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Using resonant two-step laser excitation of trapped 232Th+ ions, we observe 43 previously unknown energy levels within the energy range from 7.3 to 8.3 eV. The high density of states promises a strongly enhanced electronic bridge excitation…

Atomic Physics · Physics 2013-08-01 O. A. Herrera-Sancho , N. Nemitz , M. V. Okhapkin , E. Peik

The excitation of the 8 eV $^{229m}$Th isomer through the electronic bridge mechanism in highly charged ions is investigated theoretically. By exploiting the rich level scheme of open $4f$ orbitals and the robustness of highly charged ions…

We consider the excitation of the nuclear transition ^{229g}Th - ^{229m}Th near 7.6 eV in singly ionized thorium via an electronic bridge process. The process relies on the excitation of the electron shell by two laser photons whose sum…

Atomic Physics · Physics 2010-10-27 S. G. Porsev , V. V. Flambaum , E. Peik , Chr. Tamm

An alternative method to determine the excitation energy of the $~^{229\rm{m}}\rm{Th}$ isomer via the laser-induced electronic bridge is investigated theoretically. In the presence of an optical or ultra-violet laser at energies that…

Atomic Physics · Physics 2018-03-13 Pavlo V. Bilous , Ekkehard Peik , Adriana Pálffy

The 8.4 eV transition in the $^{229}$Th nucleus is the basis for a high-precision nuclear clock with exceptional sensitivity to new physics effects. We have identified several cases in the Th$^+$ ion where electronic excitations closely…

Atomic Physics · Physics 2025-04-29 V. A. Dzuba , V. V. Flambaum

Excitation of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+, 8.28 \pm 0.17$ eV) in the process of inelastic electron scattering is studied theoretically in the framework of the perturbation theory for the quantum…

Nuclear Theory · Physics 2020-07-01 E. V. Tkalya

Theoretical considerations are made for the nuclear excitation from the ground state to the 8 eV $^{229m}$Th isomer via near-resonant electron transitions in Sb-like ($q=39+$) thorium ions. The energy of the first excited atomic state…

Atomic Physics · Physics 2025-04-17 Karol Kozioł , Jacek Rzadkiewicz

Thorium-229 possesses the lowest nuclear first excited state with an energy of about 8 eV. The extremely narrow linewidth of the nuclear first excited state with the uncertainty of 53 THz prevents the direct laser excitation and the…

Atomic Physics · Physics 2024-05-14 Lin Li , Zi Li , Chen Wang , Wen-Ting Gan , Xia Hua , Xin Tong

High-spin spectroscopic study of $^{202}$Po ($Z$ = 84, $N$ = 118) has been carried out using the $^{195}$Pt($^{12}$C, 5n)$^{202}$Po fusion-evaporation reaction. An extended level scheme has been proposed up to an excitation energy of…

Electronic bridge excitation of the 76 eV nuclear isomeric state in $^{235}$U is shown to be strongly enhanced in the U$^{7+}$ ion, potentially enabling laser excitation of this nucleus. This is because the electronic spectrum has a very…

Atomic Physics · Physics 2019-01-08 J. C. Berengut

$^{229}$Th with a low-lying nuclear isomeric state is an essential candidate for a nuclear clock as well as many other applications. Laser excitation of the isomeric state has been a long-standing goal. With relativistic $^{229}$Th ions in…

The low-lying isomeric state of $^{229}$Th provides unique opportunities for high-resolution laser spectroscopy of the atomic nucleus. We determine the energy of this isomeric state by taking the absolute energy difference between the…

We have studied the effect of atomic electrons on the nuclear transition from the isomeric {229m}Th state to the ground {229g}Th state in {229}Th+ due to the electronic bridge process. The exact value of the nuclear transition frequency is…

Atomic Physics · Physics 2014-11-20 S. G. Porsev , V. V. Flambaum

The electronic defect states resulting from doping $^{229}$Th in CaF$_2$ offer a unique opportunity to excite the nuclear isomeric state $^{229m}$Th at approximately 8 eV via electronic bridge mechanisms. We consider bridge schemes…

Excitation of the isomeric nuclear state 229m Th in the process of thorium atom irradiation by two-color femtosecond pulse of Ti: Sa laser at the fundamental wavelength and second harmonic is analyzed. It is shown that the rate of isomeric…

Optics · Physics 2019-01-23 A. V. Andreev , A. B. Savelyev , S. Yu. Stremoukhov , O. A. Shoutova

$^{229}$Th is the only known nucleus with an excited state that offers the possibility for a direct laser excitation using existing laser technology. Its excitation energy has been measured indirectly to be 7.8(5) eV ($\approx$160 nm). The…

Instrumentation and Detectors · Physics 2018-12-14 Benedict Seiferle , Lars von der Wense , Ines Amersdorffer , Nicolas Arlt , Benjamin Kotulski , Peter G. Thirolf

When Th nuclei are doped in CaF$_2$ crystals, a set of electronic defect states appears in the crystal bandgap which would otherwise provide complete transparency to vacuum-ultraviolet radiation. The coupling of these defect states to the 8…

Using the polarisation labelling spectroscopy, we performed the detailed analysis of the level structure of excited electronic states of the $^{39}$KCs molecule in the excitation energy interval between 17500~cm$^{-1}$ and 18600~cm$^{-1}$…

We identify a potential means to extract the $^{229g}$Th $\rightarrow$ $^{229m}$Th nuclear excitation energy from precision microwave spectroscopy of the $5F_{5/2,7/2}$ hyperfine manifolds in the ion $^{229g}$Th$^{3+}$. The hyperfine…

Atomic Physics · Physics 2014-02-14 K. Beloy

We present a comprehensive theoretical investigation of hyperfine-resolved excitation and detection of the low-energy isomeric state of $^{229}$Th in trapped $^{229}\mathrm{Th}^{3+}$ ions. Using a quantum master equation approach, we…

Atomic Physics · Physics 2026-05-01 Wu Wang , Ke Zhang , Ke-Mi Xu , Shan-Gui Zhou
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