Related papers: Synthesis of ultrafast waveforms using coherent Ra…
We report the synthesis of arbitrary optical waveforms by manipulating the spectral phases of Raman sidebands with a wide frequency spacing line-by-line. Trains of rectangular and triangular pulses are stably produced at an ultrahigh…
We report line-by-line control of a coherent discrete spectrum (Raman sidebands) with a frequency spacing of 10.6 THz that is produced by an adiabatic Raman process. We show that the spectral phase of the Raman sidebands is finely…
We demonstrate the efficient generation of Raman sidebands in a medium coherently prepared in a dark state by continuous-wave low-intensity laser radiation. Our experiment is performed in sodium vapor excited in $\Lambda $ configuration on…
Low-phase-noise and pure-spectrum Raman light is vital for high-precision atom interferometry by two-photon Raman transition. A preferred and prevalent solution for Raman light generation is electro-optic phase modulation. However, phase…
Ultra-fast laser pulses have made possible the study of extreme nonlinear processes. Many of these experiments however require a full characterization of the electric field, which typically requires a separate parametric optical process. As…
Spatio-temporal mode coupling in highly multimode physical systems permits new routes for exploring complex instabilities and forming coherent wave structures. We present here the first experimental demonstration of multiple geometric…
A train of periodic optical pulses gives an optical frequency "comb" that acts as a precise ruler for light measurement due to its equally spaced frequencies. Today, such pulses last millionths of a billionth of a second (Femtoseconds/fs)…
A stable 50 mJ three-channel optical waveform synthesizer is demonstrated and used to reproducibly generate a high-order harmonics supercontinuum in the soft-x-ray region. This synthesizer is composed of pump pulses from a…
A promising route towards the heralded creation and annihilation of single-phonons is to couple a single-photon emitter to a mechanical resonator. The challenge lies in reaching the resolved-sideband regime with a large coupling rate and a…
We present experiments in which self-assembled InAs quantum dots are coupled to a thin, suspended-beam GaAs resonator. The quantum dots are driven resonantly and the resonance fluorescence is detected. The narrow quantum-dot linewidths,…
Exploration of optical non-linear response of graphene predominantly relies on ultra-short time domain measurements. Here we propose an alternate technique that uses frequency modulated continuous wavefront optical fields, thereby probing…
The recent introduction of coherent optical communications has created a compelling need for ultra-fast phase-sensitive measurement techniques operating at milliwatt peak power levels and in time scales ranging from sub-picoseconds to…
We simulate multi-shot intensity-and-phase measurements of unstable ultrashort-pulse trains using frequency-resolved-optical-gating (FROG) and spectral phase interferometry for direct electric-field reconstruction (SPIDER). Both techniques…
We propose and experimentally demonstrate a scheme to generate optically-controlled delays based on off-resonant Raman absorption. Dispersion in a transparency window between two neighboring, optically-activated Raman absorption lines is…
We have developed a novel multiscale computational scheme to describe coupled dynamics of light electromagnetic field with electrons and atoms in crystalline solids, where first-principles molecular dynamics based on time-dependent density…
We present the results of an experimental and numerical investigation into temporally non-local coherent interactions between ultrashort pulses, mediated by Raman coherence, in gas-filled kagom\'{e}-style hollow-core photonic crystal fiber.…
The emission spectra of many pi-conjugated polymers and oligomers contain side-band replicas with apparent frequencies that do not match the Raman active mode frequencies. Using a time dependent model we show that in such many mode systems,…
We numerically explore synthetic crystal diamond for realizing novel light sources in ranges which are up to now difficult to achieve with other materials, such as sub-10-fs pulse durations and challenging spectral ranges. We assess the…
Generating energetic femtosecond mid-IR pulses is crucial for ultrafast spectroscopy, and currently relies on parametric processes that, while efficient, are also complex. Here we experimentally show a simple alternative that uses a single…
Optical dual-pulse pumping actively creates quantum-mechanical superposition of the electronic and phononic states in a bulk solid. We here made transient reflectivity measurements in an n-GaAs using a pair of relative-phase-locked…