Related papers: High harmonic generation spectroscopy via orbital …
We present a new theory for orbital angular momentum (OAM) generation by chaotic phase surfaces with discrete integer bias distributions. We derive fundamental selection rules that determine which OAM modes can be coherently generated. Our…
The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…
We propose a real-time time-dependent ab__initio approach within a configuration-interaction-singles ansatz to decompose the high-harmonic generation (HHG) signal of molecules in terms of individual molecular-orbital (MO) contributions.…
We demonstrate that the strongly nonlinear regime of the magnetic dynamics driven high harmonic generation (HHG) can be captured through an adiabatic treatment. The underlying instantaneous energy dispersion reveal a highly nonlinear term…
We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…
To date, orbital angular momentum (OAM) and optical frequency combs (OFCs) are two distinct fields of research without any association. Herein, we generated OFCs with an OAM on each comb line by applying electro-optic phase modulation to…
High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…
We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…
Vector beams with spatially structured polarization and intertwined spin-orbital angular momentum (SAM-OAM) provide powerful degrees of freedom for tailoring light-matter interactions. While such structured beams are well established in the…
We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…
The high-order harmonic generation (HHG), if phase matched, opens a unique way to produce coherent ultrafast extreme-UV (XUV) or soft x-ray light sources. Here we describe a robust and tunable method for scaling and narrowing the bandwidth…
Recently, a method to image molecular electronic wave functions using high harmonic generation (HHG) was introduced by Itatani \textit{et al.\} [Nature {\textbf{432}}, 876 (2004)]. We show that, while the tomographic reconstruction of…
We developed a method to characterize arbitrary superpositions of light orbital angular momentum (OAM) with high fidelity by using astigmatic tomography and machine learning processing. In order to define each superposition unequivocally,…
We design the proof of concept for high-resolution (HR) real-time (RT), Geosynchronous and Geostationary (Geo) Polarimetric (Pol) using orbital angular momentum (OAM) interferometry - radio detection and ranging (RADAR)…
We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…
High-harmonic generation (HHG) from a compact, solid-state medium is highly desirable for applications such as coherent attosecond pulse generation and extreme ultra-violet (EUV) spectroscopy, yet the typically weak conversion of pump light…
The angular momentum propagated by a beam of radiation has two contributions: spin angular momentum (SAM) and orbital angular momentum (OAM). SAM corresponds to wave polarisation, while OAM-carrying beams are characterized by a phase which…
X-ray beams carrying orbital angular momentum (OAM), are emerging as a powerful tool to probe matter. Recently, a method called self-seeded FEL with OAM (SSOAM) has been proposed to generate high-power x-ray OAM pulses, which places the…
High-harmonic generation (HHG) is widely used for up-conversion of amplified (near) infrared ultrafast laser pulses to short wavelengths. We demonstrate that Ramsey-comb spectroscopy, based on two such pulses derived from a frequency-comb…
The recent demonstration of electron vortex beams has opened up the new possibility of studying orbital angular momentum (OAM) in the interaction between electron beams and matter. To this aim, methods to analyze the OAM of an electron beam…