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It was generally assumed that weak van der Waals interactions exist between neighboring layers in the two-dimensional group-IV chalcogenides. Using PbSe as a prototypal example, however, we find additional strong coupling between the Pb-Pb…

Materials Science · Physics 2021-08-11 Z. P. Yin , C. Y. Sheng , R. Hu , S. H. Han , D. D. Fan , G. H. Cao , H. J. Liu

Two-dimensional layered materials have attracted tremendous attentions due to their extraordinary physical and chemical properties. Using first-principles calculations and Boltzmann transport theory, we give an accurate prediction of the…

Mesoscale and Nanoscale Physics · Physics 2019-02-13 Z. Z. Zhou , H. J. Liu , D. D. Fan , G. H. Cao , C. Y. Sheng

By using a first-principles approach, monolayer PbI$_2$ is found to have great potential in thermoelectric applications. The linear Boltzmann transport equation is applied to obtain the perturbation to the electron distribution by different…

Materials Science · Physics 2021-05-24 Bo Peng , Haodong Mei , Hao Zhang , Hezhu Shao , Ke Xu , Gang Ni , Qingyuan Jin , Costas M. Soukoulis , Heyuan Zhu

We present a detailed study of the charge transport, optical reflectivity, and thermal transport properties of n-type PbSe crystals. A strong scattering, mobility-limiting mechanism was revealed to be at play at temperatures above 500 K.…

We calculate the lattice thermal conductivities of the pyrite-type ZnSe2 at pressures of 0 and 10 GPa using the linearized phonon Boltzmann transport equation. We obtain a very low value [0.69 W/(mK) at room temperature at 0 GPa],…

Materials Science · Physics 2020-10-07 Tiantian Jia , Jesus Carrete , Zhenzhen Feng , Shuping Guo , Yongsheng Zhang , Georg K. H. Madsen

Recently SnSe compound was reported to have a peak thermoelectric figure-5 of-merit (ZT) of 2.62 at 923 K, but the ZT values at temperatures below 750 K are relatively low. In this work, the electronic structures of SnSe are calculated…

Materials Science · Physics 2015-04-09 Aijun Hong , Lin Li , Haixia Zhu , Zhibo Yan , Junming Liu , Zhifeng Ren

The electronic properties of the layered black phosphorus (black-P) and its monolayer counterpart phosphorene are investigated by using the first-principles calculations based on the density functional theory (DFT). The room-temperature…

Materials Science · Physics 2014-04-22 H. Y. Lv , W. J. Lu , D. F. Shao , Y. P. Sun

Thermoelectric technology is an alternate way to efficiently utilize the energy by converting waste heat into electricity. Thermoelectric requires material with low thermal conductivity to improves its thermoelectric performance. In this…

Materials Science · Physics 2021-01-22 Rajmohan Muthaiah , Jivtesh Garg

Tungsten diselenide (WSe2) emerges as a promising thermoelectric (TE) candidate due to its high thermopower (S), cost-effectiveness, and environmentally friendly characteristics. However, pristine WSe2 exhibits limited electrical…

In this first-principles study, we investigated the thermoelectric properties of the full-Heusler compound CsK$_2$Sb at different compressive strains. This material exhibits a valence band structure with significant effective mass…

Materials Science · Physics 2025-05-14 Øven A. Grimenes , G. Jeffrey Snyder , Ole M. Løvvik , Kristian Berland

We present a first principles based model of electron-phonon scattering mechanisms and thermoelectric transport at the L and $\Sigma$ valleys in <200b>$p$-type PbTe, accounting for their thermally induced shifts. Our calculated values of…

Materials Science · Physics 2020-09-30 Ransell D'Souza , Jiang Cao , José D. Querales-Flores , Stephen Fahy , Ivana Savić

Transient cooling phenomenon in two-dimensional materials is studied based on the phonon Boltzmann transport equation (BTE). Using a heating laser pulse to heat the two-dimensional disk geometry under the environment temperature, after the…

Mesoscale and Nanoscale Physics · Physics 2024-10-10 Chuang Zhang , Lei Wu

The thermoelectric properties of PbSe have significantly improved in recent years reaching figures of merit ZT 1.6. The transport properties of the hole doped high temperature thermoelectric material PbSe are particularly interesting and…

The thermoelectric properties of distorted bismuth (110) layer are investigated using first-principles calculations combined with the Boltzmann transport equation for both electrons and phonons. To accurately predict the electronic and…

Mesoscale and Nanoscale Physics · Physics 2016-06-07 L. Cheng , H. J. Liu , J. Zhang , J. Wei , J. H. Liang , P. H. Jiang , D. D. Fan , L. Sun , J. Shi

The electronic and transport properties of (10, 0) single-walled carbon nanotube are studied by performing the first-principles calculations and semi-classical Boltzmann theory. It is found that the (10, 0) tube exhibits considerably large…

Mesoscale and Nanoscale Physics · Physics 2016-01-06 P. H. Jiang , H. J. Liu , D. D. Fan , L. Cheng , J. Wei , J. Zhang , J. H. Liang , J. Shi

Using first-principles pseudopotential method and Boltzmann transport theory, we give a comprehensive understanding of the electronic and phonon transport properties of thermoelectric material BiCuSeO. By choosing proper hybrid functional…

Materials Science · Physics 2017-06-28 D. D. Fan , H. J. Liu , L. Cheng , J. Zhang , P. H. Jiang , J. Wei , J. H. Liang , J. Shi

The electronic and thermoelectric properties of one to four monolayers of MoS$_{2}$, MoSe$_{2}$, WS$_{2}$, and WSe$_{2}$ are calculated. For few layer thicknesses,the near degeneracies of the conduction band $K$ and $\Sigma$ valleys and the…

Materials Science · Physics 2014-04-03 Darshana Wickramaratne , Ferdows Zahid , Roger K. Lake

Thermoelectric properties of polycrystalline p-type ZrTe5 are reported in temperature (T) range 2 - 340 K. Thermoelectric power (S) is positive and reaches up to 458 uV/K at 340 K on increasing T. The value of Fermi energy 16 meV, suggests…

Materials Science · Physics 2017-09-13 M. K. Hooda , C. S. Yadav

In this study, we systematically investigate the thermal and electronic transport properties of two-dimensional PbSe/PbTe monolayer heterostructure by combining first-principles calculations, Boltzmann transport theory, and machine learning…

Materials Science · Physics 2026-02-27 Ruihao Tan , Kaiwang Zhang , Yue-Wen Fang

Using first-principles density-functional theory calculations, we predict the potential for unprecedented thermoelectric efficiency $zT=5$ at 800 K in $n$-type Ba$_{2}$BiAu full-Heusler compound. Such a high efficiency arises from an…

Materials Science · Physics 2019-02-06 Junsoo Park , Yi Xia , Vidvuds Ozoliņš
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