Related papers: Second harmonic and sum-frequency generations from…
Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…
Recent experiments and calculations in topological semimetals have observed anomalously strong second-order optical nonlinearity, but yet whether the enhancement also occurs at surfaces of topological semimetals in general remains an open…
Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads…
We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…
We study surface second-harmonic generation (SHG) from a singular plasmonic structure consisting of touching metallic wires. We use the technique of transformation optics and relate the structure to a rather simpler geometry, a slab…
Vibrational sum- and difference-frequency generation (SFG and DFG) spectroscopy probes the nonlinear response of interfaces at mid-infrared (MIR) wavelengths while detecting upconverted signals in the visible. Recent work has moved from…
Two-dimensional transition metal dichalcogenides (TMDC) have shown promise for various applications in optoelectronics and so-called valleytronics. Their operation and performance strongly depend on the stacking of individual layers. Here,…
Second Harmonic Generation Microscopy (SHG) is generally acknowledged as a powerful tool for the label-free 3D visualization of tissues and advanced materials, with one of its most popular applications being collagen imaging. Although the…
Nonlinear frequency conversion plays a crucial role in advancing the functionality of next-generation optical systems. Portable metrology references and quantum networks will demand highly efficient second-order nonlinear devices, and the…
The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and…
Substantial enhancement of nonlinear high-order harmonics generation based on Fano-resonant nanostructures has received growing interest due to their promising potential for developing integrated and advanced next-generation nanophotonic…
Integrated nonlinear photonic technologies, even with state-of-the-art fabrication with only a few nanometer geometry variations, face significant challenges in achieving wafer-scale yield of functional devices. A core limitation lies in…
Optical second-harmonic generation is demonstrated to be a sensitive probe of the buried interface between the lattice matched semiconductors gallium phosphide and silicon with (001) orientation. Rotational anisotropy measurements of SHG…
Metasurfaces with local phase tuning by subwavelength elements promise unprecedented possibilities for ultra-thin and multifunctional optical devices, in which geometric phase design is widely used due to its resonant-free and large…
Successful phase-matching methods for Third Harmonics Generation (THG) include phase-matching in birefringent crystal and quasi-phase-matching (QPM) in crystal with periodically poled domains. However, these methods are not feasible in some…
Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…
We combine modeling and experiments to investigate second- and third-harmonic generation (SHG/THG) in metal-indium tin oxide (ITO) metasurfaces. Linear optics at normal incidence show moderate field enhancement near the ITO…
Integrated waveguides exhibiting efficient second-order nonlinearities are crucial to obtain compact and low power optical signal processing devices. Silicon nitride (SiN) has shown second harmonic generation (SHG) capabilities in resonant…
The resonance effects on the optical second harmonic generation from 140 nm silver nanoparticles is studied experimentally by hyper-Rayleigh scattering and numerically by finite element method calculations. We find that the interferences…
We study second-harmonic generation (SHG) arising from surface nonlinearity at a metal-dielectric interface using a spectral decomposition method. Since our method avoids the need to consider the generalized boundary condition across the…