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Controlling the crystal structure is a powerful approach for manipulating the fundamental properties of solids. Unique to two-dimensional (2D) van der Waals materials, the control can be achieved by modifying the stacking order through…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Weijong Chen , Zeyuan Sun , Lehua Gu , Xiaodong Xu , Shiwei Wu , Chunlei Gao

Magnetism in two-dimensional materials is not only of fundamental scientific interest but also a promising candidate for numerous applications. However, studies so far, especially the experimental ones, have been mostly limited to the…

Mesoscale and Nanoscale Physics · Physics 2017-01-26 Jae-Ung Lee , Sungmin Lee , Ji Hoon Ryoo , Soonmin Kang , Tae Yun Kim , Pilkwang Kim , Cheol-Hwan Park , Je-Geun Park , Hyeonsik Cheong

Using polarization-resolved Raman spectroscopy, we investigate layer number, temperature, and magnetic field dependence of Raman spectra in one- to four-layer $\mathrm{CrI_{3}}$. Layer-number-dependent Raman spectra show that in the…

The discovery of two-dimensional (2D) systems hosting intrinsic long-range magnetic order represents a seminal addition to the rich physical landscape of van der Waals (vdW) materials. CrI3 has emerged as perhaps the most salient example,…

Recent observation of intrinsic ferromagnetism in two-dimensional (2D) CrI$_3$ is associated with the large magnetic anisotropy due to strong spin-orbit coupling (SOC) of I. Magnetic anisotropy energy (MAE) defines the stability of…

Mesoscale and Nanoscale Physics · Physics 2018-10-10 Lucas Webster , Jia-An Yan

In the study of van der Waals-layered magnetic materials, the properties of CrCl$_3$ continue to attract attention. This compound is reported to undergo antiferromagnetic (AFM) ordering below $\sim$14 K, with a ferromagneticlike region…

Materials Science · Physics 2024-11-13 John A. Schneeloch , Adam A. Aczel , Feng Ye , Despina Louca

Stacking order plays a crucial role in determining the crystal symmetry and has significant impacts on electronic, optical, magnetic, and topological properties. Electron-phonon coupling, which is central to a wide range of intriguing…

Two-dimensional (2D) chromium telluride Cr2Te3 exhibits strong ferromagnetic ordering with high coercivity at low temperatures and paramagnetic behaviour when approaching room temperature. The spin states of monolayer Cr2Te3 show…

Among the numerous 2D system that can be prepared via exfoliation, iron phosphorus trisulfide (FePS3) attracts a lot of attention recently due to its broad-range photoresponse, its unusual Ising-type magnetic order and possible applications…

Materials Science · Physics 2023-01-16 Mohammad Amirabbasi , Peter Kratzer

The crystal and magnetic structures of the orthorhombic e-Fe2O3 have been studied by simultaneous Rietveld refinement of X-ray and neutron powder diffraction data in combination with Mossbauer spectroscopy, as well as magnetisation and heat…

We calculate the temperature dependent long-range magnetic coupling in the presence of dilute concentrations of random magnetic impurities in chiral multilayer two-dimensional semimetals, i.e., undoped intrinsic multilayer graphene.…

Mesoscale and Nanoscale Physics · Physics 2017-04-17 Hongki Min , E. H. Hwang , S. Das Sarma

Magneto-optical effect refers to a rotation of polarization plane, which has been widely studied in traditional ferromagnetic metal and insulator films and scarcely in two-dimensional layered materials. Here we uncover a new nonreciprocal…

We investigated complex magnetic properties of multifunctional LaCrO3-LaFeO3 system. The magnetic measurements substantiate the presence of competing complex magnetic ordering against temperature, showing paramagnetic to ferrimagnetic…

Strongly Correlated Electrons · Physics 2019-08-20 Brajesh Tiwari , Ambesh Dixit , M. S. Ramachandra Rao

Recently, three different magnetic states were observed experimentally in trilayer CrI3 under pressure,including ferromagnetic (FM)-upupup, FM-downupdown and FM-upupdown. To reveal the nature of the observed three magnetic states, we…

Materials Science · Physics 2021-12-08 Zhen Zhang , Jing-Yang You , Bo Gu , Gang Su

The recent discovery of ferromagnetic single-layer CrI3 creates ample opportunities for studying fundamental properties of atomically-thin magnets. By using first-principles calculations and model analysis, we show that a lateral strain…

Mesoscale and Nanoscale Physics · Physics 2017-09-19 Fawei Zheng , Jize Zhao , Zheng Liu , Menglei Li , Mei Zhou , Shengbai Zhang , Ping Zhang

Through advanced experimental techniques on CrI$_{3}$ single crystals, we derive a previously not discussed pressure-temperature phase diagram. We find that $T_{c}$ increases to $\sim$ 66\,K with pressure up to $\sim$ 3\,GPa followed by a…

Two-dimensional (2D) layered magnetic materials are generating a great amount of interest for the next generation of electronic devices thanks to their remarkable properties associated to spin dynamics. The recently discovered layered…

Two-dimensional (2D) chromium tellurides have attracted considerable research interest for their high Curie temperatures. Their magnetic properties have been found diverse in various experiments, the understanding of which however remains…

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…

The role of dipolar interactions and anisotropy are important to obtain, otherwise forbidden, ferromagnetic ordering at finite temperature for ions arranged in two-dimensional (2D) arrays (monolayers). Here we demonstrate that conventional…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. K. Mukhopadhyay , M. K. Sanyal , T. Sakakibara , V. Leiner , R. M. Dalgliesh , S. Langridge