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We present an interferometric pump-probe technique for the characterization of attosecond electron wave packets (WPs) that uses a free WP as a reference to measure a bound WP. We demonstrate our method by exciting helium atoms using an…

The present work focuses on the characterisation of the amount of orbital angular momentum (OAM) encoded in the twisted attosecond pulses via energy- and angle-resolved attosecond streaking in pump-probe setup. It is found that the…

Atomic Physics · Physics 2020-06-03 Irfana N. Ansari , Deependra S. Jadoun , Gopal Dixit

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…

Mesoscale and Nanoscale Physics · Physics 2025-04-25 Xin Jin , Cruz I. Velasco , F. Javier García de Abajo

Ultra-short laser pulses with femtosecond to attosecond pulse duration are the shortest systematic events humans can create. Characterization (amplitude and phase) of these pulses is a key ingredient in ultrafast science, e.g., exploring…

Optics · Physics 2018-03-19 Tom Zahavy , Alex Dikopoltsev , Oren Cohen , Shie Mannor , Mordechai Segev

Attosecond x-ray pulses offer unprecedented opportunities for probing and triggering new types of ultrafast motion. At the same time, pulse characterization of x-rays presents new challenges that do not exist in the UV regime. Inner-shell…

Atomic Physics · Physics 2017-05-24 Stefan Pabst , Jan Marcus Dahlström

Accurate and fast characterization of spatiotemporal information of high-intensity, ultrashort pulses is crucial in the field of strong-field laser science and technology. While conventional self-referenced interferometers were widely used…

Optics · Physics 2023-07-19 Yifei Chen , Zhiyuan Huang , Ding Wang , Yu Zhao , Jianhua Fu , Meng Pang , Yuxin Leng , Zhizhan Xu

We experimentally demonstrate temporal reshaping of optical waveforms in the telecom wavelength band using the principle of quantum frequency conversion. The reshaped optical pulses do not undergo any wavelength translation. The interaction…

Quantum Physics · Physics 2017-02-28 Paritosh Manurkar , Nitin Jain , Prem Kumar , Gregory S. Kanter

By means of a metal opto-acoustic transducer we generate quasi-longitudinal and quasi-transverse picosecond strain pulses in a (311)-GaAs substrate and monitor their propagation by picosecond acoustic interferometry. By probing at the…

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

Fascinating developments in optical pulse engineering over the last 20 years lead to the generation of laser pulses as short as few femtosecond, providing a unique tool for high resolution time domain spectroscopy. However, a number of the…

General Physics · Physics 2008-06-03 M Kozlowski , J Marciak-Kozlowska , M Pelc

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Ultrafast electron microscopy provides a movie-like access to structural dynamics of materials in space and time, but fundamental atomic motions or electron dynamics are, so far, too quick to be resolved. Here we report the all-optical…

Optics · Physics 2024-02-27 J. Kuttruff , D. Nabben , A. C. Zimmermann , A. Ryabov , P. Baum

We find a solution of the wave equation in the paraxial approximation that describes the attosecond pulses with spatiotemporal helical structure in the phase and in the intensity recently generated by means of highly nonlinear optical…

Optics · Physics 2019-09-25 Miguel A. Porras

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

Characterizing quantum states of the electromagnetic field at microwave frequencies requires fast and sensitive detectors that can simultaneously probe the field time-dependent amplitude and its quantum fluctuations. In this work, we…

Amplitude and phase of wavepackets encode the dynamics of quantum systems. However, the rapidity of electron dynamics on the attosecond timescale has precluded their complete measurement in the time domain. Here, we demonstrate that…

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental…

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