Related papers: Dual-comb spectroscopy for high-temperature reacti…
Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…
Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…
A phase-stabilized femtosecond laser comb is directly used for high-resolution spectroscopy and absolute optical frequency measurements of one- and two-photon transitions in laser-cooled \rb atoms. Absolute atomic transition frequencies,…
Hyperspectral imaging provides spatially resolved spectral information. Utilising dual frequency combs as active illumination sources, hyperspectral imaging with ultra-high spectral resolution can be implemented in a scan-free manner when a…
Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency…
We present an experimental and theoretical investigation of two-photon direct frequency-comb spectroscopy performed through velocity-selective excitation. In particular, we explore the effect of repetition rate on the…
Optical frequency combs based on mode-locked lasers have revolutionised the field of metrology and precision spectroscopy by providing precisely calibrated optical frequencies and coherent pulse trains. Amplification of the pulsed output…
Laser absorption Doppler velocimeters use a crossed-beam configuration to cancel error due to laser frequency drift and absorption model uncertainty. This configuration complicates the spatial interpretation of the measurement since the two…
Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…
We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…
We report the measurement of sub-Doppler double-resonance transitions in methane using a 3.3 $\mu$m continuous wave optical parametric oscillator to pump transitions in the fundamental $\nu_3$ band and a 1.67 $\mu$m frequency comb to probe…
Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…
We use optical-optical double-resonance (OODR) spectroscopy to measure for the first time hot-band transitions of ethylene (C${_2}$H${_4}$) between states in the 3000 cm$^{-1}$ and 9000 cm$^{-1}$ energy ranges. A 3.2 ${\mu}$m continuous…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…
Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…
We present a complex-valued electric field model for experimentally observed cavity transmission in coherent cavity-enhanced (CE) multiplexed spectroscopy (i.e., dual-comb spectroscopy, DCS). The transmission model for CE-DCS differs from…
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…
We report a precision realization of photonic thermometry using dual-comb spectroscopy to interrogate a $\pi$-phase-shifted fiber Bragg grating. We achieve read-out stability of 7.5 mK at 1 s and resolve temperature changes of similar…
It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…