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A series of experiments demonstrate that strong light-matter coupling between vibrational excitations in isotropic solutions of molecules and resonant infrared optical microcavity modes leads to modified thermally-activated kinetics.…

Chemical Physics · Physics 2020-06-23 Jorge A. Campos-Gonzalez-Angulo , Joel Yuen-Zhou

Polaritons are compositional light-matter quasiparticles that arise as a result of strong coupling between a vacuum field of a resonant optical cavity and electronic excitations in quantum emitters. Reaching such a regime is often hard, as…

Light-matter strong coupling (LMSC) is intriguing state in which light and matter are coherently hybridized inside cavity. It has been gaining widespread recognition as an excellent way for controlling material properties without any…

Optics · Physics 2024-03-19 Daichi Okada , Fumito Araoka

Recent experiments have demonstrated that light and matter can mix together to an extreme degree, and previously uncharted regimes of light-matter interactions are currently being explored in a variety of settings. The so-called ultrastrong…

Quantum Physics · Physics 2019-06-19 P. Forn-Díaz , L. Lamata , E. Rico , J. Kono , E. Solano

Quantum light-matter systems at strong coupling are notoriously challenging to analyze due to the need to include states with many excitations in every coupled mode. We propose a nonperturbative approach to analyze light-matter correlations…

Mesoscale and Nanoscale Physics · Physics 2021-04-15 Yuto Ashida , Atac Imamoglu , Eugene Demler

We identify form-stable coupled excitations of light and matter (``dark-state polaritons'') associated with the propagation of quantum fields in Electromagnetically Induced Transparency. The properties of the dark-state polaritons such as…

Quantum Physics · Physics 2009-11-06 M. Fleischhauer , M. D. Lukin

We observe natural exceptional points in the excitation spectrum of an exciton-polariton system by optically tuning the light-matter interactions. The observed exceptional points do not require any spatial or polarization degrees of freedom…

The electronic interaction between an optically active singlet state ($S_1S_0$) and a dark state of singlet multiplicity, known as correlated triplet pair ($^1[TT]$), plays a crucial role in the effective transformation from $S_1S_0$ to…

In the regime of ensemble vibrational strong coupling (VSC), a macroscopic number $N$ of molecular transitions couple to each resonant cavity mode, yielding two hybrid light-matter (polariton) modes, and a reservoir of $N-1$ dark states…

Chemical Physics · Physics 2020-04-03 Jorge Campos-Gonzalez-Angulo , Raphael F. Ribeiro , Joel Yuen-Zhou

There is growing interest in using strongly coupled organic microcavities to tune molecular dynamics, including the electronic and vibrational properties of molecules. However, very little attention has been paid to the utility of cavity…

Materials Science · Physics 2024-06-12 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

We examine the photoluminescence of highly-excited exciton-polariton condensates in semiconductor microcavities. Under strong pumping, exciton-polariton condensates have been observed to undergo a lasing transition where strong coupling…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Natsuko Ishida , Tim Byrnes , Tomoyuki Horikiri , Franco Nori , Yoshihisa Yamamoto

Polaritons, formed as a result of strong hybridization of matter with light, are promising for important applications including organic solar cells, optical logic gates, and qubits. Owing to large binding energies of Frenkel excitons…

The experimental realization of strong light-matter coupling with molecules initiated the rapidly evolving field of molecular polaritonics. Most studies focus on how exciton polaritons, which combine electronic excitations with confined…

Chemical Physics · Physics 2025-09-10 Lucas Borges , Thomas Schnappinger , Markus Kowalewski

Strong light-matter coupling occurs when the coupling strength between a confined electromagnetic mode and a molecular resonance exceeds losses to the environment. The study of strong coupling has been motivated by applications such as…

Mesoscale and Nanoscale Physics · Physics 2022-04-27 Philip A. Thomas , Kishan S. Menghrajani , William L. Barnes

The optical hybridization of the electronic states in strongly coupled molecule-cavity systems have revealed unique properties such as lasing, room temperature polariton condensation, and the modification of excited electronic landscapes…

We demonstrate room temperature optical trapping and generation of high-order angular harmonics in exciton-polariton condensates in a monocrystalline CsPbBr$_3$ perovskite-filled microcavity. Using an annular nonresonant excitation profile…

While the search for topological triplet-pairing superconductivity has remained a challenge, recent developments in optically stabilizing metastable superconducting states suggest a new route to realizing this elusive phase. Here, we devise…

Superconductivity · Physics 2024-03-11 Steven Gassner , Clara S. Weber , Martin Claassen

Dressing quantum states of matter with virtual photons can create exotic effects ranging from vacuum-field modified transport to polaritonic chemistry, and may drive strong squeezing or entanglement of light and matter modes. The…

Quantum Physics · Physics 2023-09-14 J. Mornhinweg , L. Diebel , M. Halbhuber , M. Prager , J. Riepl , T. Inzenhofer , D. Bougeard , R. Huber , C. Lange

We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton…

Mesoscale and Nanoscale Physics · Physics 2011-11-15 K. Müller , G. Reithmaier , E. C. Clark , V. Jovanov , M. Bichler , H. J. Krenner , M. Betz , G. Abstreiter , J. J. Finley

Polaritonic chemistry investigates the possible modification of chemical and photochemical reactions by means of strong light-matter coupling in optical cavities, as demonstrated in numerous experiments over the last few years. These…

Quantum Physics · Physics 2025-07-30 Lucas Borges , Thomas Schnappinger , Markus Kowalewski