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Lead halide perovskites have emerged as promising materials for optoelectronic applications due to their exceptional properties. In the all-inorganic CsPbBr3 perovskites, ferroelastic domains formed during phase transitions enhance bulk…

We have performed a systematic angle-resolved photoemission spectroscopy (ARPES) study of the high-Tc cuprates La2-xSrxCuO4, ranging from the underdoped insulator to the superconductor to the overdoped metal. We have revealed a systematic…

Strongly Correlated Electrons · Physics 2009-11-11 T. Yoshida , X. J. Zhou , D. H. Lu , Seiki Komiya , Yoichi Ando , H. Eisaki , T. Kakeshita , S. Uchida , Z. Hussain , Z. -X. Shen , A. Fujimori

The low energy electronic structure of LaFeAsO1-xHx (0.0 < x < 0.60), the system which exhibits two superconducting domes in its phase diagram, is investigated by utilizing the laser photoemission spectroscopy. From the precise…

Superconductivity · Physics 2017-02-08 A. Nakamura , T. Shimojima , T. Sonobe , K. Ishizaka , W. Malaeb , S. Shin , S. Iimura , S. Matsuishi , H. Hosono

The in-plane resistivity of the high-temperature oxide superconductor La$_{2-x}$Sr$_{x}$CuO$_{4}$ [LSCO] shows a strong growth of a contribution linear in temperature as the doping is reduced in the overdoped region toward optimal. This…

Strongly Correlated Electrons · Physics 2013-01-23 Jonathan M. Buhmann , Matthias Ossadnik , T. M. Rice , Manfred Sigrist

Polar discontinuities occurring at interfaces between two different materials constitute both a challenge and an opportunity in the study and application of a variety of devices. In order to cure the large electric field occurring in such…

Surfaces and interfaces offer new possibilities for tailoring the many-body interactions that dominate the electrical and thermal properties of transition metal oxides. Here, we use the prototypical two-dimensional electron liquid (2DEL) at…

We report a strategy to induce superconductivity in the BiS$_2$-based compound LaOBiS$_2$. Instead of substituting F for O, we increase the charge-carrier density (electron dope) via substitution of tetravalent Th$^{+4}$, Hf$^{+4}$,…

Superconductivity · Physics 2013-05-22 D. Yazici , K. Huang , B. D. White , I. Jeon , V. W. Burnett , A. J. Friedman , I. K. Lum , M. Nallaiyan , S. Spagna , M. B. Maple

In the present study, we investigate the thermodynamic properties of the Ba$_{x}$K$_{1-x}$BiO$_{3}$ (BKBO) superconductor in the under- ($x=0.5$) and over-doped ($x=0.7$) regime, within the framework of the Migdal-Eliashberg formalism. The…

Superconductivity · Physics 2018-07-04 D. Szczȩśniak , A. Z. Kaczmarek , R. Szczȩśniak , S. V. Turchuk , H. Zhao , E. A. Drzazga

The electronic structure of Li-doped Ni$_{1-x}$Fe$_x$O has been investigated using photoemission spectroscopy (PES) and x-ray absorption spectroscopy (XAS). The Ni $2p$ core-level PES and XAS spectra were not changed by Li doping. In…

Electronic states near surface regions can be distinct from bulk states, which are paramount in understanding various physical phenomena occurring at surfaces and in applications in semiconductors, energy, and catalysis. Here, we report an…

The electronic structure of electron-doped polycrystalline Mg$_{1-x}$Al$_{x}$(B$_{1-y}$C$_{y}$)$_2$ was examined by electron energy-loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM) and first-principle…

Superconductivity · Physics 2007-05-23 R. F. Klie , J. C. Zheng , Y. Zhu , A. J. Zambano , L. D. Cooley

We present electrical transport measurements of heterostructures comprised of BaTiO$_3$ and Ba$_{1-x}$Sr$_x$TiO$_3$ epitaxially grown on Ge. The Sr-alloying imparts compressive strain to the BaTiO$_3$, which enables the thermal expansion…

Materials Science · Physics 2014-03-05 J. H. Ngai , D. P. Kumah , C. H. Ahn , F. J. Walker

We demonstrate that the interfacial dipole associated with bonding across the SrTiO3/Si heterojunction can be tuned through space charge, thereby enabling the band alignment to be altered via doping. Oxygen impurities in Si act as donors…

We use density functional theory methods to study the electronic structures of a series of $s-p$ cubic perovskites $ABX_{3}$: the experimentally available SrBiO$_{3}$, BaBiO$_{3}$, BaSbO$_3$, CsTlF$_{3}$, and CsTlCl$_{3}$, as well as the…

To investigate the scope of ferroelectric behavior in La-substituted BiFeO3 films, LaxBi1-xFeO3 epitaxial films were synthesized using off-axis co-sputtering on SrTiO3(001) and DyScO3(110) substrates with a SrRuO3 bottom electrode layer. A…

The band gap engineering of group IV semiconductors has not been well explored theoretically and experimentally, except for SiGe. Recently, GeSn has attracted much attention due to the possibility of obtaining a direct band gap in this…

Materials Science · Physics 2022-03-22 Maciej P Polak , Paweł Scharoch , Robert Kudrawiec

We have performed an angle resolved photoemission spectroscopy (ARPES) study of lightly-doped to underdoped YBa2Cu3Oy (YBCO) untwinned single crystals and a core-level x-ray photoemission spectroscopy (XPS) study of YBCO single and…

We found that a surface state induced by hydrogenation on the surface of SrTiO$_{3}$(001) (STO) did not obey the rigid band model, which was confirmed by in situ electrical resistivity measurements in ultrahigh vacuum. With exposure of…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Y. Takeuchi , R. Hobara , R. Akiyama , A. Takayama , S. Ichinokura , R. Yukawa , I. Matsuda , S. Hasegawa

Heterostructures are ubiquitous in many optoelectronic devices and as photocatalysts. One of the key features of a heterojunction is the proper band alignment between the two materials. Estimation of the correct relative band positions with…

Mesoscale and Nanoscale Physics · Physics 2024-08-13 Raheel Hammad , Snehith Adabala , Soumya Ghosh

Doping of strongly layered ionic oxides is an established paradigm for creating novel electronic behavior. This is nowhere more apparent than in superconductivity, where doping gives rise to high temperature superconductivity in cuprates…

Superconductivity · Physics 2013-07-17 E. R. Ylvisaker , W. E. Pickett