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We use two femtosecond Erbium-doped fiber lasers with slightly different repetition rates to perform a modern type of Fourier transform spectroscopy without moving parts. The measurements are done in real time, and it takes less than 50…

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

As dual combs play a significant role in numerous high-precision measurements, their efficient generation has been widely researched. Although the single-cavity dual-comb generation can avoid the complex active stabilization methods,…

Optics · Physics 2025-05-02 Pan Guo , Yuan Gao , Yongjie Pu , Zhigang Zhao , Zhenhua Cong , Sha Wang

Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…

Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…

Optics · Physics 2016-08-29 Viktor O. Smolski , Honglei Yang , Jia Xu , Konstantin L. Vodopyanov

Fast (sub-second) spectroscopy with high spectral resolution is of vital importance for revealing quantum chemistry kinetics of complex chemical and biological reactions. Fourier transform (FT) spectrometers can achieve high spectral…

The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter…

Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…

We demonstrate a simple system for dual-comb spectroscopy based on two inherently coherent optical frequency combs generated via seeded parametric down-conversion. The inbuilt coherence is established by making the two combs share a common…

Optics · Physics 2024-08-13 Mikhail Roiz , Santeri Larnimaa , Touko Uotila , Mikko Narhi , Markku Vainio

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…

Open-path dual-comb spectroscopy (DCS) significantly enhances our understanding of regional trace gases. However, due to technical challenges, cost considerations, and eye-safety regulations, its sensing range and flexibility remain…

Two-photon interference underlies the functioning of many quantum photonics devices. It also serves as the prominent tool for testing the indistinguishability of distinct photons. However, as their time-spectral profile becomes more…

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure…

Quantum Physics · Physics 2020-07-15 Valérian Thiel , Alex O. C. Davis , Ke Sun , Peru D'Ornellas , Xian-Min Jin , Brian J. Smith

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

For the first time to our knowledge, a dual-comb laser based on thin-disk technology and its application to direct frequency comb spectroscopy are presented. The peak power (0.6 MW) and the average power (12 W) of our Yb:YAG thin-disk…

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

We introduce a novel laser-scanning optical microscopy technique that employs optical-frequency-comb (OFC) lasers. This method facilitates multimodal spectroscopic imaging by analyzing interferograms produced via a dual-comb spectroscopic…