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We propose utilizing a polarization-tailored high-power laser pulse to extract and accelerate electrons from the edge of a solid foil target to produce isolated attosecond electron bunches. The laser pulse consists of two…

Plasma Physics · Physics 2024-03-18 Ke Hu , Longqing Yi

The ability to manipulate ferroelectrics at ultrafast speeds has long been an elusive target for materials research. Coherently exciting the ferroelectric mode with ultrashort optical pulses holds the promise to switch the ferroelectric…

Materials Science · Physics 2017-05-17 Roman Mankowsky , Alexander von Hoegen , Michael Först , Andrea Cavalleri

X-ray free-electron lasers (XFELs) as the world's brightest light sources provide ultrashort X-ray pulses with a duration typically in the order of femtoseconds. Recently, they have approached and entered the attosecond regime, which holds…

There has been an explosion of interest in time-varying photonics due to the recent discovery and design of materials and metamaterials with strong, time-varying, nonlinear optical responses. This opens the door to novel optical phenomena…

Optics · Physics 2023-07-05 Joshua Baxter , Lora Ramunno

Owning to their high controllability, laser pulses have contributed greatly to our understanding of strongly correlated electron systems. However, typical multicycle pulses do not control the symmetry of systems that plays an important role…

Strongly Correlated Electrons · Physics 2023-05-05 Kazuya Shinjo , Shigetoshi Sota , Seiji Yunoki , Takami Tohyama

We calculate the ferroelectric polarization dynamics induced by a femtosecond midinfrared pulse as measured in the recent experiment by R. Mankowsky et al., Phys. Rev. Lett. 118, 197601 (2017). It is due to the nonlinear coupling of the…

Materials Science · Physics 2020-01-15 Veniamin A. Abalmasov

Electronic wave functions of planar molecules can be reconstructed via inverse Fourier transform of angle-resolved photoelectron spectroscopy (ARPES) data, provided the phase of the electron wave in the detector plane is known. Since the…

Other Condensed Matter · Physics 2016-09-23 Pavel Kliuiev , Tatiana Latychevskaia , Juerg Osterwalder , Matthias Hengsberger , Luca Castiglioni

The phasing problem of heterodyne-detected nonlinear spectroscopy states that the relative time delay between the exciting pulses and a local oscillator must be known with subcycle precision to separate absorptive and dispersive…

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

We propose a theoretical and computational approach to investigate temporal behavior of a nonlinear polarization in perturbative regime induced by an intense and ultrashort pulsed electric field. First-principles time-dependent density…

Optics · Physics 2019-03-27 Mitsuharu Uemoto , Yuki Kuwabara , Shunsuke A. Sato , Kazuhiro Yabana

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

Atomic and Molecular Clusters · Physics 2015-05-20 C. -H. Zhang , U. Thumm

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…

Atomic Physics · Physics 2015-10-28 Lukas Medišauskas , Jack Wragg , Hugo van der Haart , Misha Yu. Ivanov

We propose a novel spectral method for reconstructing quantum wavefunction of an electron pulse, free-electron spectral shearing interferometry (FESSI). We employ a Wien filter to generate two time-delayed replicas of the electron…

Quantum Physics · Physics 2025-08-18 Zhaopin Chen , Bin Zhang , Yiming Pan , Michael Krueger

We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…

In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time)…

Atomic Physics · Physics 2019-09-04 Jan Troß , Georgios Kolliopoulos , Carlos A. Trallero-Herrero

A new method to generate short wavelength Free Electron Laser output with modulated polarisation at attosecond timescales is presented. Simulations demonstrate polarisation switching timescales that are four orders of magnitude faster than…

Accelerator Physics · Physics 2021-01-20 J. Morgan , B. W. J. McNeil

Electro-optic time lenses are promising experimental components for photonic spectral-temporal processing of quantum information. We report a stable method to realize an electro-optic time lens, which relies on the amplification of an…

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…