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We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

We present and theoretically demonstrate a method for generating helicity-selected near-circularly polarized attosecond pulses in mixed He-Ne gases using bichromatic counter-rotating circularly polarized (BCCP) fields. High-order harmonics…

Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…

It is shown that when relativistically intense ultrashort laser pulses are reflected from the boundary of a plasma with a near-critical density, Doppler frequency shift leads to generation of intense radiation both in the high-frequency, up…

Plasma Physics · Physics 2023-02-03 Nikita A. Mikheytsev , Artem V. Korzhimanov

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer

We demonstrate extremely narrow resonances for polarization rotation in an atomic vapor. The resonances are created using a strong control laser on the same transition, which polarizes the atoms due to optical pumping among the magnetic…

Atomic Physics · Physics 2015-02-25 Sapam Ranjita Chanu , Kanhaiya Pandey , Vineet Bharti , Ajay Wasan , Vasant Natarajan

Photoelectron angular distributions (PADs) of oriented polar molecules in response to different polarized lasers are systematically investigated. It is found that the PADs of polar CO molecules show three distinct styles excited by…

Chemical Physics · Physics 2013-03-05 Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu , Zhizhan Xu

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

Quantum Physics · Physics 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh

In conditions where the interaction betweeen an atom and a short high-frequency extreme ultraviolet laser pulse is a perturbation, we show that a simple theoretical approach, based on Coulomb-Volkov-type states, can make reliable…

Atomic Physics · Physics 2009-11-07 Guillaume Duchateau , Eric Cormier , Robert Gayet

While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…

Atomic Physics · Physics 2013-02-27 Felipe Herrera , Sabre Kais , K. Birgitta Whaley

A method for the generation of ultrarelativistic electron beams with high spin polarization is put forward, where a tightly-focused linearly-polarized ultraintense laser pulse interacts with a nonprepolarized transverse-size-tailored solid…

Plasma Physics · Physics 2024-06-11 Xiaofei Shen , Zheng Gong , Karen Z. Hatsagortsyan , Christoph H. Keitel

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the…

Atomic and Molecular Clusters · Physics 2013-07-02 Paul Venn , Hendrik Ulbricht

Several laser techniques have been suggested and demonstrated recently for preparing polarizable molecules in rapidly spinning states with a disc-like angular distribution. We consider motion of these spinning discs in inhomogeneous fields,…

Chemical Physics · Physics 2015-05-20 Johannes Floss , Erez Gershnabel , Ilya Sh. Averbukh

When a high-power, femtosecond, circularly polarized (CP) laser pulse is incident on a micrometer-scale aperture in a solid foil target, it drives surface plasma oscillation, generating high-order harmonic vortices in the diffracted light.…

Plasma Physics · Physics 2025-10-28 Runze Li , Wenchao Yan , Longqing Yi

Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…

Atomic Physics · Physics 2015-05-28 Elmar V. van der Zwan , Manfred Lein

We present experimental evidence of a fourth order process in electric field in supercontinuum generation. We also show laser induced polarization preference in the supercontinuum generating media. These results have become possible through…

Quantum Physics · Physics 2007-05-23 Alok Srivastava , Debabrata Goswami