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We demonstrate the performance of a dual frequency comb QCL spectrometer for the application of vibrational Stark spectroscopy. Measurements performed on fluorobenzene with the dual-comb spectrometer (DCS) were compared to results obtained…

Chemical Physics · Physics 2019-11-22 Urszula Szczepaniak , Samuel H. Schneider , Raphael Horvath , Jacek Kozuch , Markus Geiser

Mid-infrared dual-comb spectroscopy has the potential to supplant conventional high-resolution Fourier transform spectroscopy in applications that require high resolution, accuracy, signal-to-noise ratio, and speed. Until now, dual-comb…

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…

Optics · Physics 2026-04-30 Pei-Ling Luo , I-Yun Chen

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

Accurate parameters of molecular hot-band transitions, i.e., those starting from vibrationally excited levels, are needed to accurately model high-temperature spectra in astrophysics and combustion, yet laboratory spectra measured at high…

Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…

Here, ultra-low relative phase jitters over a wide optical spectrum were achieved for dual Ti:Sapphire optical frequency combs. The two optical frequency combs were independently phase-locked to a Sr optical lattice clock laser delivered…

Optics · Physics 2022-05-25 Eunmi Chae , Kota Nakashima , Kosuke Yoshioka

Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…

Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…

Dual-comb spectroscopy (DCS) is useful for gas spectroscopy due to high potential of optical frequency comb (OFC). However, fast Fourier transform (FFT) calculation of a huge amount of temporal data spends significantly longer time than the…

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

We demonstrate fiber mode-locked dual frequency comb spectroscopy for broadband, high resolution measurements in a rapid compression machine (RCM). We apply an apodization technique to improve the short-term signal-to-noise-ratio (SNR),…

We demonstrate 1D simultaneous laser cooling of $^{87}$Rb and $^{85}$Rb atoms using an optical frequency comb. By adjusting the pulse repetition frequency and the offset frequency, the frequency comb spectrum is tuned to ensure that two…

Atomic Physics · Physics 2020-09-02 D. Buhin , D. Kovacic , F. Schmid , M. Kruljac , V. Vulic , T. Ban , D. Aumiler

Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…

Optical two-dimensional coherent spectroscopy (2DCS) has become a powerful tool for studying energy level structure, dynamics, and coupling in many systems including atomic ensembles. Various types of two-dimensional (2D) spectra, including…

Atomic Physics · Physics 2022-05-25 Jieli Yan , Stephen Revesz , Danfu Liang , Hebin Li

Laser spectroscopy and interferometry have provided an unparalleled view into the fundamental nature of matter and the universe through ultra-precise measurements of atomic transition frequencies and gravitational waves. Optical frequency…

We present a new type of dual optical frequency comb source capable of scaling applications to high measurement speeds while combining high average power, ultra-low noise operation, and a compact setup. Our approach is based on a…

We explore the advantages of a free-form dual-comb spectroscopy (DCS) platform based on time-programmable frequency combs for real-time, penalty-free apodized scanning. In traditional DCS, the fundamental spectral resolution, which equals…