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Intermolecular correlations in liquid acetonitrile (CH3CN) have been revisited by calculating orientational correlation functions. In the present approach, hydrogen atoms are included, so that a concept applicable for molecules of (nearly)…

Chemical Physics · Physics 2019-06-12 Szilvia Pothoczki , László Pusztai

Laser pulses with stable electric field waveforms establish the opportunity to achieve coherent control on attosecond timescales. We present experimental and theoretical results on the steering of electronic motion in a multi-electron…

Electrons in atoms and molecules move on attosecond time scales. Deciphering their quantum dynamics in space and time calls for high-resolution microscopy at this speed. While scanning tunnelling microscopy (STM) driven with terahertz…

We investigate theoretically the relative time delay of photoelectrons originating from the different subshells (2s and 2p) of neon. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…

Atomic Physics · Physics 2017-02-15 J. Wätzel , A. S. Moskalenko , Y. Pavlyukh , J. Berakdar

Current and next-generation particle tracking detectors will incorporate precision timing capabilities with resolutions approaching tens of picoseconds. Using Technology Computer-Aided Design (TCAD) simulations of Low-Gain Avalanche Diode…

A numerical model based on hydrodynamic approach has been developed to emulate the device dynamics of active target Time Projection Chamber which is utilized for studying nuclear reaction through three dimensional tracking of concerned low…

Instrumentation and Detectors · Physics 2025-06-03 Pralay Kumar Das , Jaydeep Datta , Nayana Majumdar , Supratik Mukhopadhyay

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

Atomic Physics · Physics 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

This article explains and illustrates the use of a set of coupled dynamical equations, second order in a fictitious time, which converges to solutions of stationary Schr\"{o}dinger equations with additional constraints. We include three…

Computational Physics · Physics 2020-10-21 M. Ogren , M. Gulliksson

Attochemistry aims to exploit the properties of coherent electronic wavepackets excited via attosecond pulses, to control the formation of photoproducts. Such molecular processes can in principle be simulated with various nonadiabatic…

Chemical Physics · Physics 2024-05-28 Thierry Tran , Anthony Ferté , Morgane Vacher

In order to elucidate the correlated motion of atomic electrons, we investigate the attosecond-scale dynamics of their entanglement arising due to nonsequential ionization driven by a strong, linearly-polarized laser field. The calculation…

Atomic Physics · Physics 2024-03-18 Daniel Younis , Songbo Xie , Joseph H. Eberly

We investigate the tagged-particle motion in a strongly interacting quasi-confined liquid using periodic boundary conditions along the confining direction. Within a mode-coupling theory of the glass transition (MCT) we calculate the…

Soft Condensed Matter · Physics 2021-09-14 Lukas Schrack , Charlotte F. Petersen , Michele Caraglio , Gerhard Jung , Thomas Franosch

We consider a simple model of lossless interaction between a two-level single atom and a standing-wave single-mode laser field which creates a one-dimensional optical lattice. Internal dynamics of the atom is governed by the laser field…

Quantum Physics · Physics 2011-11-09 V. Yu. Argonov , S. V. Prants

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…

Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…

Atomic Physics · Physics 2016-10-03 Jonas Wätzel , Jamal Berakdar

We use molecular dynamics to study the ordering of a nematic liquid crystal around a spherical particle or droplet. Homeotropic boundary conditions and strong anchoring create a hedgehog director configuration on the particle surface and in…

Soft Condensed Matter · Physics 2013-03-19 D. Andrienko , G. Germano , M. P. Allen

Experiments and numerical simulations are described that develop quantitative understanding of atomic motion near the surfaces of nanoscopic photonic crystal waveguides (PCWs). Ultracold atoms are delivered from a moving optical lattice…

Quantum Physics · Physics 2019-03-06 A. P. Burgers , L. S. Peng , J. A. Muniz , A. C. McClung , M. J. Martin , H. J. Kimble

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

We use three dimensional time-dependent Schr\"odinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous…

Atomic Physics · Physics 2013-06-26 M. F. Ciappina , J. A. Pérez-Hernández , T. Shaaran , L. Roso , M. Lewenstein

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…

Atomic Physics · Physics 2015-10-28 Lukas Medišauskas , Jack Wragg , Hugo van der Haart , Misha Yu. Ivanov
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