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The spectral characterization of quantum emitter luminescence over broad wavelength ranges and fast timescales is important for applications ranging from biophysics to quantum technologies. Here we present the application of time-domain…

The feasibility of sub-Doppler broadband multi-heterodyne spectroscopy with two laser frequency combs is demonstrated with two-photon excitation spectra of the 5S-5D transitions of rubidium vapor.

We present a dual-comb spectrometer based on two passively mode-locked waveguide lasers integrated in a single Er-doped ZBLAN chip. This original design yields two free-running frequency combs having a high level of mutual stability. We…

Two semiconductor optical frequency combs consuming less than 1 W of electrical power are used to demonstrate high-sensitivity mid-infrared dual-comb spectroscopy in the important 3-4 $\mu$m spectral region. The devices are 4 millimeters…

Nonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors…

Optics · Physics 2025-08-11 Kazuki Hashimoto , Dmitri B. Horoshko , Maria V. Chekhova

The second-order temporal interference between two independent single-mode continuous-wave lasers is discussed by employing two-photon interference in Feynman's path integral theory. It is concluded that whether the second-order temporal…

Optics · Physics 2016-03-18 Jianbin Liu , Dong Wei , Hui Chen , Yu Zhou , Huaibin Zheng , Hong Gao , Fu-li Li , Zhuo Xu

We perform a high resolution Fourier Transform Spectroscopy of optical sources in the few-photon regime based on the phenomenon of two-photon interference in a beam splitter. From the heterodyne interferogram between test and reference…

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

We have performed sub-Doppler spectroscopy on the narrow intercombination line of cold calcium atoms using the amplified output of a femtosecond laser frequency comb. Injection locking of a 657-nm diode laser with a femtosecond comb allows…

Atomic Physics · Physics 2010-03-19 T. M. Fortier , Y. Le Coq , J. E. Stalnaker , D. Ortega , S. A. Diddams , C. W. Oates , L. Hollberg

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Laser dynamics underpin a broad range of modern photonic technologies and continue to reveal rich nonlinear behaviors. However, existing spectroscopic tools, most notably time-stretched dispersive Fourier transform spectroscopy (TS-DFT),…

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

We report an experiment of observation of classical double-slit interference fringes of two-photon interference. In the experiment, a commercial continuous-wave multi-mode F-P laser diode without either mode-locked or frequency-locked is…

Quantum Physics · Physics 2024-02-26 Hongmin Liu

We characterize a new mid-infrared frequency comb generator based on difference frequency generation around 3.2 microns. High power per comb mode (>10-7 W/mode) is obtained over a broad spectral span (>700 nm). The source is used for direct…

Dual-frequency comb spectroscopy permits broadband precision spectroscopic measurements with short acquisition time. A dramatic improvement of the maximal spectral bandwidth and the minimal measurement time can be expected when the lasers'…

The extraction of information carried by light plays an increasingly important role in optical communication, imaging, and detection. However, the information can only be successfully extracted when the light pulse is comparably strong,…

Optics · Physics 2026-05-25 Zhen Yang , Zeng-Quan Yan , Li Wang , Xiao-Wei Wang , Ka-Di Zhu , Xian-Min Jin

We introduce a new parallelized approach to photothermal microscopy that utilizes mid-infrared dual-comb lasers, enabling simultaneous measurements at hundreds of wavelengths. This technology allows for high-speed, label-free chemical…

An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision…

Atomic Physics · Physics 2013-07-11 Itan Barmes , Stefan Witte , Kjeld S. E. Eikema

We demonstrate two solid-state sources of indistinguishable single photons. High resolution laser spectroscopy and optical microscopy were combined at T = 1.4 K to identify individual molecules in two independent microscopes. The Stark…

Quantum Physics · Physics 2009-11-13 R. Lettow , V. Ahtee , R. Pfab , A. Renn , E. Ikonen , S. Gotzinger , V. Sandoghdar

We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum…