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The coupling between lattice vibration quanta and valence electrons can induce charge density modulations and decisively influence the transport properties of materials, e.g. leading to conventional superconductivity. In high critical…

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order,…

Strongly Correlated Electrons · Physics 2017-07-03 T. P. Devereaux , A. M. Shvaika , K. Wu , K. Wohlfeld , C. J. Jia , Y. Wang , B. Moritz , L. Chaix , W. -S. Lee , Z. -X. Shen , G. Ghiringhelli , L. Braicovich

The experimental determination of the magnitude and momentum dependence of electron-phonon coupling (EPC) is an outstanding problem in condensed matter physics. The intensity of phonon peaks in Resonant Inelastic X-ray Scattering (RIXS)…

We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Michel van Veenendaal , Jeroen van den Brink

We report an ultrahigh resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. Phonon softening and lifetime shortening are…

Interactions between electrons and lattice vibrations are responsible for a wide range of material properties and applications. Recently, there has been considerable interest in the development of resonant inelastic x-ray scattering (RIXS)…

Resonant inelastic X-ray scattering (RIXS) is used increasingly for characterizing low-energy collective excitations in materials. RIXS is a powerful probe, which often requires sophisticated theoretical descriptions to interpret the data.…

Strongly Correlated Electrons · Physics 2021-09-22 Krzysztof Bieniasz , Steven Johnston , Mona Berciu

Phonons, the quantum mechanical representation of lattice vibrations, and their coupling to the electronic degrees of freedom are important for understanding thermal and electric properties of materials. For the first time, phonons have…

Strongly Correlated Electrons · Physics 2011-01-25 H. Yavas , M. van Veenendaal , J. van den Brink , L. J. P. Ament , A. Alatas , B. M. Leu , M. -O. Apostu , N. Wizent , G. Behr , W. Sturhahn , H. Sinn , E. E. Alp

How electron-phonon interactions influence high-temperature superconductivity in cuprates remains contested, and their role outside the CuO$_2$ planes has been largely overlooked. The most conspicuous evidence for such coupling is the…

Inelastic x-ray scattering with meV energy resolution (IXS) is an ideal tool to measure collective excitations in solids and liquids. In non-resonant scattering condition, the cross section is strongly dominated by lattice vibrations…

Recent improvements in the energy resolution of resonant inelastic x-ray scattering experiments (RIXS) at the Cu-L$_3$ edge have enabled the study of lattice, spin, and charge excitations. Here, we report on the detection of a low intensity…

The community currently lacks a complete understanding of how resonant inelastic x-ray scattering (RIXS) experiments probe the electron-phonon ($e$-ph) interaction in solids. For example, most theoretical models of this process have focused…

Strongly Correlated Electrons · Physics 2022-05-25 Krzysztof Bieniasz , Steve Johnston , Mona Berciu

The exciton-phonon coupling in highly oriented pyrolytic graphite is studied using resonant inelastic X-ray scattering (RIXS) spectroscopy. With ~ 70 meV energy resolution, multiple low energy excitations associated with coupling to phonons…

A description of electron-phonon coupling at a defect or impurity is essential to characterizing and harnessing its functionality for a particular application. Electron-phonon coupling limits the amount of useful light produced by a…

Materials Science · Physics 2026-04-21 Mark E. Turiansky , John L. Lyons

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Materials Science · Physics 2015-06-23 Robert P. Chatelain , Vance R. Morrison , Bart L. M. Klarenaar , Bradley J. Siwick

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

Strongly Correlated Electrons · Physics 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

We report high-resolution inelastic x-ray scattering measurements of the acoustic phonons in the single-layer cuprate $Bi_{2}Sr_{2-x)La_{x}CuO_{6+\delta}$. These measurements reveal anomalous broadening of the longitudinal acoustic phonon…

Time resolved measurements provide a new way to disentangle complex interactions in quantum materials due to their different timescales. We used pump-probe Raman scattering to investigate the apical oxygen vibration in…

Superconductivity · Physics 2021-12-07 N. Pellatz , S. Roy , J-W. Lee , J. L. Schad , H. Kandel , N. Arndt , C. B. Eom , A. F. Kemper , D. Reznik

We have developed a first-principles method to calculate the electron-phonon coupling for specific modes and q-points in the Brillouin Zone for crystalline organic semiconductors. Using the obtained coupling strengths, we propose an…

Despite the intensive efforts for determining the mechanism that causes high-temperature superconductivity in copper oxide materials, no consensus on the pairing mechanism has been reached. Recent advances in high resolution angle-resolved…

Superconductivity · Physics 2011-02-18 H. S. Ruiz , A. Badía-Majós
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