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Three-color coherent anti-Stokes Raman scattering represents non-degenerate four wave mixing process that includes both a non-resonant and resonant processes, the contributions of which depend on how the molecular vibrational modes are…

Optics · Physics 2020-10-14 Supriya Nagpal , Bryan Semon , Gombojav O. Ariunbold

We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Wellens , B. Gremaud , D. Delande , C. Miniatura

Statistical properties of light produced in spontaneous Raman scattering on an ensemble of molecules indicate the quantum nature of this phenomenon. The scattered light is non-classical and has high non-classical intensity correlations…

Optics · Physics 2026-05-15 Ivan V. Panyukov , Evgeny S. Andrianov

Quantum theoretical treatment of coherent forward scattering of light in a polarized atomic ensemble with an arbitrary angular momentum is developed. We consider coherent forward scattering of a weak radiation field interacting with a…

Quantum Physics · Physics 2007-05-23 D. V. Kupriyanov , O. S. Mishina , I. M. Sokolov , B. Julsgaard , E. S. Polzik

We present a scheme to obtain the coherently enhanced Raman scattering in atomic vapor which is induced by a spin wave initially written by a weak write laser. The enhancement of Raman scattering is dependent on the number and the spatial…

Quantum Physics · Physics 2015-05-19 Chun-Hua Yuan , L. Q. Chen , Jietai Jing , Z. Y. Ou , Weiping Zhang

We study Raman scattering in active media placed in proximity of different types of metal nanostructures, at wavelengths that display either Fabry-Perot or plasmonic resonances, or a combination of both. We use a semi-classical approach to…

Optics · Physics 2015-06-05 M. Scalora , M. A. Vincenti , D. de Ceglia , M. Grande , J. W. Haus

We present super-resolved coherent anti-Stokes Raman scattering (CARS) microscopy by implementing phase-resolved image scanning microscopy (ISM), achieving up to two-fold resolution increase as compared with a conventional CARS microscope.…

Optics · Physics 2024-11-22 Anna Zhitnitsky , Elad Benjamin , Ora Bitton , Dan Oron

We develop a computational framework to examine the factors responsible for scattering-induced distortions of coherent anti-Stokes Raman scattering (CARS) signals in turbid samples. We apply the Huygens-Fresnel Wave-based Electric Field…

Computational Physics · Physics 2020-12-18 Janaka C. Ranasinghesagara , Giuseppe de Vito , Vincenzo Piazza , Eric O. Potma , Vasan Venugopalan

The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…

Surface-enhanced coherent anti-Stokes Raman scattering (SE-CARS) takes advantage of surface plasmon resonances supported on metallic nanostructures to amplify the coherent Raman response of target molecules. While these metallic antennas…

Optics · Physics 2022-09-07 Shamsul Abedin , Yong Li , Abid Anjum Sifat , Khokan Roy , Eric Olaf Potma

Coherent backscattering is a coherence effect in the propagation of waves through disordered media involving two or more scattering events. Here, we report on the observation of coherent backscattering from individual atoms and their mirror…

We demonstrate coherent anti-Stokes Raman scattering (CARS) microscopy with 1089 foci, enabled by a high repetition rate amplified oscillator and optical parametric amplifier. We employ a camera as multichannel detector to acquire and…

Optics · Physics 2024-08-27 Dominykas Gudavicius , Lukas Kontenis , Wolfgang Langbein

Conventional femtosecond coherent laser spectroscopy predominantly focuses on the temporal phase coherence through time- or frequency-resolved methods. In this work, we suggest an alternative experimental framework based on spatial phase…

Spin-polarised atomic ensembles probed by light based on the Faraday interaction are a versatile platform for numerous applications in quantum metrology and quantum information processing. Here we consider an ensemble of Alkali atoms that…

Quantum Physics · Physics 2022-05-11 Alexander Roth , Klemens Hammerer , Kirill S. Tikhonov

Coherent effects manifested in light scattering from cold, optically dense and disordered atomic systems are reviewed from a primarily theoretical point of view. Development of the basic theoretical tools is then elaborated through several…

Quantum Physics · Physics 2017-12-15 D. V. Kupriyanov , I. M. Sokolov , M. D. Havey

Resonant inelastic (Raman) light scattering off neutral GaAs quantum dots which contain a mean number, N=42, of electron-hole pairs is computed. We find Raman amplitudes corresponding to strongly collective final states (charge-density…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Alain Delgado , Augusto Gonzalez , Eduardo Menendez-Proupin

The recent observations of the coherent neutrino- and antineutrino-nucleus scattering have opened up a plethora of opportunities to probe physics within standard and non-standard theories of the electroweak interactions. In the present…

High Energy Physics - Phenomenology · Physics 2026-01-01 T. S. Kosmas , R. Sahu , V. K. B. Kota

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

We apply coherent anti-Stokes Raman Scattering (CARS) microscopy to characterize director structures in liquid crystals.

Soft Condensed Matter · Physics 2016-09-08 A. V. Kachynski , A. N. Kuzmin , P. N. Prasad , I. I. Smalyukh

Coherent Raman scattering microscopy is a fast, label-free and chemically specific imaging technique that has a high potential for future in-vivo optical histology. However, its imaging depth into tissues is limited to the sub-millimeter…