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Multiphoton microscopy has enabled us to image cellular dynamics in vivo. However, the excitation wavelength for imaging with commercially available lasers is mostly limited between 650-1040 nm. Here we develop a femtosecond fiber laser…
Optical pulse shaping stands as a formidable technique in ultrafast optics, radio-frequency photonics, and quantum communications. While existing systems rely on bulk optics or integrated platforms with planar waveguide sections for spatial…
We report on the generation of 6.1 mJ, 3.8 fs pulses by the compression of a kHz Ti:sapphire laser in a large-aperture long hollow fiber. In order to find optimal conditions for spectral broadening at high pulse energies, we explore…
Synchronously pumped optical parametric oscillators (OPOs) provide uniquely versatile platforms to generate ultrafast mid-infrared pulses within a spectral range beyond the access of conventional mode-locked lasers. However, conventional…
Nonlinear optical phenomena in silicon such as self-focusing and multi-photon absorption are strongly dependent on the wavelength, energy and duration of the exciting pulse. Thus, a pronounced wavelength dependence of the sub-surface…
Molecular cavity optomechanics (COM) leverages ultrastrong interactions between confined optical fields and high-frequency molecular vibration, providing a unique platform for exploring high-frequency phonon dynamics. In this work, we…
We use shaped near-infrared (NIR) pulses to control the generation of coherent broadband ultraviolet (UV) radiation in an atomic resonance-mediated (2+1) three-photon excitation. Experimental and theoretical results are presented for phase…
Optical techniques for spatiotemporal control can produce laser pulses with custom amplitude, phase, or polarization structure. In nonlinear optics and plasma physics, the use of structured pulses typically follows a forward design…
The quantum cascade laser (QCL) has evolved to be a compact, powerful source of coherent mid-infrared (mid-IR) light. However, its fast gain dynamics strongly restricts the formation of ultrashort pulses. As such, the shortest pulses…
Single-photon laser ranging has widespread applications in remote sensing and target recognition. However, highly-sensitive light detection and ranging (LiDAR) has long been restricted in visible or near-infrared bands. An appealing quest…
Ultrafast optical excitation with intense mid-infrared and terahertz pulses has emerged as a new tool to control materials dynamically. As most experiments are performed with femtosecond pulse excitation, typical lifetimes of most…
Applications relying on mid-infrared radiation (Mid-IR, $\lambda\sim$ 3-30 $\mu$m) have progressed at a very rapid pace in recent years, stimulated by scientific and technological breakthroughs. Mid-IR cameras have propelled the field of…
The availability of intense, ultrashort coherent radiation sources in the infrared region of the spectrum is enabling the generation of attosecond X-ray pulses via high harmonic generation, pump-probe experiments in the "molecular…
Broadband microwave waveforms with programmable chirp shapes are captivating in numerous practical applications. Compared with electronic technology, photonic-assisted solutions exhibit excellent performance in bandwidth and flexibility,…
Femtosecond laser pulses enable the synthesis of light across the electromagnetic spectrum and provide access to ultrafast phenomena in physics, biology, and chemistry. Chip-integration of femtosecond technology could revolutionize…
We experimentally demonstrate a simple configuration for mid-infrared (MIR) frequency comb generation in quasi-phase-matched lithium niobate waveguides using the cascaded-$\chi^{(2)}$ nonlinearity. With nanojoule-scale pulses from an…
We describe the design of a new family of high spectral brightness narrow linewidth (NLW) mid-infrared (MIR) lasers of < 1 MHz anticipated linewidths with potential for operation at any target wavelength between 2.5 and 9.5 um. More…
Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field's oscillation period. However, synthesizing such a gate pulse is…
The spectrum of a CW field whose phase experiences a periodic sawtooth modulation is analyzed. Two types of the sawtooth phase modulation are considered. One is created by combining many harmonics of the fundamental frequency. The second is…
The availability of electromagnetic pulses with controllable field waveform and extremely short duration, even below a single optical cycle, is imperative to fully harness strong-field processes and to gain insight into ultrafast…