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Chemical short-range order (SRO) provides new opportunities for tuning alloy properties, but conventional computational thermodynamics frameworks such as CALPHAD, based on Bragg-Williams mean-field approximations, cannot properly describe…

Materials Science · Physics 2025-08-12 Chuliang Fu

Tailoring the performance of next-generation high entropy materials requires a deep understanding of the competition between entropy-driven random solid solution and enthalpy-driven chemical ordering. Investigating such order and disorder…

Materials Science · Physics 2026-03-24 Fanli Zhou , Hao Chen , Pengxiang Xu , Kai Yang , Zongrui Pei , Xianglin Liu

In many concentrated alloys of current interest, the observation of diffuse superlattice intensities by transmission electron microscopy has been attributed to chemical short-range order. We briefly review these findings and comment on the…

Materials Science · Physics 2023-08-23 Flynn Walsh , Mingwei Zhang , Robert O. Ritchie , Andrew M. Minor , Mark Asta

The growth and microstructural properties of ternary monolayers of two-dimensional hexagonal materials are examined, including both individual two-dimensional crystalline grains and in-plane heterostructures, multijunctions, or…

Materials Science · Physics 2022-07-06 Zhi-Feng Huang

The unusual correlated state that emerges in URu$_2$Si$_2$ below T$_{HO}$ = 17.5 K is known as "hidden order" because even basic characteristics of the order parameter, such as its dimensionality (whether it has one component or two), are…

Strongly Correlated Electrons · Physics 2020-03-12 Sayak Ghosh , Michael Matty , Ryan Baumbach , Eric D. Bauer , K. A. Modic , Arkady Shekhter , J. A. Mydosh , Eun-Ah Kim , B. J. Ramshaw

Analysis of nanoscale short-range chemical and/or structural order via (scanning) transmission electron microscopy (S/TEM) imaging is fundamentally limited by projection of the three dimensional sample, which averages informational along…

Materials Science · Physics 2022-08-25 Michael Xu , Abinash Kumar , James M. LeBeau

The atomic structure of Ni64.5Zr35.5 metallic glass has been investigated by molecular dynamics (MD) simulations. The calculated structure factors from the MD glassy sample at room temperature agree well with the X-ray diffraction (XRD) and…

Mesoscale and Nanoscale Physics · Physics 2018-03-14 Ling Tang , Tongqi Wen , Nan Wang , Yang Sun , Feng Zhang , Zejin Yang , Kai-Ming Ho , Cai-Zhuang Wang

We present theoretical study of ordering phenomena in binary $C_{1-x}B_{x}$, $C_{1-x}N_{x}$ and ternary $B_{x}C_{1-x-y}N_{y}$ alloys forming two-dimensional, graphene-like systems. For calculating energy of big systems (20 000 atoms in the…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 Agnieszka Jamróz , Jacek A. Majewski

We study the phase behaviour of the Al$_x$CrFeCoNi high-entropy alloy. Our approach is based on a perturbative analysis of the internal energy of the paramagnetic solid solution as evaluated within the Korringa-Kohn-Rostoker formulation of…

Materials Science · Physics 2024-12-02 Christopher D. Woodgate , George A. Marchant , Livia B. Pártay , Julie B. Staunton

Due to the lack of long-range order, it remains challenging to characterize the structure of disordered solids and understand the nature of the glass transition. Here we propose a new structural order parameter by taking into account…

Soft Condensed Matter · Physics 2024-08-26 Ding Xu , Qinyi Liao , Ning Xu

We have used density functional theory to study the structural stability of surface alloys. Our systems consist of a single pseudomorphic layer of $M_xN_{1-x}$ on the Ru(0001) surface, where $M$ = Fe or Co, and $N$ = Pt, Au, Ag, Cd, or Pb.…

Materials Science · Physics 2009-11-13 Madhura Marathe , Mighfar Imam , Shobhana Narasimhan

Crystals are a state of matter characterised by periodic order. Yet crystalline materials can harbour disorder in many guises, such as non-repeating variations in composition, atom displacements, bonding arrangements, molecular…

Materials Science · Physics 2019-12-03 Arkadiy Simonov , Andrew L. Goodwin

Chemical short-range order (CSRO) is believed to be a key contributor to the exceptional properties of multicomponent alloys. However, direct validation and confirmation of CSRO has been highly elusive in most compounds. Recent studies for…

Materials Science · Physics 2022-11-11 A. Naghdi , F. J. Dominguez-Gutierrez , W. Y. Huo , K. Karimi , S. Papanikolaou

The degree of randomness, or partial order, present in two-dimensional supramolecular arrays of isophthalate tetracarboxylic acids is shown to vary due to subtle chemical changes such as the choice of solvent or small differences in…

Ni-W based medium heavy alloys offer a promising pathway to bridge the density-strength gap between tungsten heavy alloys and ultrahigh-strength steels. In this study, the effects of W concentration on short-range order (SRO), deformation…

Since the discovery of charge disproportionation in the FeO$_2$ square-lattice compound Sr$_3$Fe$_2$O$_7$ by M\"ossbauer spectroscopy more than fifty years ago, the spatial ordering pattern of the disproportionated charges has remained…

Many systems in nature and the synthetic world involve ordered arrangements of units on two-dimensional surfaces. We review here the fundamental role payed by both the topology of the underlying surface and its detailed curvature. Topology…

Soft Condensed Matter · Physics 2009-07-31 Mark J. Bowick , Luca Giomi

Magnetic high entropy alloys (HEAs) are a new category of high-performance magnetic materials, with multi-component concentrated compositions and complex multi-phase structures. Although there have been numerous reports of their interesting…

Whereas exceptional mechanical and radiation performances have been found in the emergent medium- and high-entropy alloys (MEAs and HEAs), the importance of their complex atomic environment, reflecting diversity in atomic size and…

Materials Science · Physics 2019-02-26 Yang Tong , Shijun Zhao , Hongbin Bei , Takeshi Egami , Yanwen Zhang , Fuxiang Zhang

Complexity in materials often arises from competing interactions at the atomic length scale. One such example are the strongly correlated heavy-fermion materials where the competition between Kondo screening and antiferromagnetic ordering…

Strongly Correlated Electrons · Physics 2015-05-18 Jeremy Figgins , Dirk K. Morr