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We present a fully three-dimensional kinetic framework for modeling intense short pulse lasers interacting with dielectric materials. Our work modifies the open-source Particle-In-Cell (PIC) code EPOCH to include new models for molecular…

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

Atomic Physics · Physics 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

We consider the motion of charge carriers in a bulk wide-gap dielectric interacting with a few-cycle laser pulse. A semiclassical model based on Bloch equations is applied to describe the emerging time-dependent macroscopic currents for…

Mesoscale and Nanoscale Physics · Physics 2013-07-22 Peter Foldi , Mihaly G. Benedict , Vladislav S. Yakovlev

In this manuscript we present a theoretical framework and its numerical implementation to simulate the out-of-equilibrium electron dynamics induced by the interaction of ultrashort laser pulses in condensed-matter systems. Our approach is…

The electron dynamics in dielectric materials induced by intense femtosecond laser pulses is theoretically addressed. The laser driven temporal evolution of the energy distribution of electrons in the conduction band is described by a…

Mesoscale and Nanoscale Physics · Physics 2016-11-23 L. Barilleau , G. Duchateau , B. Chimier , G. Geoffroy , V. Tikhonchuk

We provide analytic solutions of the optical Bloch equations for a two-level system interacting with a broadband light field. We will focus on two special examples: incident light with a Lorentzian spectral density and the limit of incident…

Disordered Systems and Neural Networks · Physics 2007-05-23 Tom Savels , Allard P. Mosk , Ad Lagendijk

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

We predict that optical Bloch oscillations can be observed in layered structures with left-handed metamaterials and zero average refractive index where the layer thickness varies linearly across the structure. We demonstrate a new type of…

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We present a time-domain model for the simulation of light-matter interaction in semiconductors in arbitrary geometries and across a wide range of excitation conditions. The electromagnetic field is treated classically using the…

Optics · Physics 2015-01-21 Robert Buschlinger , Michael Lorke , Ulf Peschel

In laser-plasma interactions it is widely accepted that a non-uniform interaction surface will invariably seed hydrodynamic instabilities and a growth in the amplitude of the initial modulation. Recent experimental results [Dromey, Nat.…

Plasma Physics · Physics 2016-03-02 S. G. Rykovanov , H. Ruhl , J. Meyer-ter-Vehn , R. Hoerlein , B. Dromey , M. Zepf , G. D. Tsakiris

We study the nonequilibrium dynamics of photoinduced phase transitions in charge ordered (CO) systems with a strong electron-lattice interaction and analyze the interplay between electrons, periodic lattice distortions, and a phonon thermal…

Strongly Correlated Electrons · Physics 2018-03-22 Linghua Zhu , Tsezar F. Seman , Michel van Veenendaal , Keun Hyuk Ahn

The equations-of-motion for the density matrix are derived in a multiband model to describe the response of semiconductors (bulk or quantum well structures) under optical excitation with arbitrary polarization. The multiband model used,…

Condensed Matter · Physics 2016-08-16 U. Rössler

Laser excitation of nanometer-sized atomic and molecular clusters offers various opportunities to explore and control ultrafast many-particle dynamics. Whereas weak laser fields allow the analysis of photoionization, excited-state…

Atomic and Molecular Clusters · Physics 2010-06-15 Th. Fennel , K. -H. Meiwes-Broer , J. Tiggesbaumker , P. -G. Reinhard , P. M. Dinh , E. Suraud

A beyond electric-dipole light-matter theory is needed to describe emerging X-ray and THz applications for characterization and control of quantum materials but inaccessible as nondipole lattice-aperiodic terms impede on the use of Bloch's…

A short, tutorial introduction to some basic concepts of laser-plasma interactions at ultra-high intensities is given. The selected topics include a) elements of the relativistic dynamics of an electron in electromagnetic fields, including…

Plasma Physics · Physics 2019-08-12 Andrea Macchi

A simplified model for a collective dynamics in ionic melts is proposed for the description of optic-like excitations. Within a polarization model of ionic melt the analytical expressions for optic and relaxation dipole modes are obtained.…

Soft Condensed Matter · Physics 2015-12-09 B. Markiv , M. Tokarchuk

We derive a set of optical Bloch equations (OBEs) directly from the minimal-coupling Hamiltonian density of the bound-state quantum electrodynamics (bound-state QED). Such optical Bloch equations are beyond the former widely-used ones due…

Atomic Physics · Physics 2012-09-05 Wen-Zhuo Zhang , Wu-Ming Liu

The dynamics of an electron in a strong laser field can be significantly altered by radiation reaction. This usually results in a strongly damped motion, with the electron losing a large fraction of its initial energy. Here we show that the…

Plasma Physics · Physics 2014-02-12 Matteo Tamburini , Christoph H. Keitel , Antonino Di Piazza

Optical response of free-electron gas leads to inherent nonlinear optical behaviour of nanostructured plasmonic materials enabled via both strong local field enhancements and inherent complex electron dynamics. We present a comprehensive…

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