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Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and…

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

Realistic attosecond wave packets have complex profiles that, in dispersive conditions, rapidly broaden or split into multiple components. Such behaviors are encoded in sharp features of the wave packet spectral phase. Here, we exploit the…

A new method for efficiently generating an isolated single-cycle attosecond pulse is proposed. It is shown that the ultraviolet (UV) attosecond pulse can be utilized as a robust tool to control the dynamics of electron wave packets (EWPs).…

Atomic Physics · Physics 2009-11-13 Pengfei Lan , Peixiang Lu , Wei Cao , Xinlin Wang

We propose a novel method to reconstruct the spatio-temporal amplitude and phase of the electric field of ultrashort laser pulses using spatially-resolved spectral interferometry. This method is based on a fiber-optic coupler interferometer…

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate…

Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…

Atomic Physics · Physics 2020-01-08 D. Hammerland , P. Zhang , S. Kuehn , P. Jojart , I. Seres , V. Zuba , Z. Varallyay , K. Osvay , T. T. Luu , H. J. Woerner

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

Ultrafast processes in matter can be captured and even controlled by using sequences of few-cycle optical pulses, which need to be well characterized, both in amplitude and phase. The same degree of control has not yet been achieved for…

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…

Optics · Physics 2019-05-15 Martin Kozák , Norbert Schönenberger , Peter Hommelhoff

We study the influence of polarization effects in streaking by combined atto- and femtosecond pulses. The polarization-induced terms alter the streaking spectrum. The normal streaking spectrum, which maps to the vector potential of the…

Atomic Physics · Physics 2015-05-14 Jan Conrad Baggesen , Lars Bojer Madsen

The power spectrum of an optical field can be acquired without a spectrally resolving detector by means of Fourier-transform spectrometry, based on measuring the temporal autocorrelation of the optical field. Analogously, we here perform…

The interaction of high-intensity laser pulses and solid targets provides a promising way to create compact, tunable and bright XUV attosecond sources that can become a unique tool for a variety of applications. However, it is important to…

Plasma Physics · Physics 2018-10-17 M. Blanco , M. T. Flores-Arias , A. Gonoskov

The generation of ultrafast laser pulses and the reconstruction of their electric fields is essential for many applications in modern optics. Quantum optical fields can also be generated on ultrafast time scales, however, the tools and…

Quantum Physics · Physics 2019-10-02 Jean-Philippe W. MacLean , Sacha Schwarz , Kevin J. Resch

Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…

In this paper, we propose a new method to characterize the temporal structure of arbitrary optical laser pulses with low pulse energies. This approach is based on strong field photoelectron holography with the glory rescattering effect as…

Atomic Physics · Physics 2020-04-29 J. F. Tao , J. Cai , Q. Z. Xia , J. Liu

In this article we present a closed analytical description for few-cycle, focused electromagnetic pulses of arbitrary duration and carrier-envelope-phase (CEP). Because of the vectorial character of light, not all thinkable one-dimensional…

Classical Physics · Physics 2011-08-10 Daniel an der Brügge , Alexander Pukhov

Probing the evolution of physical systems at the femto- or attosecond timescale with light requires accurate characterization of ultrashort optical pulses. The time profiles of such pulses are usually retrieved by methods utilizing optical…

Optics · Physics 2011-07-26 Osip Schwartz , Oren Raz , Ori Katz , Nirit Dudovich , Dan Oron