Related papers: An $^{27}$Al$^{+}$ quantum-logic clock with system…
For the past 15 years, tremendous progress within the fields of laser stabilization, optical frequency combs and atom cooling and trapping have allowed the realization of optical atomic clocks with unrivaled performances. These instruments…
We report a comprehensive evaluation of all known sources of systematic uncertainty for two independent $^{176}$Lu$^+$ single-ion optical references, finding total systematic uncertainty of $1.1\times10^{-19}$ and $1.4\times10^{-19}$ for…
We demonstrate how to realize an optical clock with neutral atoms that is competitive to the currently best single ion optical clocks in accuracy and superior in stability. Using ultracold atoms in a Ca optical frequency standard we show…
We report on a $^{88}$Sr$^{+}$ single-ion optical clock with an estimated fractional systematic uncertainty of $7.9\times 10^{-19}$. The low uncertainty is enabled by small rf losses, a thorough evaluation of the blackbody-radiation…
We report a systematic uncertainty of $9.2\times 10^{-19}$ for the USTC Sr1 optical lattice clock, achieving accuracy at the level required for the roadmap of the redefinition of the SI second. A finite-element model with {\it in…
The rapid increase in accuracy and stability of optical atomic clocks compared to the caesium atomic clock as primary standard of time and frequency asks for a future re-definition of the second in the International System of Units (SI).…
We identify two metastable excited states in Sm$ ^{10+} $ highly charged ion as candidates for high accuracy optical clocks. Several atomic properties relevant to optical clock development are calculated using relativistic many-body…
The passage of time is tracked by counting oscillations of a frequency reference, such as Earth's revolutions or swings of a pendulum. By referencing atomic transitions, frequency (and thus time) can be measured more precisely than any…
State-of-the-art atomic clocks are based on the precise detection of the energy difference between two atomic levels, measured as a quantum phase accumulated in a given time interval. Optical-lattice clocks (OLCs) now operate at or near the…
We evaluate the electric quadrupole moments of the ${^1}\!S_0$ and ${^3}\!P_0$ clock states of $^{27}$Al$^+$ and $^{115}$In$^+$. To capture all dominant contributions, our analysis extends through third order of perturbation theory and…
Optical atomic clocks have demonstrated revolutionary advances in precision timekeeping, but their applicability to the real world is critically dependent on whether such clocks can operate outside a laboratory setting. The challenge to…
We present an assessment of the (6s^{2})1S0 -> (6s7s)3P0 clock transition frequency in 199Hg with an uncertainty reduction of nearly three orders of magnitude and demonstrate an atomic quality factor, Q, of ~10^(14). The 199Hg atoms are…
The differential polarizability, due to near-infrared light at 1126 nm, of the 27Al+ 1S0 -> 3P0 clock transition is measured to be 4\pi\epsilon_0 x (1.6 +/- 0.5) x 10^{-31} m^3. This measurement is combined with experimental oscillator…
Our study is motivated by the prospect of several metastable states in the Sb$ ^{+} $, Au$ ^{+} $, and Hg$ ^{2+} $ ions being used as possible candidates for optical clocks. We calculate several atomic properties relevant to the development…
We propose a high-performance atomic clock based on the 1.81 PHz transition between the ground and first-excited state of doubly ionized lead. Utilizing an even isotope of lead, both clock states have $I=J=F=0$, where $I$, $J$, and $F$ are…
Optical atomic clocks are the most accurate measurement devices ever constructed and have found many applications in fundamental science and technology. The use of highly charged ions (HCI) as a new class of references for highest accuracy…
Transition frequencies of atoms and ions are among the most accurately accessible quantities in nature, playing important roles in pushing the frontiers of science by testing fundamental laws of physics, in addition to a wide range of…
Multi-ion optical clocks offer the possibility of overcoming the low signal-to-noise ratio of single-ion clocks, while still providing low systematic uncertainties. We present simultaneous spectroscopy of up to four ${}^{115}$In${}^+$ clock…
Optical frequency comparison of the 40Ca+ clock transition \nu_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition \nu_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio \nu_{Ca} / \nu_{Sr} = 0.957 631 202 358…
We propose a many-ion optical atomic clock based on three-dimensional Coulomb crystals of order one thousand Sn$^{2+}$ ions confined in a linear RF Paul trap. Sn$^{2+}$ has a unique combination of features that is not available in…