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Vibrational sum frequency generation (SFG) is a nonlinear spectroscopic technique widely used to study the molecular structure and dynamics of surface systems. However, the spatial resolution achieved by far-field observations is…

This work presents a feasible design of an integrated photonic circuit performing as a device for single-qubit preparation and rotations through the third-order nonlinear process of difference frequency generation (DFG) and defined in the…

Quantum Physics · Physics 2022-07-21 A. L. Aguayo-Alvarado , F. Domínguez-Serna , W. De La Cruz , K. Garay-Palmett

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

Accurate low-order structure factors (Fg) measured by quantitative convergent beam electron diffraction (QCBED) were used for validation of different density functional theory (DFT) approximations. 23 low-order Fg were measured by QCBED for…

Materials Science · Physics 2013-02-26 Xiahan Sang , Andreas Kulovits , Guofeng Wang , Jorg Wiezorek

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We propose Raman-induced collinear difference-frequency generation (DFG) as a method to manipulate dynamical magnetization. When a fundamental beam propagates along a threefold rotational axis, this coherent second-order optical process is…

Materials Science · Physics 2011-02-22 Takuya Higuchi , Natsuki Kanda , Hiroharu Tamaru , Makoto Kuwata-Gonokami

To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…

Materials Science · Physics 2024-09-04 Akihito Kato , Nobuhiko Yokoshi

We consider the spontaneous creation of a dc voltage across a strongly coupled semiconductor superlattice subjected to THz radiation. We show that the dc voltage may be approximately proportional either to an integer or to a half- integer…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kirill N. Alekseev , Ethan H. Cannon , Feodor V. Kusmartsev , David K. Campbell

The nonlinear optical responses from topological semimetals are crucial in both understanding the fundamental properties of quantum materials and designing next-generation light-sensors or solar-cells. However, previous work was focusing on…

In this paper, the partial-wave expansion method is applied to describe the difference-frequency pressure generated in a nonlinear scattering of two acoustic waves with an arbitrary wavefront by means of a rigid sphere. Particularly, the…

Classical Physics · Physics 2012-08-28 Glauber T. Silva , Anderson Bandeira

We present a universal and rigorous approach to study difference frequency generation in the terahertz domain, keeping the number of degrees of freedom to a minimum, through the definition of a suitable figure of merit. The proposed method…

Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…

Nonlinear metal-dielectric layered structures are shown to be able to efficiently generate entangled photon pairs using spontaneous parametric down-conversion. Increase of electric-field amplitudes in these structures enhanced by the…

Quantum Physics · Physics 2015-01-12 Dalibor Javůrek , Jan Peřina , Jiří Svozilík

The combination of grating-based frequency-selective optical feedback mechanisms, such as distributed feedback (DFB) or distributed Bragg reflector (DBR) structures, with quantum dot (QD) gain materials is a main approach towards…

Second harmonic generation (SHG) is a fundamental nonlinear optical phenomenon widely used both for experimental probes of materials and for application to optical devices. Even-order nonlinear optical responses including SHG generally…

Mesoscale and Nanoscale Physics · Physics 2021-10-13 Kazuaki Takasan , Takahiro Morimoto , Joseph Orenstein , Joel E. Moore

Dielectric relaxation in disordered dielectric mixtures are presented by emphasizing the interfacial polarization. The obtained results coincide with and cause confusion with those of the low frequency dispersion behavior. The considered…

Disordered Systems and Neural Networks · Physics 2007-05-23 Enis Tuncer

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

The equations providing to describe generation process in FEL with varied parameters of diffraction grating (photonic crystal) are obtained. It is shown that applying diffraction gratings (photonic crystal) with the variable period one can…

Accelerator Physics · Physics 2007-05-23 V. G. Baryshevsky , A. A. Gurinovich

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein