Related papers: Polarization shaping of high-order harmonics in la…
We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary…
We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…
We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…
Many studies have shown that high-energy $\gamma$-photon beams can be efficiently generated via nonlinear Compton scattering driven by laser pulses with intensities $> 10^{22}\rm{W/cm^2}$ recently available in laboratories. Here, we propose…
We demonstrate to image asymmetric molecular orbitals via high-order harmonic generation in a one-color inhomogeneous field. Due to the broken inversion symmetry of the inhomogeneous field in space, the returning electrons with energy in a…
Extreme-ultraviolet (XUV) light is notoriously difficult to control due to its strong interaction cross-section with media. We demonstrate a method to overcome this problem by using Opto-Optical Modulation guided by a geometrical model to…
We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…
XFELs provide X-ray pulses with unprecedented peak brightness and ultrashort duration. They are usually driven by planar undulators, meaning that the output radiation is linearly polarized. For many experimental applications, however,…
Photon pairs, highly entangled in polarization have been generated under femtosecond laser pulse excitation by a type I crystal source, operating in a single arm interferometric scheme. The relevant effects of temporal walk-off existing in…
We propose a feasible scenario to directly polarize a relativistic electron beam and obtain overall polarization in various directions through a filter mechanism for single-shot collision between an ultrarelativistic unpolarized electron…
Laser control of molecular rotation is an area of active research. A number of recent studies has aimed at expanding the reach of rotational control to extreme, previously inaccessible rotational states, as well as controlling the…
We show that a laser pulse designed as an adiabatic ramp followed by a kick allows one to reach a perfect postpulse molecular alignment, free of saturation. The mechanism is based on an optimized distribution of the energy between a weakly…
Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…
We demonstrate a novel technique for producing high-order harmonics with designer spectral combs in the extreme ultraviolet-soft X-ray range for resonance applications using spectrally controlled visible lasers. Our approach enables…
We show that dressing polar molecules with a far-off-resonant optical field leads to new types of intermolecular potentials, which undergo a crossover from the inverse-power to oscillating behavior depending on the intermolecular distance,…
Control of the angular momentum of light is a key technology for next-generation nano-optical devices and optical communications, including quantum communication and encoding. We propose an approach to controllably generate circularly…
A scheme for quasi-phase-matching high-harmonic generation is proposed in which polarization beating within a hollow core birefringent waveguide modulates the generation of harmonics. The evolution of the polarization of a laser pulse…
We propose utilizing a polarization-tailored high-power laser pulse to extract and accelerate electrons from the edge of a solid foil target to produce isolated attosecond electron bunches. The laser pulse consists of two…
An interesting property of high harmonic generation in solids is its laser polarization dependent nature which in turn provides information about the crystal and band structure of the generation medium. Here we report on the linear…
Ultrashort laser pulses are widely used for transient field-free molecular orientation -- a phenomenon important in chemical reaction dynamics, ultrafast molecular imaging, high harmonics generation, and attosecond science. However,…