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We demonstrate the complete reconstruction of the electric field of visible-infrared pulses with energy as low as a few tens of nanojoules. The technique allows for the reconstruction of the instantaneous electric field vector direction and…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

We propose the scheme of temporal double-slit interferometer to precisely measure the electric field of shaped intense femtosecond laser pulse directly, and apply it to control the electron tunneling wave packets in attosecond precision. By…

Atomic Physics · Physics 2023-11-13 Xiaoyun Zhao , Mingqing Liu , Yizhang Yang , Zhou Chen , Xiaolei Hao , Chuncheng Wang , Weidong Li , Jing Chen

Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

The waveforms of attosecond pulses produced by high-harmonic generation carry information on the electronic structure and dynamics in atomic and molecular systems. Current methods for the temporal characterization of such pulses have…

Light-phase-sensitive techniques, such as coherent multidimensional spectroscopy, are well-established in a broad spectral range, already spanning from radio-frequencies in nuclear magnetic resonance spectroscopy to visible and ultraviolet…

Comprehending the unique characteristics of structured ultrafast optical pulses is essential to the physics, applications and instrumentations of ultrafast lasers. However, full-vectrorial characterizations of the pulses remain challenging…

Optics · Physics 2020-02-03 Tiancheng Huo , Li Qi , Janson J. Chen , Yusi Miao , Zhongping Chen

Despite the multitude of available methods, the characterisation of ultrafast pulses remains a challenging endeavour, especially at the single-photon level. We introduce a pulse characterisation scheme that maps the magnitude of its…

We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.

Optics · Physics 2016-08-16 Antoine Monmayrant , Béatrice Chatel , Bertrand Girard

We demonstrate an all-optical approach for precise characterization of attosecond extreme ultraviolet pulses. Isolated attosecond pulse is produced from high order harmonics using intense driving pulse with proper gating technique. When a…

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…

Optics · Physics 2018-03-21 Yuya Morimoto , Peter Baum

We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…

Optics · Physics 2016-07-19 Stefan Pabst , Jan Marcus Dahlström

Recently discovered reactive optical forces have nule time-average of their instantaneous values on monochromatic illumination, so that their detection suggests the use of ultrafast optics, specially in the femto and attosecond domains. By…

The use of structured ultrashort pulses with coupled spatiotemporal properties is emerging as a key tool for ultrafast manipulation. Ultrafast vector beams are opening exciting opportunities in different fields such as microscopy,…

We present a setup for complete characterization of femtosecond pulses generated by seeded free-electron lasers (FEL's) in the extreme-ultraviolet spectral region. Two delayed and spectrally shifted replicas are produced and used for…

The attosecond streaking technique is normally utilized to characterize the attosecond pulses in extreme ultraviolet spectrum, while the pulse simulation and reconstruction schemes turn out to be unreliable for extremely short sub-100as…

Optics · Physics 2018-09-05 Renzhi Shao , Bin Li

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

We demonstrate a new attosecond pulse reconstruction modality which uses an algorithm that is derived from ptychography. In contrast to other methods, energy and delay sampling are not correlated, and as a result, the number of electron…

Optics · Physics 2015-11-17 M. Lucchini , M. H. Brügmann , A. Ludwig , L. Gallmann , U. Keller , T. Feurer

Interferometry, as the key technique in modern precision measurements, has been used for length diagnosis in the fields of engineering metrology and astronomy. Analogous interferometric technique for time domain precision measurement is a…

Optics · Physics 2019-11-15 Zhen Yang , Wei Cao , Yunlong Mo , Huiyao Xu , Kang Mi , Pengfei Lan , Qingbin Zhang , Peixiang Lu

Ultrashort light pulses are ubiquitous in modern research, but the electromagnetic field of the optical cycles is usually not easy to obtain as a function of time. Field-resolved pulse characterization requires either a nonlinear-optical…

Optics · Physics 2022-11-30 Yuya Morimoto , Bo-Han Chen , Peter Baum
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