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We report a voltage-induced oxidation technique using conductive atomic force microscopy to enhance the single-photon purity and reproducibility of quantum emitters in monolayer tung-sten diselenide (WSe2). By applying a controlled electric…

Monolayers and multilayers of semiconducting transition metal dichalcogenides (TMDCs) offer an ideal platform to explore valley-selective physics with promising applications in valleytronics and information processing. Here we manipulate…

Moir\'e superlattices created by stacking atomic layers of transition metal dichalcogenide semiconductors have emerged as a class of fascinating artificial photonic and electronic materials. An appealing attribute of these structures is the…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Yueh-Chun Wu , Matthew DeCapua , ZhongChen Xu , Takashi Taniguchi , Kenji Watanabe , YouGuo Shi , Jun Yan

For over a decade, cold atoms in lattice potentials have been an attractive platform to simulate phenomena known from solid state theory, as the Mott-insulator transition. In contrast, the field of photonics usually deals with…

Structural defects can crucially impact the optical response of monolayer (ML) thick materials as they enable trapping sites for excitons. These trapped excitons appear in photoluminescence spectra as new emissions below the free bright…

Mesoscale and Nanoscale Physics · Physics 2021-09-29 R. Eddhib , S. Ayari , A. Hichri , S. Jaziri

We demonstrate robust power- and wavelength-dependent optical bistability in fully suspended monolayers of WSe2 near the exciton resonance. Bistability has been achieved under continuous-wave optical excitation at an intensity level of 10^3…

Mesoscale and Nanoscale Physics · Physics 2018-05-23 Hongchao Xie , Shengwei Jiang , Jie Shan , Kin Fai Mak

We observe the interlayer A1s^I, A2s^I, and B1s^I excitons in bilayer WSe2 under applied electric fields using reflectance contrast spectroscopy. Remarkably, these interlayer excitons remain optically bright despite being well separated…

Single-photon sources with near-unity efficiency and indistinguishability play a major role in the development of quantum technologies. However, on-demand excitation of the emitter imposes substantial limitations to the source performance.…

Quantum Physics · Physics 2023-05-30 Luca Vannucci , Niels Gregersen

Development of stable room-temperature bright single-photon emitters using atomic defects in hexagonal-boron nitride flakes (h-BN) provides significant promises for quantum technologies. However, an outstanding challenge in h-BN is creating…

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

Materials Science · Physics 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

With the both spin and valley degrees of freedom, the low-lying excitonic spectra of photo-excited transition-metal dichalcogenide monolayers (TMDC-MLs) are featured by rich fine structures, comprising the intra-valley bright exciton states…

Mesoscale and Nanoscale Physics · Physics 2019-04-10 Guan-Hao Peng , Ping-Yuan Lo , Wei-Hua Li , Yan-Chen Huang , Yan-Hong Chen , Chi-Hsuan Lee , Chih-Kai Yang , Shun-Jen Cheng

Advanced quantum technologies, as well as fundamental tests of quantum physics, crucially require the interference of multiple single photons in linear-optics circuits. This interference can result in the bunching of photons into higher…

Quantum Physics · Physics 2021-05-26 P. Zapletal , T. Darras , H. Le Jeannic , A. Cavaillès , G. Guccione , J. Laurat , R. Filip

Single photon emitters often rely on a strong nonlinearity to make the behaviour of a quantum mode susceptible to a change in the number of quanta between one and two. In most systems the strength of nonlinearity is weak, such that changes…

Mesoscale and Nanoscale Physics · Physics 2011-01-13 T C H Liew , V Savona

Monolayer semiconductors are atomically thin quantum wells with strong confinement of electrons in two-dimensional (2D) plane. Here, we experimentally study the out-of-plane polarizability of excitons in hBN-encapsulated monolayer WSe$_{2}$…

Mesoscale and Nanoscale Physics · Physics 2019-02-19 Ivan A. Verzhbitskiy , Daniele Vella , Kenji Watanabe , Takashi Taniguchi , Goki Eda

Single-photon sources are used in numerous quantum technologies, from sensing and imaging to communication, making the accurate modeling of their emissions essential. In this work, we propose a statistical framework for describing…

Optical resonators are a powerful platform to control the spontaneous emission dynamics of excitons in solid-state nanostructures. Here, we study a MoSe$_2$-WSe$_2$ van-der-Waals heterostructure that is integrated in a widely tunable open…

Photonic integrated circuits (PICs) enable miniaturization of optical quantum circuits because several optic and electronic functionalities can be added on the same chip. Single photon emitters (SPEs) are central building blocks for such…

Twisted bilayers of two-dimensional (2D) materials have emerged as a highly tunable platform to study and engineer properties of excitons. However, the atomistic description of these properties has remained a significant challenge as a…

Materials Science · Physics 2025-03-13 Indrajit Maity , Arash A. Mostofi , Johannes Lischner

Momentum resolved electron energy-loss spectroscopy was used to measure the dispersions of excitons in a free-standing monolayer of WSe2. Besides the parabolically dispersed valley excitons, a sub-gap dispersive exciton was observed at…

Materials Science · Physics 2020-03-04 Jinhua Hong , Ryosuke Senga , Thomas Pichler , Kazu Suenaga

We study the screened dynamics of the nonequilibrium excitonic consensate forming in a bulk WSe$_{2}$ when illuminated by coherent light resonant with the lowest-energy exciton. Intervalley scattering causes electron migration from the…

Mesoscale and Nanoscale Physics · Physics 2021-06-16 E. Perfetto , G. Stefanucci
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