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Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…

YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…

Strongly Correlated Electrons · Physics 2015-10-20 Yuesheng Li , Gang Chen , Wei Tong , Li Pi , Juanjuan Liu , Zhaorong Yang , Xiaoqun Wang , Qingming Zhang

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

Strongly Correlated Electrons · Physics 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

We present a nuclear magnetic resonance (NMR) and electron spin resonance (ESR) study of rare-earth titanates derived from the spin-1/2 Mott insulator YTiO$_3$. Measurements of single-crystalline samples of (Y,Ca,La)TiO$_3$ in a wide range…

Strongly Correlated Electrons · Physics 2024-05-10 Ana Najev , Sajna Hameed , Alexey Alfonsov , Joseph Joe , Vladislav Kataev , Martin Greven , Miroslav Požek , Damjan Pelc

We investigate the electron-spin resonance (ESR) phenomenon in the heavy-fermion metal YbRh2Si2 by applying hydrostatic pressure up to 3 GPa and by inducing internal pressure on the Yb site chemically in Yb(Rh1-xCox)2Si2 samples. We found…

We present a neutron diffraction study of NaYbO$_2$, a candidate quantum spin liquid compound hosting a geometrically frustrated triangular lattice of magnetic Yb$^{3+}$ ions. We observe diffuse magnetic scattering that persists to at least…

We report an electron spin resonance (ESR) study of the s=1/2-Heisenberg pseudo-ladder magnet CaCu2O3 in pulsed magnetic fields up to 40 T. At sub-Terahertz frequencies we observe an ESR signal originating from a small amount of…

Strongly Correlated Electrons · Physics 2009-11-11 M. Goiran , M. Costes , J. M. Broto , F. C. Chou , R. Klingeler , E. Arushanov , S. -L. Drechsler , B. Büchner , V. Kataev

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

Strongly Correlated Electrons · Physics 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with…

Strongly Correlated Electrons · Physics 2009-08-04 L. M. Holanda , J. M. Vargas , C. Rettori , S. Nakatsuji , K. Kuga , Z. Fisk , S. B. Oseroff , P. G. Pagliuso

We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but…

Strongly Correlated Electrons · Physics 2015-03-18 K. Yu. Povarov , A. I. Smirnov , O. A. Starykh , S. V. Petrov , A. Ya. Shapiro

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

We investigate the electron and nuclear spin coherence properties of ytterbium ($\mathrm{Yb}^{3+}$) ions with non-zero nuclear spin, within an yttrium orthosilicate (Y$_2$SiO$_5$) crystal, with a view to their potential application in…

Quantum Physics · Physics 2019-08-06 Hee-Jin Lim , Sacha Welinski , Alban Ferrier , Philippe Goldner , J. J. L. Morton

The Heisenberg triangular lattice quantum spin liquid and the phase transitions to nearby magnetic orders have received much theoretical attention, but clear experimental manifestations of these states are rare. This work investigates a new…

The electronic structure of a quantum spin liquid compound, EtMe3Sb[Pd(dmit)2]2, has been studied with angle-resolved photoemission spectroscopy, together with two other Pd(dmit)2 salts in the valence bond solid or antiferromagnetic state.…

Strongly Correlated Electrons · Physics 2015-06-15 Q. Q. Ge , H. C. Xu , X. P. Shen , M. Xia , B. P. Xie , F. Chen , Y. Zhang , R. Kato , T. Tsumuraya , T. Miyazaki , M. Matsunami , S. Kimura , D. L. Feng

We study the electron spin resonance (ESR) of low-dimensional spin systems at high temperature, and test the Kubo-Tomita theory of exchange narrowing. In finite-size systems (molecular magnets), we found a double-peak resonance which…

Strongly Correlated Electrons · Physics 2015-05-18 S. El Shawish , O. Cepas , S. Miyashita

A multi-frequency electron spin resonance (ESR) study provides evidence for the occurrence of low temperature ferromagnetic/spin-glass behavior in aligned arrays of sub-nanometer single walled carbon nanotubes confined in zeolite…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 S. S. Rao , A. Stesmans , J. V. Noyen , P. Jacobs , B. Sels

High-field electron spin resonance (ESR) measurements have been performed on vesignieite BaCu$_3$V$_2$O$_8$(OH)$_2$, which is considered as a nearly ideal model substance of $S$=1/2 kagome antiferromagnet, in the temperature region from 1.9…

An electron spin resonance (ESR) study of the heavy fermion compound YbRh2Si2 for fields up to ~ 8 T reveals a strongly anisotropic signal below the single ion Kondo temperature T_K ~ 25 K. A remarkable similarity between the T-dependence…

Strongly Correlated Electrons · Physics 2009-11-13 U. Schaufuß , V. Kataev , A. A. Zvyagin , B. Büchner , J. Sichelschmidt , J. Wykhoff , C. Krellner , C. Geibel , F. Steglich

We have investigated the electron spin resonance (ESR) on single crystals of BaCu$\_2$Ge$\_2$O$\_7$ at temperatures between 300 and 2 K and in a large frequency band, 9.6 -134 GHz, in order to test the predictions of a recent theory,…

Strongly Correlated Electrons · Physics 2007-05-23 Sylvain Bertaina , V. A. Pashchenko , Anatoli Stepanov , T. Masuda , K. Uchinokura