}O_{3}$ (PZT) films on glass substrates for applications such as data storage and adaptive optics. Accordingly, new methodologies are being…

First-principles calculations are performed to investigate alloying and ferroelectric effects in lead zirconate titanate (PZT) with high Ti composition. We find that the main effect of alloying in the paraelectric phase of PZT is the…

Materials Science · Physics 2009-10-31 L. Bellaiche , J. Padilla , David Vanderbilt

Perovskite oxide heteroepitaxy receives much attention because of the possibility to com- bine the diverse functionalities of perovskite oxide building blocks. A general boundary con- dition for the epitaxy is the presence of polar…

In piezoelectric ceramics the changes in the phase stabilities versus stress and temperature in the vicinity of the phase boundary play a central role. The present study was dedicated to the classical piezoelectric, lead-zirconate-titanate…

Materials Science · Physics 2015-06-04 J. Frantti , Y. Fujioka , J. Zhang , S. Wang , S. C. Vogel , R. M. Nieminen , A. M. Asiri , Y. Zhao , A. Y. Obaid

Interface effect in complex oxide thin film heterostructures lies at the vanguard of current research to design technologically relevant functionality and explore emergent physical phenomena. While most of the previous works focus on the…

Materials Science · Physics 2019-01-30 B. C. Behera , Subhadip Jana , Shwetha G. Bhat , G. Tripathy , P. S. Anil Kumar , D. Samal

Heterointerfaces have been pivotal in unveiling extraordinary interfacial properties and enabling multifunctional material platforms. Despite extensive research on all-oxide interfaces, heterointerfaces between different material classes,…

We present a comprehensive first-principles study of the electronic charge redistribution in atomically sharp LaAlO$_3$/SrTiO$_3$(001) heterointerfaces of both n- and p-types allowing for non-stoichiometric composition. Using two different…

Materials Science · Physics 2012-11-13 Alexandre Sorokine , Dmitry Bocharov , Sergei Piskunov , Vyacheslavs Kashcheyevs

The electronic reconstruction at the interface between two insulating oxides can give rise to a highly-conductive interface. In analogy to this remarkable interface-induced conductivity we show how, additionally, magnetism can be induced at…

Strongly Correlated Electrons · Physics 2007-06-13 A. Brinkman , M. Huijben , M. van Zalk , J. Huijben , U. Zeitler , J. C. Maan , W. G. van der Wiel , G. Rijnders , D. H. A. Blank , H. Hilgenkamp

In metal/oxide heterostructures, rich chemical, electronic, magnetic and mechanical properties can emerge from interfacial chemistry and structure. The possibility to dynamically control interface characteristics with an electric field…

Materials Science · Physics 2015-06-22 Uwe Bauer , Lide Yao , Satoru Emori , Harry L. Tuller , Sebastiaan van Dijken , Geoffrey S. D. Beach