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Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…

Chemical Physics · Physics 2025-03-07 Andrés Ordóñez , Patricia Vindel-Zandbergen , David Ayuso

We provide a statistically robust and accurate framework to measure and track the polarisation state of light employing Hong-Ou-Mandel interference. This is achieved by combining the concepts of maximum likelihood estimation and Fisher…

Quantum Physics · Physics 2020-02-19 Natapon Harnchaiwat , Feng Zhu , Niclas Westerberg , Erik Gauger , Jonathan Leach

Attosecond noncollinear four wave mixing spectroscopy with one attosecond extreme ultraviolet (XUV) pulse and two few-cycle near-infrared (NIR) pulses was used to measure the autoionization decay lifetimes of inner valence electronic…

Temporal imaging systems are outstanding tools for single-shot observation of optical signals that have irregular and ultrafast dynamics. They allow long time windows to be recorded with femtosecond resolution, and do not rely on complex…

We propose a simple scheme to measure squeezing and phase properties of a harmonic oscillator. We treat in particular the case of a the field, but the scheme may be easily realized in ion traps. It is based on integral transforms of…

Quantum Physics · Physics 2013-03-13 G. T. Rubin-Linares , H. Moya-Cessa

Quantum imaging with undetected light (QIUL) can retrieve amplitude and phase information of an object by exploiting the quantum correlations of photon-pairs generated through spontaneous parametric down conversion (SPDC), where the…

Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultra-violet (XUV)…

Atomic Physics · Physics 2022-02-02 Lorenz Drescher , Tobias Witting , Oleg Kornilov , Marc J. J. Vrakking

Photoionization is a key step in many attosecond processes. Accurately determining the photoionization time delay is critical to understanding electron dynamics during and after ionization and can guide future efforts to manipulate electron…

Atomic Physics · Physics 2026-02-26 J. Aygun , D. Yaacoub , A. L. Harris

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

We have operated a Medipix2 CMOS readout chip, with amplifying, shaping and charge discriminating front-end electronics integrated on the pixel-level, as a highly segmented direct charge collecting anode in a three-stage gas electron…

Instrumentation and Detectors · Physics 2008-11-26 A. Bamberger , K. Desch , U. Renz , M. Titov , N. Vlasov , P. Wienemann , A. Zwerger

Time-resolved optical filtering (TROF) measures the spectrogram or sonogram by a fast photodiode followed a tunable narrowband optical filter. For periodic signal and to match the sonogram, numerical TROF algorithm is used to find the…

Optics · Physics 2013-01-15 KeangPo Ho , Hsi-Cheng Wang , Hau-Kai Chen , Cheng-Chen Wu

Our last experimental results on the realization of a measurement-conditional unitary operation at single photon level are presented. This gate operates by rotating by $90^o$ the polarization of a photon produced by means of Type-II…

Quantum Physics · Physics 2015-06-26 M. Genovese , G. Brida , M. Chekhova , M. Gramegna , L. Krivitsky , S. Kulik , M. L. Rastello

We propose a method to map the conventional optical interferometry setup into quantum circuits. The unknown phase shift inside a Mach-Zehnder interferometer in the presence of photon loss is estimated by simulating the quantum circuits. For…

Quantum Physics · Physics 2021-08-04 Peyman Najafi , Ghasem Naeimi , Shahpoor Saeidian

Molecular chirality is a key design property for many technologies including bioresponsive imaging, circularly polarized light detection and emission, molecular motors and switches. Imaging and manipulating the primary steps of transient…

A proposed phase-estimation protocol based on measuring the parity of a two-mode squeezed-vacuum state at the output of a Mach-Zehnder interferometer shows that the Cram\'{e}r-Rao sensitivity is sub-Heisenberg [Phys.\ Rev.\ Lett.\ {\bf104},…

Quantum Physics · Physics 2017-05-17 Zixin Huang , Keith R. Motes , Petr M. Anisimov , Jonathan P. Dowling , Dominic W. Berry

Highly intense, sub-picosecond terahertz (THz) pulses can be used to induce ultrafast temperature jumps (T-jumps) in liquid water. A supercritical state of gas-like water with liquid density is established, and the accompanying structural…

Chemical Physics · Physics 2019-01-24 Caroline Arnold , Ludger Inhester , Sergio Carbajo , Ralph Welsch , Robin Santra

Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the beam's intensity profile or wave front. While shaping and controlling the light field is a highly researched topic,…

We demonstrate coherent control over the photoelectron circular dichroism in randomly oriented chiral molecules, based on quantum interference between multiple photoionization pathways. To significantly enhance the chiral signature, we use…

Quantum Physics · Physics 2019-01-16 R. Esteban Goetz , Christiane P. Koch , Loren Greenman

Holographic optical tweezers can be applied to manipulate microscopic particles in arbitrary optical patterns, which classical optical tweezers cannot do. This ability relies on accurate computer-generated holography (CGH), yet most CGH…

Optics · Physics 2019-10-21 Xionggui Tang , Fan Nan , Fei Han , Zijie Yan