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We investigated the influence of the photonic mode density (PMD) on the triplet dynamics of individual chromophores on a dielectric interface by comparing their response in the presence and absence of a nearby gold film. Lifetimes of the…

Optics · Physics 2009-11-13 F. D. Stefani , K. Vasilev , N. Bocchio , F. Gaul , A. Pomozzi , M. Kreiter

We report on experimental evidences of the preservation of energy-time entanglement for extraordinary plasmonic light transmission through sub-wavelength metallic hole arrays, and for long range surface plasmon polaritons. Plasmons are…

Quantum Physics · Physics 2013-01-22 Sylvain Fasel , Nicolas Gisin , Hugo Zbinden , Daniel Erni , Esteban Moreno , Frank Robin

Electron-electron scattering is one of the most important hot carrier relaxation pathways in plasmonic nanoparticles. Understanding the dynamics of this scattering process and the effects of this on excited state dephasing and relaxation is…

Chemical Physics · Physics 2026-03-09 Yanze Wu , George C. Schatz

We theoretically investigate charged collective modes in a two-dimensional conductor with hot electrons where the instantaneous mode frequencies gradually increase or decrease with time. We show that the loss compensation or even…

Mesoscale and Nanoscale Physics · Physics 2016-10-31 Zhiyuan Sun , D. N. Basov , M. M. Fogler

Bosonic condensates offer exciting prospects for studies of non-equilibrium quantum dynamics. Understanding the dynamics is particularly challenging in the sub-picosecond timescales typical for room temperature luminous driven-dissipative…

Plasmonic nanoparticles influence the absorption and emission processes of nearby emitters due to local enhancements of the illuminating radiation and the photonic density of states. Here, we use the plasmon resonance of metal nanoparticles…

Highly nonlinear optical processes, such as multiphoton photoemission, require high intensities, typically achieved with ultrashort laser pulses and, hence, were first observed with the advent of picosecond laser technology. An alternative…

The fluorescence of organic fluorophore molecules is enhanced when they are placed in contact with certain metals (Al, Ag, Cu, Au, etc.) whose surface plasmon waves couple into the radiative modes of the molecules and increase the radiative…

Mesoscale and Nanoscale Physics · Physics 2015-04-21 S. Sarkar , B. Kanchibotla , J. D. Nelson , J. D. Edwards , J. Anderson , G. C. Tepper , S. Bandyopadhyay

In our work we investigate the propagation of optical modes in nanoscale hybrid plasmonic waveguides. Frequency domain Maxwell equations based simulations are implemented to study properties of mixed modes in 3D. The results of our analysis…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

We have studied the plasmonic properties of aperiodic arrays of identical nanoparticles (NPs) formed by two opposite and equal graded-chains (a chain where interactions change gradually). We found that these arrays concentrate the external…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Natalia Esteves-López , Horacio M. Pastawski , Raúl A. Bustos-Marún

Light-driven plasmonic enhancement of chemical reactions on metal catalysts is a promising strategy to achieve highly selective and efficient chemical transformations. The study of plasmonic catalyst materials has traditionally focused on…

Materials Science · Physics 2021-06-16 Oscar A. Douglas-Gallardo , Connor L. Box , Reinhard J. Maurer

The collective response of metal nanostructures to optical excitation leads to localized plasmon generation with nanoscale field confinement driving applications in e.g. quantum optics, optoelectronics, and nanophotonics, where a bottleneck…

Plasmons in low-dimensional systems respresent an important tool for coupling energy into nanostructures and the localization of energy on the scale of only a few nanometers. Contrary to ordinary surface plasmons of metallic bulk materials,…

Mesoscale and Nanoscale Physics · Physics 2017-01-19 H. Pfnür , C. Tegenkamp , L. Vattuone

Surface plasmon resonances, the coherent oscillation of free electrons, can concentrate incident field into small volumes much smaller than the incident wavelength. The intense fields at these \textit{hot spots} enhance the light-matter…

Optics · Physics 2021-09-17 Mehmet Gunay

We demonstrate how the controlled positioning of a plasmonic nanoparticle modifies the photoluminescence of a single epitaxial GaAs quantum dot. The antenna particle leads to an increase of the luminescence intensity by about a factor of…

Resonant optical excitation was used to create a macroscopic non-equilibrium ensemble of dark excitons with unprecedentedly long lifetime in a two-dimensional (2D) electron system placed in a quantizing magnetic field. Exotic three-particle…

Mesoscale and Nanoscale Physics · Physics 2016-11-09 A. S. Zhuravlev , V. A. Kuznetsov , V. E. Bisti , L. V. Kulik , V. E. Kirpichev , I. V. Kukushkin

Optical polaritons appear when a material excitation strongly couples to the optical mode. Such strong coupling between molecular transitions and optical cavities results in far-reaching opportunities in modifying fundamental properties of…

The nonclassical modification of plasmon-assisted fluorescence enhancement is theoretically explored by placing two-level dipole emitters at the narrow gaps encountered in canonical plasmonic architectures, namely dimers and trimers of…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Christos Tserkezis , N. Asger Mortensen , Martijn Wubs

The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…

Mesoscale and Nanoscale Physics · Physics 2016-02-10 Philippe Roelli , Christophe Galland , Nicolas Piro , Tobias J. Kippenberg