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Related papers: Ferromagnetic van der Waals crystal VI3

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We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 by specific heat and magnetization measurements of single crystals in high magnetic fields and by ab initio density functional theory calculations…

We report a comprehensive investigation of the lattice and magnetic structure in van der Waals antiferromagnet VBr3, characterized by a BiI3-type structure at room temperature. Neutron diffraction experiments were performed on both…

Strongly Correlated Electrons · Physics 2024-08-06 Yimeng Gu , Yiqing Hao , Zeyu Kao , Yiqing Gu , Feiyang Liu , Shiyi Zheng , Huibo Cao , Lunhua He , Jun Zhao

The van der Waals ferromagnet (FM), VI$_3$, was studied by muon spin relaxation ($\mu^+$SR) and first principle calculations based on density functional theory (DFT). Temperature dependent zero field muon spin relaxation ($\mu^+$SR)…

Strongly Correlated Electrons · Physics 2022-11-01 Ola Kenji Forslund , Yuqing Ge , Hiroto Ohta , Chennan Wang , Mahmoud Abdel-Hafiez , Jun Sugiyama , Martin Månsson , Yasmine Sassa

We present the observation of an isostructural Mott insulator-metal transition in van-der-Waals honeycomb antiferromagnet V$_{0.9}$PS$_3$ through high-pressure x-ray diffraction and transport measurements. The MPX$_3$ family of magnetic…

Strongly Correlated Electrons · Physics 2019-03-27 M. J. Coak , S. Son , D. Daisenberger , H. Hamidov , C. R. S. Haines , P. L. Alireza , A. R. Wildes , C. Liu , S. S. Saxena , J. -G. Park

Recent discoveries of intrinsic two-dimensional (2D) ferromagnetism in insulating/semiconducting van der Waals (vdW) crystals open up new possibilities for studying fundamental 2D magnetism and devices employing localized spins. However, a…

Van der Waals (vdW) Dirac magnon system CrI$_3$, a potential host of topological edge magnons, orders ferromagnetically (FM) (T$_C=61$ K) in the bulk, but antiferromagnetic (AFM) order has been observed in nanometer thick flakes, attributed…

Materials Science · Physics 2024-05-14 John A. Schneeloch , Luke Daemen , Despina Louca

The discovery of ordered magnetism in two-dimensional van der Waals materials at the monolayer limit challenges the Mermin-Wagner theorem, which forbids spontaneous breaking of continuous symmetries in two dimensions at finite temperatures.…

Van der Waals (vdW) heterostructures have attracted great interest because of their rich material combinations.The discovery of two-dimensional magnets has provided a new platform for magnetic vdW heterointerfaces; however, research on…

Ferromagnetic van der Waals (vdW) materials are in demand for spintronic devices with all-two-dimensional-materials heterostructures. Here, we demonstrate mechanical exfoliation of magnetic-atom-intercalated transition metal dichalcogenide…

Mesoscale and Nanoscale Physics · Physics 2017-09-26 Yuji Yamasaki , Rai Moriya , Miho Arai , Satoru Masubuchi , Sunseng Pyon , Tsuyoshi Tamegai , Keiji Ueno , Tomoki Machida

CrI3 is a two-dimensional ferromagnetic van der Waals material with a charge gap of 1.1-1.2 eV. In this study, the electronic structure and magnetism of CrI3 are investigated by using density functional theory and dynamical mean-field…

Strongly Correlated Electrons · Physics 2022-04-27 Tianye Yu , Rui Liu , Huican Mao , Xiaobo Ma , Guangwei Wang , Zhihong Yuan , Pengyu Zheng , Yiran Peng , Zhiping Yin

Since the celebrated discovery of graphene, the family of two-dimensional (2D) materials has grown to encompass a broad range of electronic properties. Recent additions include spin-valley coupled semiconductors, Ising superconductors that…

Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

Materials Science · Physics 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

To broaden the scope of van der Waals 2D magnets, we report the synthesis and magnetism of covalent 2D magnetic Cr$_2$Te$_3$ with a thickness down to one-unit-cell. The 2D Cr$_2$Te$_3$ crystals exhibit robust ferromagnetism with a Curie…

Magnetism in two-dimensional (2D) materials has attracted considerable attention recently for both fundamental understanding of magnetism and their tunability towards device applications. The isostructural Fe$_3$GeTe$_2$ and Fe$_3$GaTe$_2$…

VI$_{3}$ is a ferromagnet with planar honeycomb sheets of bonded V$^{3+}$ ions held together by van der Waals forces. We apply neutron spectroscopy to measure the two dimensional ($J/J_{c} \approx 17$) magnetic excitations in the…

Strongly Correlated Electrons · Physics 2021-07-23 H. Lane , E. Pachoud , J. A. Rodriguez-Rivera , M. Songvilay , G. Xu , P. M. Gehring , J. P. Attfield , R. A. Ewings , C. Stock

The synthesis, structural, magnetic, thermal and transport properties are reported for polycrystalline PrIr3. At room temperature PrIr3 displays the rhombohedral space group R-3m and a PuNi3- type structure. At around 70 K a phase…

Two-dimensional (2D) materials with robust magnetism have drawn immense attention for their promising applications in spintronics. Recently, intrinsic ferromagnetic vanadium triiodide (VI3) has been synthesized experimentally. To enhance…

Materials Science · Physics 2021-09-28 Charles Sun , Xuan Luo

The van der Waals ferromagnet Fe$_3$GeTe$_2$ has recently attracted extensive research attention due to its intertwined magnetic, electronic and topological properties. Here, using high-resolution angle-resolved photoemission spectroscopy,…

When combined with transition metals with partially filled $d$-orbitals, magnetism can be incorporated in two-dimensional materials, which greatly expands the scope for fundamental researches and potential applications of these materials.…

Materials Science · Physics 2019-12-24 Ming An , Yang Zhang , Jun Chen , Hui-Min Zhang , Yunjun Guo , Shuai Dong

Van der Waals (vdW) magnet heterostructures have emerged as new platforms to explore exotic magnetic orders and quantum phenomena. Here, we study heterostructures of layered antiferromagnets, CrI3 and CrCl3, with perpendicular and in-plane…