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In this short note, we report on the first inelastic neutron scattering (INS) study on high-energy magnetic excitations in Sr$_3$Ir$_2$O$_7$. We observed excitations between $\sim$80 meV and $\sim$180 meV. The peak position of the…

Strongly Correlated Electrons · Physics 2021-01-12 Masaki Fujita , Kazuhiko Ikeuchi , Ryoichi Kajimoto , Mitsutaka Nakamura

We theoretically investigate spin dynamics and $L_3$-edge resonant inelastic X-ray scattering (RIXS) of Chromium with commensurate spin-density wave (SDW) order, based on a multi-band Hubbard model composed of 3$d$ and 4$s$ orbitals.…

Strongly Correlated Electrons · Physics 2013-04-24 Koudai Sugimoto , Zhi Li , Eiji Kaneshita , Kenji Tsutsui , Takami Tohyama

We investigate the Cu $L_3$ edge resonant inelastic x-ray scattering (RIXS) spectra of a quasi-1D antiferromagnet Ca$_2$CuO$_3$. In addition to the magnetic excitations, which are well-described by the two-spinon continuum, we observe two…

Using Raman spectroscopy to study the correlated 4$d$-electron metal Sr$_2$RhO$_4$, we observe pronounced excitations at 220 meV and 240 meV with $A_\mathrm{1g}$ and $B_\mathrm{1g}$ symmetries, respectively. We identify them as transitions…

The strongly correlated insulator Ca$_{2}$RuO$_4$ is considered as a paradigmatic realization of both spin-orbital physics and a band-Mott insulating phase, characterized by orbitally selective coexistence of a band and a Mott gap. We…

One of the most intensely studied scenarios of high-temperature superconductivity (HTS) postulates pairing by exchange of magnetic excitations [1]. Indeed, such excitations have been observed up to around optimal doping in the cuprates…

Motivated by RIXS experiments on a wide range of complex heavy oxides, including rhenates, osmates, and iridates, we discuss the theory of RIXS for site-localized $t_{2g}$ orbital systems with strong spin-orbit coupling. For such systems,…

Strongly Correlated Electrons · Physics 2018-06-20 Arun Paramekanti , David J. Singh , Bo Yuan , Diego Casa , Ayman Said , Young-June Kim , Andrew D. Christianson

Resonant inelastic X-ray scattering (RIXS) experiments performed at the oxygen-$K$ edge on the iridate perovskites {\SIOS} and {\SION} reveal a sequence of well-defined dispersive modes over the energy range up to $\sim 0.8$ eV. The…

Transition-metal ions with $5d^2$ electronic configuration in a cubic crystal field are prone to have a vanishing dipolar magnetic moment but finite higher-order multipolar moments, and they are expected to exhibit exotic physical…

Strongly Correlated Electrons · Physics 2025-07-16 J. Okamoto , G. Shibata , Yu. S. Posonov , H. Hayashi , K. Yamaura , H. Y. Huang , A. Singh , C. T. Chen , A. Tanaka , S. V. Streltsov , D. J. Huang , A. Fujimori

We investigate magnetic excitations in the spin-ladder compound Sr$_{14}$Cu$_{24}$O$_{41}$ using high-resolution Cu $L_3$-edge Resonant Inelastic X-ray Scattering (RIXS). Our findings demonstrate that RIXS couples to collective spin…

Recent experiments on La$_2$CuO$_4$ suggest that indirect resonant inelastic X-ray scattering (RIXS) might provide a probe for transversal spin dynamics. We present in detail a systematic expansion of the relevant magnetic RIXS cross…

Strongly Correlated Electrons · Physics 2011-07-22 Filomena Forte , Luuk J. P. Ament , Jeroen van den Brink

Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

Strongly Correlated Electrons · Physics 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

In the rich phases of van der Waals (vdW) materials featuring intertwined electronic order and collective phenomena, characterizing elementary dynamics that entail the low-energy Hamiltonian and electronic degrees of freedom is of paramount…

Low-energy electron excitation spectra were measured on a single crystal of a typical iron-based superconductor PrFeAsO$_{0.7}$ using resonant inelastic X-ray scattering (RIXS) at the Fe-$L_3$ edge. Characteristic RIXS features are clearly…

Strongly Correlated Electrons · Physics 2016-07-18 T. Nomura , Y. Harada , H. Niwa , K. Ishii , M. Ishikado , S. Shamoto , I. Jarrige

We use resonant inelastic x-ray scattering (RIXS) at the Cu L$_3$ edge to measure the charge and spin excitations in the "half-stuffed" Cu--O planes of the cuprate antiferromagnet Ba$_2$Cu$_3$O$_4$Cl$_2$. The RIXS line shape reveals…

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

We present a combined oxygen $K$-edge x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) study of the bilayer ruthenate Ca$_3$Ru$_2$O$_7$. Our RIXS experiments on Ca$_3$Ru$_2$O$_7$ were carried out on the…

Strongly Correlated Electrons · Physics 2025-04-01 K. von Arx , F. Forte , M. Horio , V. Granata , Q. Wang , L. Das , Y. Sassa , R. Fittipaldi , C. G. Fatuzzo , O. Ivashko , Y. Tseng , E. Paris , A. Vecchione , T. Schmitt , M. Cuoco , J. Chang

We present a theory of the resonant inelastic x-ray scattering (RIXS) to study electronic excitations in orbital ordered manganites. The charge and orbital excitations of the Mn 3d electron are caused by the Coulomb interactions in the…

Strongly Correlated Electrons · Physics 2009-10-31 H. Kondo , S. Ishihara , S. Maekawa

We present a resonant inelastic x-ray scattering (RIXS) study of spin and charge excitations in overdoped La1.77Sr0.23CuO4 along two high-symmetry directions. The line shape of these excitations is analyzed and they are shown to be highly…

Superconductivity · Physics 2016-02-05 C. Monney , T. Schmitt , C. E. Matt , J. Mesot , V. N. Strocov , O. J. Lipscombe , S. M. Hayden , J. Chang