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Harnessing the optical properties of noble metals down to the nanometer-scale is a key step towards fast and low-dissipative information processing. At the 10-nm length scale, metal crystallinity and patterning as well as probing of surface…

The ability to control and modify infrared excitations in condensed matter is of both fundamental and application interests. Here we explore a system supporting low-energy excitations, in particular, mid-infrared localized plasmon modes and…

We theoretically investigate electron energy loss spectroscopy (EELS) of metallic nanoparticles in the optical frequency domain. Using a quasistatic approximation scheme together with a plasmon eigenmode expansion, we show that EELS can be…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Anton Hörl , Andreas Trügler , Ulrich Hohenester

We present an optical mode solver for a whispering gallery resonator coupled to an adjacent arbitrary shaped nano-particle that breaks the axial symmetry of the resonator. Such a hybrid resonator-nanoparticle is similar to what was recently…

Although fluorescence is the prevailing labeling technique in biosensing applications, sensitivity improvement is still a striving challenge. We show that coating standard microscope slides with nanoroughened silver films provides a high…

Instrumentation and Detectors · Physics 2013-07-29 Eric Le Moal , Sandrine Lévêque-Fort , Marie-Claude Pottier , Emmanuel Fort

Two-dimensional hexagonal boron nitride (hBN) has been known to host a variety of quantum emitters with properties suitable for a broad range of quantum photonic applications. Among them, the negatively charged boron vacancy (VB-) defect…

Nanostructured metal surfaces comprised of periodically arranged spherical voids are grown by electrochemical deposition through a self-assembled template. Detailed measurements of the angle- and orientation-dependent reflectivity reveal…

Optics · Physics 2007-05-23 T. A. Kelf , Y. Sugawara , J. J. Baumberg , M. Abdelsalam , P. N. Bartlett

We introduce an efficient computational scheme based on Macro Basis Function (MBF) method, to analyze the scattering of a plane wave by the V-shaped plasmonic optical nano-antennas. The polarization currents and the scattered fields for…

A many-body Green's function approach to the microscopic theory of plasmon-enhanced spectroscopy is presented within the context of localized surface-plasmon resonance spectroscopy and applied to investigate the coupling between…

Chemical Physics · Physics 2015-05-14 David J. Masiello , George C. Schatz

The temperature dependence of peak widths in high resolution angle-resolved photoelectron spectroscopy from quantum well states in ultra thin Ag films on V(100) has been used to determine the electron-phonon coupling constant, lambda, for…

Strongly Correlated Electrons · Physics 2009-10-31 T. Valla , M. Kralj , A. Siber , M. Milun , P. Pervan , P. D. Johnson , D. P. Woodruff

The ability to engineer localized surface plasmon resonances at large scale usually relies on precise nanoscale patterning. Here, we demonstrate that mid-infrared plasmonic responses can instead emerge in unpatterned polysilicon films…

We theoretically investigate several types of plasmonic slot waveguides for enhancing the measured signal in Raman spectroscopy, which is a consequence of electric field and Purcell factor enhancements, as well as an increase in…

The physics of electrons, photons, and their plasmonic interactions changes greatly when one or more dimensions are reduced down to the nanometer scale. For example, graphene shows unique electrical, optical, and plasmonic properties, which…

We present a theoretical study of the dispersion relation of surface plasmon resonances of mesoscopic metal-dielectric-metal microspheres. By analyzing the solutions to Maxwell's equations, we obtain a simple geometric condition for which…

Optics · Physics 2009-11-11 Keisuke Hasegawa , Charles A. Rohde , Miriam Deutsch

The vibrational density of states of silicon nanoparticles in the range from 2.3 to 10.3 nm is studied with the help of molecular-dynamics simulations. From these simulations the vibrational density of states and frequencies of bulk-like…

Materials Science · Physics 2011-01-20 R. Meyer , D. Comtesse

Hexagonal boron nitride (hBN) has emerged as a promising two-dimensional platform for quantum sensing, due to its optically addressable spin defects, such as the negatively charged boron vacancy ($V_{\text{B}}^-$). Despite hBN being…

We image the field enhancement at Ag nanostructures using femtosecond laser pulses with a center wavelength of 1.55 micrometer. Imaging is based on non-linear photoemission observed in a photoemission electron microscope (PEEM). The images…

Mesoscale and Nanoscale Physics · Physics 2015-03-09 Erik Mårsell , Esben W. Larsen , Cord L. Arnold , Hongxing Xu , Johan Mauritsson , Anders Mikkelsen

A strong electron-phonon interaction in a metal increases the electron density of states in the vicinity of the Fermi energy dramatically. This phenomenon is called electron-phonon mass enhancement. In this paper the question is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Gerd Bergmann

Localized plasmons in metallic nanostructures have been widely used to enhance nonlinear optical effects due to their ability to concentrate and enhance light down to extreme-subwavelength scales. As alternatives to noble metal…

Mesoscale and Nanoscale Physics · Physics 2015-02-24 Joel D. Cox , F. Javier Garcia de Abajo

Propagating atomic vibrational waves, phonons, rule important thermal, mechanical, optoelectronic and transport characteristics of materials. Thus the knowledge of phonon dispersion, namely the dependence of vibrational energy on momentum…

Materials Science · Physics 2019-10-09 Ryosuke Senga , Kazu Suenaga , Paolo Barone , Shigeyuki Morishita , Francesco Mauri , Thomas Pichler