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We investigated the temperature-dependent evolution of the electronic structure of the Jeff,1/2 Mott insulator Sr2IrO4 using optical spectroscopy. The optical conductivity spectra $\sigma(\omega)$ of this compound has recently been found to…

Strongly Correlated Electrons · Physics 2009-10-23 S. J. Moon , Hosub Jin , W. S. Choi , J. S. Lee , S. S. A. Seo , J. Yu , G. Cao , T. W. Noh , Y. S. Lee

We performed Raman spectroscopy measurements under temperature changes from 10 K up to 850 K to probe the phonon-spin coupling in Y$_2$NiMnO$_6$. The spin-phonon coupling was observed as a softening of the stretching mode, indicating this…

We perform a time-resolved optical study of Sr$_2$IrO$_4$ to understand the influence of magnetic ordering on the low energy electronic structure of a strongly spin-orbit coupled $J_{eff}$=1/2 Mott insulator. By studying the recovery…

Strongly Correlated Electrons · Physics 2012-03-21 D. Hsieh , F. Mahmood , D. H. Torchinsky , G. Cao , N. Gedik

We report inelastic light scattering experiments on CaFe_2As_2 in the temperature range of 4 to 290 K. In in-plane polarizations two Raman-active phonon modes are observed at 189 and 211 cm-1, displaying A_1g and B_1g symmetries,…

Superconductivity · Physics 2009-11-13 K. -Y. Choi , D. Wulferding , P. Lemmens , N. Ni , S. L. Bud'ko , P. C. Canfield

Magnon-polarons, a type of hybridized excitations between magnons and phonons, were first reported in yttrium iron garnet as anomalies in the spin Seebeck effect responses. Here we report an observation of antiferromagnetic (AFM)…

Using infrared (IR) and Raman spectroscopies combined with high-resolution x-ray diffraction, we address several controversial aspects of altermagnetic $\alpha$-MnTe. We show that mechanical stress applied to crystals of this material…

By means of neutron inelastic scattering, magnetic excitations and phonons were measured for a single crystal of slightly overdoped superconductor Ca10Pt4As8(Fe1-xPtxAs)10 (x ~ 0.2) with the transition temperature Tc of ~33 K. Below Tc,…

We studied magneto-optical response of a canonical topological insulator Bi$_2$Se$_3$ with the goal of addressing a controversial issue of electron-phonon coupling. Magnetic-field induced modifications of reflectance are very pronounced in…

Strongly Correlated Electrons · Physics 2016-10-12 S. V. Dordevic , G. M. Foster , M. S. Wolf , N. Stojilovic , H. Lei , C. Petrovic , Z. Chen , Z. Q. Li , L. C. Tung

The crystal lattice of Sr$_2$IrO$_4$ is investigated with synchrotron X-ray powder diffraction under hydrostatic pressures up to $P=43$ GPa and temperatures down to $20$ K. The tetragonal unit cell is maintained over the whole investigated…

Strongly Correlated Electrons · Physics 2020-02-26 K. Samanta , R. Tartaglia , U. F. Kaneko , N. M. Souza-Neto , E. Granado

We present and analyze Raman spectra of the Mott insulator Ca$_2$RuO$_4$, whose quasi-two-dimensional antiferromagnetic order has been described as a condensate of low-lying spin-orbit excitons with angular momentum $J_{eff}=1$. In the…

We consider the implications of spin-phonon coupling within the slave-boson, mean-field treatment of the extended t-J model of a high-temperature superconductor. In bilayer cuprates such as YBaCuO, where the $CuO_2$ plane is buckled, this…

Condensed Matter · Physics 2009-10-28 B. Normand , H. Kohno , H. Fukuyama

In this work we study phonon-phonon coupling in bismuth vanadate (BiVO4), known for its second-order transition involving a variety of coupling mechanisms. Using Raman spectroscopy as a probe, we identify two optical coupled phonon modes of…

Materials Science · Physics 2023-06-09 Christina Hill , Georgy Gordeev , Mael Guennou

Sr2IrO4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr2Ir1-xFexO4 (0<x<0.32) and Sr2Ir1-xCoxO4 (0<x<0.22). Fe doping retains the…

Strongly Correlated Electrons · Physics 2020-12-21 Bing Hu , Hengdi Zhao , Yu Zhang , Pedro Schlottmann , Feng Ye , Gang Cao

We report an inelastic light scattering study of single-crystalline NaCu$_2$O$_2$, a spin-chain compound known to exhibit a phase with helical magnetic order at low temperatures. Phonon excitations were studied as a function of temperature…

Strongly Correlated Electrons · Physics 2009-11-11 K. -Y. Choi , V. P. Gnezdilov , P. Lemmens , L. Capogna , M. R. Johnson , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

(Sr$_{2}$,Ba$_{2}$)Cu$_{3}$O$_{4}$Cl$_{2}$ are antiferromagnetic insulators which are akin to the parent compounds of the cuprate superconductors but with two distinct magnetic ordering temperatures related to two magnetic Cu$_{I}$ and…

Strongly Correlated Electrons · Physics 2009-02-13 J. Holmlund , C. S. Knee , J. Andreasson , M. Granath , A. P. Litvinchuk , L. Borjesson

An experimental study of optical phonon modes, both normal and interface (IF) phonons, in bilayer strain-coupled InAs/GaAs_(1-x)Sb_x quantum dot heterostructures has been presented by means of low-temperature polarized Raman scattering. The…

Mesoscale and Nanoscale Physics · Physics 2024-09-17 Priyesh Kumar , Sudip Kumar Deb , Subhananda Chakrabarti , Jhuma Saha

We report results on the electrodynamic response of $TiOCl$, a low-dimensional spin-1/2 quantum magnet that shows a spin gap formation for T$<T_{c1}$= 67 $K$. The Fano-like shape of a few selected infrared active phonons suggests an…

Strongly Correlated Electrons · Physics 2009-11-10 G. Caimi , L. Degiorgi , N. N. Kovaleva , P. Lemmens , F. C. Chou

We study interaction between two magnetic impurities on top of a two dimensional insulator in the presence of chiral phonons by second-order perturbation theory. We show that this exchange interaction arises from angular momentum of phonons…

Mesoscale and Nanoscale Physics · Physics 2025-10-13 Takehito Yokoyama

In this letter we investigated the temperature-dependent Raman spectra of CaMn7O12 helimagnet from room temperature down to 10 K. The temperature dependence of the Raman mode parameters show remarkable anomalies for both antiferromagnetic…

The doping dependence of the micro-Raman spectra of high quality La_{2-x}Sr_xCuO_4 microcrystals with x=0.0-0.45 has been investigated in the region 10-300 K. The phonon at ~100 cm^{-1} of the orthorhombic phase shows a classical soft mode…

Superconductivity · Physics 2009-11-13 D. Lampakis , E. Liarokapis , C. Panagopoulos