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We study an excited atom-polar molecular ion chemical reaction (Ca$^*$ + BaCl$^+$) at low temperature by utilizing a hybrid atom-ion trapping system. The reaction rate and product branching fractions are measured and compared to model…

Ultracold temperatures in dilute quantum gases opened the way to an exquisite control of matter at the quantum level. Here we focus on the control of ultracold atomic collisions using a laser to engineer their interactions at large…

Quantum Gases · Physics 2022-02-23 T. Xie , A. Orbán , X. Xing , E. Luc-Koenig , R. Vexiau , O. Dulieu , N. Bouloufa-Maafa

We present a method to control collisions between ultracold neutral atoms in the electronic ground state and trapped ions. During the collision, the neutral atom is resonantly excited by a laser to a low-field-seeking Rydberg state, which…

Quantum Gases · Physics 2020-06-24 Limei Wang , Markus Deiß , Georg Raithel , Johannes Hecker Denschlag

The control of the ultracold collisions between neutral atoms is an extensive and successful field of study. The tools developed allow for ultracold chemical reactions to be managed using magnetic fields, light fields and spin-state…

Atomic Physics · Physics 2017-09-05 Tomas Sikorsky , Ziv Meir , Ruti Ben-shlomi , Nitzan Akerman , Roee Ozeri

Hybrid atom-ion systems are a rich and powerful platform for studying chemical reactions, as they feature both excellent control over the electronic state preparation and readout as well as a versatile tunability over the scattering energy,…

Calculations have been carried out for the vibrational quenching of excited H$_2$ molecules which collide with Li$^+$ ions at ultralow energies. The dynamics has been treated exactly using the well known quantum coupled-channel expansions…

Chemical Physics · Physics 2009-11-13 S. Bovino , E. Bodo , F. A. Gianturco

Intense laser-matter interactions are at the center of interest in research and technology since the development of high power lasers. They have been widely used for fundamental studies in atomic, molecular, and optical physics, and they…

Engineering atom-atom interactions is essential both for controlling novel phases of matter and for efficient preparation of many-body entangled states, which are key resources in quantum communication, computation, and metrology. In this…

Quantum Physics · Physics 2025-03-11 Sankalp Sharma , Jan Chwedeńczuk , Tomasz Wasak

Accurate \textit{ab initio} potential energy surfaces are essential to understand and predict collisional outcomes in ultracold molecular systems. In this study, we explore the intermolecular interactions between two laser-cooled CaF…

Atomic Physics · Physics 2025-11-12 Dibyendu Sardar , Marcin Gronowski , Michał Tomza , John L. Bohn

Great advances in precision quantum measurement have been achieved with trapped ions and atomic gases at the lowest possible temperatures. These successes have inspired ideas to merge the two systems. In this way one can study the unique…

Quantum Physics · Physics 2023-03-21 T. Feldker , H. Fürst , H. Hirzler , N. V. Ewald , M. Mazzanti , D. Wiater , M. Tomza , R. Gerritsma

We present a formalism for rigorous calculations of cross sections for inelastic and reactive collisions of ultracold atoms and molecules confined by laser fields in quasi-2D geometry. Our results show that the elastic-to-inelastic ratios…

Atomic Physics · Physics 2015-05-13 Zhiying Li , Roman V. Krems

Experimental setups that study laser-cooled ions immersed in baths of ultracold atoms merge the two exciting and well-established fields of quantum gases and trapped ions. These experiments benefit both from the exquisite read-out and…

Atomic Physics · Physics 2022-06-30 Rianne S. Lous , Rene Gerritsma

The laser excitation of an ion crystal to high lying and long-lived electronic states is a genuine many-body process even if in fact only a single ion is excited. This is a direct manifestation of the strong coupling between internal and…

Atomic Physics · Physics 2012-01-16 Weibin Li , Igor Lesanovsky

Pairs of free particles cannot form bound states in elastic collision due to momentum and energy conservation. In many ultracold experiments, however, the particles collide in the presence of an external trapping potential which can couple…

Atomic Physics · Physics 2023-11-17 Meirav Pinkas , Or Katz , Jonathan Wengrowicz , Nitzan Akerman , Roee Ozeri

Measurements of interactions between cold molecules and ultracold atoms can allow for a detailed understanding of fundamental collision processes. These measurements can be done using various experimental geometries including where both…

Atomic Physics · Physics 2020-03-25 N. J. Fitch , L. P. Parazzoli , H. J. Lewandowski

Ultracold atomic physics offers myriad possibilities to study strongly correlated many-body systems in lower dimensions. Typically, only ground state phases are accessible. Using a tunable quantum gas of bosonic cesium atoms, we realize and…

We propose a platform for observing and controlling the interactions between atomic ions and a quantum gas of polar molecules in the ultracold regime. This approach is based on the combination of several recently developed methods in two…

Atomic Physics · Physics 2025-06-26 Leon Karpa , Olivier Dulieu

Entanglement lies at the heart of quantum mechanics and in recent years has been identified as an essential resource for quantum information processing and computation. Creating highly entangled multi-particle states is therefore one of the…

Quantum Physics · Physics 2009-11-10 Olaf Mandel , Markus Greiner , Artur Widera , Tim Rom , Theodor W. Haensch , Immanuel Bloch

Collisions between ultracold calcium monohydroxide (CaOH) molecules are realized and studied. Inelastic collision rate constants are measured for CaOH prepared in ground and excited vibrational states, and the electric field dependence of…

Ultracold collisions of the polyatomic species CaOH are considered, in internal states where the collisions should be dominated by long-range dipole-dipole interactions. The computed rate constants suggest that evaporative cooling can be…

Chemical Physics · Physics 2019-06-25 Lucie D. Augustovičová , John L. Bohn
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