English
Related papers

Related papers: Comments on the linear modified Poisson-Boltzmann …

200 papers

Treating water as a linearly responding dielectric continuum on molecular length scales allows very simple estimates of solvation structure and thermodynamics for charged and polar solutes. While this approach can successfully account for…

Statistical Mechanics · Physics 2021-07-07 Stephen J. Cox , Kranthi K. Mandadapu , Phillip L. Geissler

The combinatorial explosion of empirical parameters in tens of thousands presents a tremendous challenge for extended Debye-H\"uckel models to calculate activity coefficients of aqueous mixtures of most important salts in chemistry. The…

Soft Condensed Matter · Physics 2018-03-14 Jinn-Liang Liu , Bob Eisenberg

We evaluate the exponentially rare fluctuations of the ionic current for a dilute electrolyte by means of macroscopic fluctuation theory. We consider the fluctuating hydrodynamics of a fluid electrolyte described by a stochastic…

Statistical Mechanics · Physics 2025-07-25 Jafar Farhadi , David T. Limmer

We present two successive mean-field approximations for describing the mechanical properties and the swelling equilibrium of polyelectrolyte gels in contact with a salt solution. The first mean-field approximation reduces the many-chain…

Soft Condensed Matter · Physics 2019-11-22 Jonas Landsgesell , Christian Holm

Porous electrodes{made of hierarchically nanostructured materials{are omnipresent in various electrochemical energy technologies from batteries and supercapacitors to sensors and electrocatalysis. Modeling the system-level macroscopic…

Applied Physics · Physics 2022-02-03 Anis Allagui , Hachemi Benaoum

An extension of the renormalized Jellium model which allows to study colloidal suspensions containing trivalent counterions is proposed. The theory is based on a modified Poisson-Boltzmann equation which incorporates the effects of…

Soft Condensed Matter · Physics 2012-03-26 Thiago E. Colla , Yan Levin

We develop a first-principle equation of state of salt-free polyelectrolyte solution in the limit of infinitely long flexible polymer chains in the framework of a field-theoretical formalism beyond the linear Debye-Hueckel theory and…

Soft Condensed Matter · Physics 2015-08-04 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , E. A. Nogovitsyn , M. G. Kiselev

We study a model Coulomb fluid consisting of dipolar solvent molecules of finite extent generalizing the point-like Dipolar Poisson-Boltzmann model (DPB) previously introduced by Coalson and Duncan (J. Phys. Chem 100, 2612 (1996)) and…

Soft Condensed Matter · Physics 2014-06-18 Sahin Buyukdagli , Ralf Blossey

We investigate the screening properties of Gaussian charge models of electrolyte solutions by analysing the asymptotic behaviour of the pair distribution functions. We use a combination of Monte-Carlo simulations with the hyper-netted chain…

Soft Condensed Matter · Physics 2015-06-15 Patrick B. Warren , Andrey Vlasov , Lucian Anton , Andrew J. Masters

The classical treatment of the electrical double-layer (EDL) structure at a planar metal/electrolyte junction via the Gouy-Chapman-Stern (GCS) approach is based on the Poisson equation relating the electrostatic potential to the net mean…

Applied Physics · Physics 2022-01-11 Anis Allagui , Hachemi Benaoum , Oleg Olendski

A theory of a confined two dimensional electrolyte is presented. The positive and negative ions, interacting by a $1/r$ potential, are constrained to move on an interface separating two solvents with dielectric constants $\epsilon_1$ and…

Statistical Mechanics · Physics 2009-11-07 J. E. Flores-Mena , Marcia C. Barbosa , Yan Levin

The cell-model and its treatment on the Poisson-Boltzmann level are two important concepts in the theoretical description of charged macromolecules. In this brief contribution to the Proceedings of the NATO-ASI on ``Electrostatic Effects in…

Soft Condensed Matter · Physics 2007-05-23 Markus Deserno , Christian Holm

Density functional theory is used to describe electrolyte solutions in contact with electrodes of planar or spherical shape. For the electrolyte solutions we consider the so-called civilized model, in which all species present are treated…

Soft Condensed Matter · Physics 2017-04-24 Andreas Reindl , Markus Bier , S. Dietrich

The Drude-Lorentz model for the motion of electrons in a solid is a classical model in statistical mechanics, where electrons are represented as point particles bouncing on a fixed system of obstacles (the atoms in the solid). Under some…

Mathematical Physics · Physics 2016-06-29 François Golse

The Cauchy problem for the linearization of a system of equations arising in the kinetic theory of a condensed gas of bosons near the critical temperature around one of its equilibria is solved for radially symmetric initial data. It is…

Analysis of PDEs · Mathematics 2022-01-19 Miguel Escobedo

Two overall neutral surfaces with positive and negative charged domains ("patches") have been shown in recent experiments to exhibit long-range attraction when immersed in an ionic solution. Motivated by the experiments, we calculate…

Soft Condensed Matter · Physics 2016-08-31 Ram M. Adar , David Andelman , Haim Diamant

A quantum linear Boltzmann equation is proposed, constructed in terms of the operator-valued dynamic structure factor of the macroscopic system the test particle is interacting with. Due to this operator structure it is a non-Abelian linear…

Quantum Physics · Physics 2009-11-07 Bassano Vacchini

Recent results on the fluid dynamic limits of the Boltzmann equation based on the DiPerna-Lions theory of renormalized solutions are reviewed in this paper, with an emphasis on regimes where the velocity field behaves to leading order like…

Analysis of PDEs · Mathematics 2012-07-26 François Golse

We present a theory of effective electrostatic interactions in polydisperse suspensions of charged macroions, generalizing to mixtures a theory previously developed for monodisperse suspensions. Combining linear response theory with a…

Soft Condensed Matter · Physics 2013-08-20 Jun Kyung Chung , Alan R. Denton

A modified Poisson-Nernst-Planck system in a bounded domain with mixed Dirichlet-Neumann boundary conditions is analyzed. It describes the concentrations of ions immersed in a polar solvent and the correlated electric potential due to the…

Analysis of PDEs · Mathematics 2023-05-25 Ansgar Jüngel , Annamaria Massimini